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Register a new userSpin correlations and exchange in square lattice frustrated ferromagnets
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The J1-J2 model on a square lattice exhibits a rich variety of different forms of magnetic order that depend sensitively on the ratio of exchange constants J2/J1. We use bulk magnetometry and polarized neutron scattering to determine J1 and J2 unambiguously for two materials in a new family of vanadium phosphates, Pb2VO(PO4)2 and SrZnVO(PO4)2, and we find that they have ferromagnetic J1. The ordered moment in the collinear antiferromagnetic ground state is reduced, and the diffuse magnetic scattering is enhanced, as the predicted bond-nematic region of the phase diagram is approached.
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We present a model compound with a spin-1/2 frustrated square lattice, in which three ferromagnetic (F) interactions and one antiferromagnetic (AF) compet. Considering the effective spin-1 formed by the dominant F dimer, this square lattice can be mapped to a spin-1 spatially anisotropic triangular lattice. The magnetization curve exhibits gapped behavior indicative of a dominant one-dimensional (1D) AF correlation. In the field-induced gapless phase, the specific heat and magnetic susceptibility show a phase transition to an ordered state with 2D characteristics. These results indicate that the spin-1 Haldane state is extended to the 2D system. We demonstrate that the gapped ground state observed in the present spin-1/2 frustrated square lattice originates from the one-dimensionalization caused by frustration.
We use the coupled cluster method for infinite chains complemented by exact diagonalization of finite periodic chains to discuss the influence of a third-neighbor exchange J3 on the ground state of the spin-1/2 Heisenberg chain with ferromagnetic nearest-neighbor interaction J1 and frustrating antiferromagnetic next-nearest-neighbor interaction J2. A third-neighbor exchange J3 might be relevant to describe the magnetic properties of the quasi-one-dimensional edge-shared cuprates, such as LiVCuO4 or LiCu2O2. In particular, we calculate the critical point J2^c as a function of J3, where the ferromagnetic ground state gives way for a ground state with incommensurate spiral correlations. For antiferromagnetic J3 the ferro-spiral transition is always continuous and the critical values J2^c of the classical and the quantum model coincide. On the other hand, for ferromagnetic J3 lesssim -(0.01...0.02)|J1| the critical value J2^c of the quantum model is smaller than that of the classical model. Moreover, the transition becomes discontinuous, i.e. the model exhibits a quantum tricritical point. We also calculate the height of the jump of the spiral pitch angle at the discontinuous ferro-spiral transition.
Frustration in quantum spin systems promote a variety of novel quantum phases. An important example is the frustrated spin-$1$ model on the square lattice with the nearest-neighbor bilinear ($J_1$) and biquadratic ($K_1$) interactions. We provide strong evidence for a nematic spin liquid phase in a range of $K_1/J_1$ near the SU(3)-symmetric point ($J_1 = K_1$), based on the linear flavor-wave theory and extensive density matrix renormalization group calculation. This phase displays no spin dipolar or quadrupolar order, preserves translational symmetry but spontaneously breaks $C_4$ lattice rotational symmetry, and possesses fluctuations peaked at the wavevector $(pi, 2pi/3)$. The spin excitation gap drops rapidly with system size and appears to be gapless, and the nematic order is attributed to the dominant $(pi, 2pi/3)$ fluctuations. Our results provide a novel mechanism for electronic nematic order and, more generally, open up a new avenue to explore frustration-induced exotic ground states.
The Ising triangular lattice remains the classic test-case for frustrated magnetism. Here we report neutron scattering measurements of short range magnetic order in CuMnO$_2$, which consists of a distorted lattice of Mn$^{3+}$ spins with single-ion anisotropy. Physical property measurements on CuMnO$_2$ are consistent with 1D correlations caused by anisotropic orbital occupation. However the diffuse magnetic neutron scattering seen in powder measurements has previously been fitted by 2D Warren-type correlations. Using neutron spectroscopy, we show that paramagnetic fluctuations persist up to $sim$25 meV above TN= 65 K. This is comparable to the incident energy of typical diffractometers, and results in a smearing of the energy integrated signal, which hence cannot be analysed in the quasi-static approximation. We use low energy XYZ polarised neutron scattering to extract the purely magnetic (quasi)-static signal. This is fitted by reverse Monte Carlo analysis, which reveals that two directions in the triangular layers are perfectly frustrated in the classical spin-liquid phase at 75 K. Strong antiferromagnetic correlations are only found along the b-axis, and our results hence unify the pictures seen by neutron scattering and macroscopic physical property measurements.
Thermodynamic properties of cubic Heisenberg ferromagnets with competing exchange interactions are considered near the frustration point where the coefficient $D$ in the spin-wave spectrum $E_{mathbf{k}}sim D k^{2}$ vanishes. Within the Dyson-Maleev formalism it is found that at low temperatures thermal fluctuations stabilize ferromagnetism by increasing the value of $D$. For not too strong frustration this leads to an unusual concave shape of the temperature dependence of magnetization, which is in agreement with experimental data on the europium chalcogenides. Anomalous temperature behavior of magnetization is confirmed by Monte Carlo simulation. Strong field dependence of magnetization (paraprocess) at finite temperature is found near the frustration point.
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