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Uniaxial pressure dependence of magnetic order in MnSi

107   0   0.0 ( 0 )
 Publication date 2015
  fields Physics
and research's language is English




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We report comprehensive small angle neutron scattering (SANS) measurements complemented by ac susceptibility data of the helical order, conical phase and skyrmion lattice phase (SLP) in MnSi under uniaxial pressures. For all crystallographic orientations uniaxial pressure favours the phase for which a spatial modulation of the magnetization is closest to the pressure axis. Uniaxial pressures as low as 1kbar applied perpendicular to the magnetic field axis enhance the skyrmion lattice phase substantially, whereas the skyrmion lattice phase is suppressed for pressure parallel to the field. Taken together we present quantitative microscopic information how strain couples to magnetic order in the chiral magnet MnSi.



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In the temperature-magnetic field phase diagram, the binary metallic compound MnSi exhibits three magnetic phases below Tc ~ 29 K. An unconventional helicoidal phase is observed in zero field. At moderate field intensity a conical phase sets in. Near Tc, in an intermediate field range, a skyrmion lattice phase appears. Here we show the magnetic structure in the conical phase to strongly depend on the field direction and to deviate substantially from a conventional conical structure.
The suppression of magnetic order with pressure concomitant with the appearance of pressure- induced superconductivity was recently discovered in CrAs. Here we present a neutron diffraction study of the pressure evolution of the helimagnetic ground-state towards and in the vicinity of the superconducting phase. Neutron diffraction on polycrystalline CrAs was employed from zero pressure to 0.65 GPa and at various temperatures. The helimagnetic long-range order is sustained under pressure and the magnetic propagation vector does not show any considerable change. The average ordered magnetic moment is reduced from 1.73(2) {mu}B at ambient pressure to 0.4(1) {mu}B close to the critical pressure Pc=0.7 GPa, at which magnetic order is completely suppressed. The width of the magnetic Bragg peaks strongly depends on temperature and pressure, showing a maximum in the region of the onset of superconductivity. We interpret this as associated with competing ground-states in the vicinity of the superconducting phase.
The itinerant quasi-ferromagnetic metal MnSi has been studied by detailed thermal expansion measurements under pressures and magnetic fields. A sudden decrease of the volume at the critical pressure Pc ~1.6 GPa has been observed and is in good agreement with the pressure variation of the volume fraction of the spiral magnetic ordering. This confirms that the magnetic order disappears by a first order phase transition. The energy change estimated by the volume discontinuity on crossing Pc is of similar order as the Zeeman energy of the transition from the spiral ground state to a polarized paramagnetic one under magnetic field. In contrast to the strong pressure dependence of the transition temperature, the characteristic fields are weakly pressure dependent, indicating that the strength of the ferromagnetic and the Dzyaloshinskii-Moriya interactions do not change drastically around Pc. The evaluated results of the thermal expansion coefficient and the magnetostriction are analyzed thermodynamically. The Sommerfeld coefficient of the linear temperature term of the specific heat is enhanced just below Pc. The magnetic field-temperature phase diagrams in the ordered and paramagnetic phases are also compared. Comparison is made with other heavy fermion compounds with first order phase transition at 0 K.
We report a study of the topological Hall effect (THE) in Fe-doped MnSi and compare with results from pure MnSi under pressure. We find that Fe doping increases the THE, indicating an enhancement of the magnitude of the emergent gauge field. This is consistent with the concurrent reduction in the length scale of the skyrmion lattice. For both pressurized and doped samples, we calculate the emergent magnetic field based on the size of the measured THE, and compare it with a theoretical upper-bound. We find that the ratio of these two remains more or less constant with pressure or Fe doping, but differs greatly from that of pure MnSi at ambient pressure. We discuss the implications of this ratio with respect to trends in the saturated magnetic moment and helical pitch length as T_C rightarrow 0 via doping and pressure, respectively.
We report grazing incidence small angle neutron scattering (GISANS) and complementary off-specular neutron reflectometry (OSR) of the magnetic order in a single-crystalline epitaxial MnSi film on Si(111) in the thick film limit. Providing a means of direct reciprocal space mapping, GISANS and OSR reveal a magnetic modulation perpendicular to the films under magnetic fields parallel and perpendicular to the film, where additional polarized neutron reflectometry (PNR) and magnetization measurements are in excellent agreement with the literature. Regardless of field orientation, our data does not suggest the presence of more complex spin textures, notably the formation of skyrmions. This observation establishes a distinct difference with bulk samples of MnSi of similar thickness under perpendicular field, in which a skyrmion lattice dominates the phase diagram. Extended x-ray absorption fine structure measurements suggest that small shifts of the Si positions within the unstrained unit cell control the magnetic state, representing the main difference between the films and thin bulk samples.
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