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Register a new userDeviation from the Wiedemann-Franz law induced by nonmagnetic impurities in overdoped La_{2-x}Sr_{x}CuO_{4}
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X. F. Sun
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To investigate the validity of the Wiedemann-Franz (WF) law in disordered but metallic cuprates, the low-temperature charge and heat transport properties are carefully studied for a series of impurity-substituted and carrier-overdoped La_{1.8}Sr_{0.2}Cu_{1-z}M_zO_4 (M = Zn or Mg) single crystals. With moderate impurity substitution concentrations of z = 0.049 and 0.082 (M = Zn), the resistivity shows a clear metallic behavior at low temperature and the WF law is confirmed to be valid. With increasing impurity concentration to z = 0.13 (M = Zn) or 0.15 (M = Mg), the resistivity shows a low-T upturn but its temperature dependence indicates a finite conductivity in the T to 0 limit. In this weakly-localized metallic state that is intentionally achieved in the overdoped regime, a {it negative} departure from the WF law is found, which is opposite to the theoretical expectation.
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Recently, advances in film synthesis methods have enabled a study of extremely overdoped $La_{2-x}Sr_{x}CuO_{4}$. This has revealed a surprising behavior of the superfluid density as a function of doping and temperature, the explanation of which is vividly debated. One popular class of models posits electronic phase separation, where the superconducting phase fraction decreases with doping, while some competing phase (e.g. ferromagnetic) progressively takes over. A problem with this scenario is that all the way up to the dome edge the superconducting transition remains sharp, according to mutual inductance measurements. However, the physically relevant scale is the Pearl penetration depth, $Lambda_{P}$, and this technique probes the sample on a length scale $L$ that is much larger than $Lambda_{P}$. In the present paper, we use local scanning SQUID measurements that probe the susceptibility of the sample on the scale $L << Lambda_{P}$. Our SQUID maps show uniform landscapes of susceptibility and excellent overall agreement of the local penetration depth data with the bulk measurements. These results contribute an important piece to the puzzle of how high-temperature superconductivity vanishes on the overdoped side of the cuprates phase diagram.
We have performed zero-field muon spin rotation measurements on single crystals of La_{2-x}Sr_{x}CuO_{4} to search for spontaneous currents in the pseudo-gap state. By comparing measurements on materials across the phase diagram, we put strict upper limits on any possible time-reversal symmetry breaking fields that could be associated with the pseudo-gap. Comparison between experimental limits and proposed circulating current states effectively eliminates the possibility that such states exist in this family of materials.
A central issue for copper oxides is the nature of the insulating ground state at low carrier densities and the emergence of high-temperature superconductivity from that state with doping. Even though this superconductor-insulator transition (SIT) is a zero-temperature transition, measurements are not usually carried out at low temperatures. Here we use magnetoresistance to probe both the insulating state at very low temperatures and the presence of superconducting fluctuations in La_{2-x}Sr_{x}CuO_{4}(LSCO) films, for doping levels that range from the insulator to the superconductor (x=0.03-0.08). We observe that the charge glass behavior, characteristic of the insulating state, is suppressed with doping, but it coexists with superconducting fluctuations that emerge already on the insulating side of the SIT. The unexpected quenching of the superconducting fluctuations by the competing charge order at low temperatures provides a new perspective on the mechanism for the SIT.
Superstructure reflections due to the ordering of holes into stripes in La_(1.45)Nd_(0.4)Sr_(0.15)CuO_4 have been studied with high energy x-ray diffraction. These reflections have been observed clearly for the first time in a sample which is superconducting at low temperatures (T_c = 10 K). The stripe peaks vanish above 62(5) K whereas the magnetic signal of the stripe ordering which has been seen with neutrons before is already suppressed at 45 K. Our results confirm that the ordering of spins and holes is driven by the charges as it is found in the case of La_(1.6-x)Nd_(0.4)Sr_(x)CuO_(4) at the doping level of x = 0.12.
Possible influence of spatially inhomogeneous distribution of strontium impurities on the temperature of antiferromagnetic (AFM) ordering in ceramic samples La2-xSrxCuO4 has been revealed.
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