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Register a new userUnusual Hall Effect Anomaly in MnSi Under Pressure
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We report the observation of a highly unusual Hall current in the MnSi in an applied pressure P = 6-12 kbar. The Hall conductivity displays a distinctive step-wise field profile quite unlike any other Hall response observed in solids. We identify the origin of this Hall current with the effective real-space magnetic field due to chiral spin textures, which may be a precursor of the partial-order state at P>14.6 kbar. We discuss evidence favoring the chiral spin mechanism for the origin of the observed Hall anomaly.
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Recent small angle neutron scattering suggests, that the spin structure in the A-phase of MnSi is a so-called triple-$Q$ state, i.e., a superposition of three helices under 120 degrees. Model calculations suggest that this structure in fact is a lattice of so-called skyrmions, i.e., a lattice of topologically stable knots in the spin structure. We report a distinct additional contribution to the Hall effect in the temperature and magnetic field range of the proposed skyrmion lattice, where such a contribution is neither seen nor expected for a normal helical state. Our Hall effect measurements constitute a direct observation of a topologically quantized Berry phase that identifies the spin structure seen in neutron scattering as the proposed skyrmion lattice.
The archetype cubic chiral magnet MnSi is home to some of the most fascinating states in condensed matter such as skyrmions and a non-Fermi liquid behavior in conjunction with a topological Hall effect under hydrostatic pressure. Using small angle neutron scattering, we study the evolution of the helimagnetic, conical and skyrmionic correlations with increasing hydrostatic pressure. We show that the helical propagation vector smoothly reorients from $langle 111 rangle$ to $langle100rangle$ at intermediate pressures. At higher pressures, above the critical pressure, the long-range helimagnetic order disappears at zero magnetic field. Nevertheless, skyrmion lattices and conical spirals form under magnetic fields, in a part of the phase diagram where a topological Hall effect and a non-Fermi liquid behavior have been reported. These unexpected results shed light on the puzzling behavior of MnSi at high pressures and the mechanisms that destabilize the helimagnetic long-range order at the critical pressure.
Measurements of the Hall conductivity in MnSi can provide incisive tests of theories of the anomalous Hall (AH) effect, because both the mean-free-path and magnetoresistance (MR) are unusually large for a ferromagnet. The large MR provides an accurate way to separate the AH conductivity $sigma_{xy}^A$ from the ordinary Hall conductivity $sigma_{xy}^N$. Below the Curie temperature $T_C$, $sigma_{xy}^A$ is linearly proportional to $ M$ (magnetization) with a proportionality constant $S_H$ that is independent of both $T$ and $H$. In particular, $S_H$ remains a constant while $sigma_{xy}^N$ changes by a factor of 100 between 5 K and $T_C$. We discuss implications of the hidden constancy in $S_H$.
We study the electronic structure, magnetic state, and phase stability of paramagnetic BiNiO$_3$ near a pressure-induced Mott insulator-to-metal transition (MIT) by employing a combination of density functional and dynamical mean-field theory. We obtain that BiNiO$_3$ exhibits an anomalous negative-charge-transfer insulating state, characterized by charge disproportionation of the Bi $6s$ states, with Ni$^{2+}$ ions. Upon a compression of the lattice volume by $sim$4.8%, BiNiO$_3$ is found to make a Mott MIT, accompanied by the change of crystal structure from triclinic $Pbar{1}$ to orthorhombic $Pbnm$. The pressure-induced MIT is associated with the melting of charge disproportionation of the Bi ions, caused by a charge transfer between the Bi $6s$ and O $2p$ states. The Ni sites remain to be Ni$^{2+}$ across the MIT, which is incompatible with the valence-skipping Ni$^{2+}$/Ni$^{3+}$ model. Our results suggest that the pressure-induced change of the crystal structure drives the MIT in BiNiO$_3$.
We report comprehensive small angle neutron scattering (SANS) measurements complemented by ac susceptibility data of the helical order, conical phase and skyrmion lattice phase (SLP) in MnSi under uniaxial pressures. For all crystallographic orientations uniaxial pressure favours the phase for which a spatial modulation of the magnetization is closest to the pressure axis. Uniaxial pressures as low as 1kbar applied perpendicular to the magnetic field axis enhance the skyrmion lattice phase substantially, whereas the skyrmion lattice phase is suppressed for pressure parallel to the field. Taken together we present quantitative microscopic information how strain couples to magnetic order in the chiral magnet MnSi.
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