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Register a new userUpper critical fields of the 11-system iron-chalcogenide superconductor FeSe$_{0.25}$Te$_{0.75}$
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We have performed electrical resistivity measurements of a polycrystalline sample of FeSe$_{0.25}$Te$_{0.75}$, which exhibits superconductivity at $T_{rm c} sim 14$ K, in magnetic fields up to 55 T to determine the upper critical field $mu_{0}H_{rm c2}$. In this compound, very large slopes of $mu_{0}H_{rm c2}$ at the onset, the mid-point, the zero-resistivity temperatures on superconductivity are determined to be -13.7, -10.1, and -6.9 T/K, respectively. The observed $mu_{0}H_{rm c2}(T)$s of this compound are considerably smaller than those expected from the Werthamer-Helfand-Hohenberg model, manifesting the Pauli limiting behavior. These results suggest that this compound has a large Maki parameter, but it is smaller than that calculated for a weak-coupling superconductor, indicating a large superconducting gap of this compound as a strong-coupling superconductor.
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The high upper critical field characteristic of the recently discovered iron-based superconducting chalcogenides opens the possibility of developing a new type of non-oxide high-field superconducting wires. In this work, we utilize a buffered metal template on which we grow a textured FeSe$_{0.5}$Te$_{0.5}$ layer, an approach developed originally for high temperature superconducting coated conductors. These tapes carry high critical current densities (>1$times10^{4}$A/cm$^{2}$) at about 4.2K under magnetic field as high as 25 T, which are nearly isotropic to the field direction. This demonstrates a very promising future for iron chalcogenides for high field applications at liquid helium temperatures. Flux pinning force analysis indicates a point defect pinning mechanism, creating prospects for a straightforward approach to conductor optimization.
An SDW antiferromagnetic (SDW-AF) low temperature phase transition is generally observe and the AF spin fluctuations are considered to play an important role for the superconductivity paring mechanism in FeAs superconductors. However, a similar magnetic phase transition is not observed in FeSe superconductors, which has caused considerable discussion. We report on the intrinsic electronic states of FeSe as elucidated by transport measurements under magnetic fields using a high quality single crystal. A mobility spectrum analysis, an ab initio method that does not make assumptions on the transport parameters in a multicarrier system, provides very import and clear evidence that another hidden order, most likely the symmetry broken from the tetragonal C4 symmetry to the C2 symmetry nematicity associated with the selective d-orbital splitting, exists in the case of superconducting FeSe other than the AF magnetic order spin fluctuations. The intrinsic low temperature phase in FeSe is in the almost compensated semimetallic states but is additionally accompanied by Dirac cone like ultrafast electrons $sim$ 10$^4$cm$^2$(VS)$^{-1}$ as minority carriers.
Shubnikov-de Haas (SdH) oscillations and upper critical magnetic field ($H_{c2}$) of the iron-based superconductor FeSe ($T_c$ = 8.6 K) have been studied by tunnel diode oscillator-based measurements in magnetic fields of up to 55 T and temperatures down to 1.6 K. Several Fourier components enter the SdH oscillations spectrum with frequencies definitely smaller than predicted by band structure calculations indicating band renormalization and reconstruction of the Fermi surface at low temperature, in line with previous ARPES data. The Werthamer-Helfand-Hohenberg model accounts for the temperature dependence of $H_{c2}$ for magnetic field applied both parallel (textbf{H} $|$ $ab$) and perpendicular (textbf{H} $|$ $c$) to the iron conducting plane, suggesting that one band mainly controls the superconducting properties in magnetic fields despite the multiband nature of the Fermi surface. Whereas Pauli pair breaking is negligible for textbf{H} $|$ $c$, a Pauli paramagnetic contribution is evidenced for textbf{H} $|$ $ab$ with Maki parameter $alpha$ = 2.1, corresponding to Pauli field $H_{P}$ = 36.5 T
We demonstrate that the differential conductance, $dI/dV$, measured via spectroscopic imaging scanning tunneling microscopy in the doped iron chalcogenide FeSe$_{0.45}$Te$_{0.55}$, possesses a series of characteristic features that allow one to extract the orbital structure of the superconducting gaps. This yields nearly isotropic superconducting gaps on the two hole-like Fermi surfaces, and a strongly anisotropic gap on the electron-like Fermi surface. Moreover, we show that the pinning of nematic fluctuations by defects can give rise to a dumbbell-like spatial structure of the induced impurity bound states, and explains the related $C_2$-symmetry in the Fourier transformed differential conductance.
A detailed magnetization study for the novel FeSe superconductor is carried out to investigate the behavior of the intrinsic magnetic susceptibility $chi$ in the normal state with temperature and under hydrostatic pressure. The temperature dependencies of $chi$ and its anisotropy $Delta chi=chi_{|}-chi_{bot}$ are measured for FeSe single crystals in the temperature range 4.2-300 K, and a substantial growth of susceptibility with temperature is revealed. The observed anisotropy $Delta chi$ is very large and comparable with the averaged susceptibility at low temperatures. For a polycrystalline sample of FeSe, a significant pressure effect on $chi$ is determined to be essentially dependent on temperature. Ab initio calculations of the pressure dependent electronic structure and magnetic susceptibility indicate that FeSe is close to magnetic instability with dominating enhanced spin paramagnetism. The calculated paramagnetic susceptibility exhibits a strong dependence on the unit cell volume and especially on the height $Z$ of chalcogen species from the Fe plane. The change of $Z$ under pressure determines a large positive pressure effect on $chi$ which is observed at low temperatures. It is shown that the literature experimental data on the strong and nonmonotonic pressure dependence of the superconducting transition temperature in FeSe correlate qualitatively with calculated behavior of the density of electronic states at the Fermi level.
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