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Using Resonances to Control Chaotic Mixing within a Translating and Rotating Droplet

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 Added by Rodolphe Chabreyrie
 Publication date 2009
  fields Physics
and research's language is English




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Enhancing and controlling chaotic advection or chaotic mixing within liquid droplets is crucial for a variety of applications including digital microfluidic devices which use microscopic ``discrete fluid volumes (droplets) as microreactors. In this work, we consider the Stokes flow of a translating spherical liquid droplet which we perturb by imposing a time-periodic rigid-body rotation. Using the tools of dynamical systems, we have shown in previous work that the rotation not only leads to one or more three-dimensional chaotic mixing regions, in which mixing occurs through the stretching and folding of material lines, but also offers the possibility of controlling both the size and the location of chaotic mixing within the drop. Such a control was achieved through appropriate tuning of the amplitude and frequency of the rotation in order to use resonances between the natural frequencies of the system and those of the external forcing. In this paper, we study the influence of the orientation of the rotation axis on the chaotic mixing zones as a third parameter, as well as propose an experimental set up to implement the techniques discussed.



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The design of strategies to generate efficient mixing is crucial for a variety of applications, particularly digital microfluidic devices that use small discrete fluid volumes (droplets) as fluid carriers and microreactors. In recent work, we have presented an approach for the generation and control of mixing inside a translating spherical droplet. This was accomplished by considering Stokes flow within a droplet proceeding downstream to which we have superimposed time dependent (sinusoidal) rotation. The mixing obtained is the result of the stretching and folding of material lines which increase exponentially the surface contact between reagents. The mixing strategy relies on the generation of resonances between the steady and the unsteady part of the flow, which is achieved by tuning the parameters of the periodic rotation. Such resonances, in our system, offer the possibility of controlling both the location and the size of the mixing region within the droplet, which may be useful to manufacture inhomogeneous particles (such as Janus particles). While the period and amplitude of the periodic rotation play a major role, it is shown here by using a triangular function that the particular shape of the rotation (as a function of time) has a minor influence. This finding demonstrates the robustness of the proposed mixing strategy, a crucial point for its experimental realization.
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We consider the rotating and translating equilibria of open finite vortex sheets with endpoints in two-dimensional potential flows. New results are obtained concerning the stability of these equilibrium configurations which complement analogous results known for unbounded, periodic and circular vortex sheets. First, we show that the rotating and translating equilibria of finite vortex sheets are linearly unstable. However, while in the first case unstable perturbations grow exponentially fast in time, the growth of such perturbations in the second case is algebraic. In both cases the growth rates are increasing functions of the wavenumbers of the perturbations. Remarkably, these stability results are obtained entirely with analytical computations. Second, we obtain and analyze equations describing the time evolution of a straight vortex sheet in linear external fields. Third, it is demonstrated that the results concerning the linear stability analysis of the rotating sheet are consistent with the infinite-aspect-ratio limit of the stability results known for Kirchhoffs ellipse (Love 1893; Mitchell & Rossi 2008) and that the solutions we obtained accounting for the presence of external fields are also consistent with the infinite-aspect-ratio limits of the analogous solutions known for vortex patches.
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