Do you want to publish a course? Click here

Linear and Nonlinear Optical constants of BiFeO_3

196   0   0.0 ( 0 )
 Added by Amit Kumar
 Publication date 2008
  fields Physics
and research's language is English




Ask ChatGPT about the research

Using spectroscopic ellipsometry, the refractive index and absorption versus wavelength of the ferroelectric antiferromagnet Bismuth Ferrite, BiFeO_3 is reported. The material has a direct band-gap at 442 nm wavelength (2.81 eV). Using optical second harmonic generation, the nonlinear optical coefficients were determined to be d_15/d_22 = 0.20 +/- 0.01, d_31/d_22 = 0.35 +/- 0.02, d_33/d_22 = -11.4 +/- 0.20 and |d_22| = 298.4 +/- 6.1 pm/V at a fundamental wavelength of 800 nm.

rate research

Read More

272 - Evgenia Kim , Feng Wang , Wei Wu 2007
We have obtained spectra of second-harmonic generation, third harmonic generation, and four-wave mixing from a fishnet metamaterial around its magnetic resonance. The resonant behaviors are distinctly different from those for ordinary materials. They result from the fact that the resonance is plasmonic, and its enhancement appears through the local field in the nanostructure.
Chiral topological semimetals are materials that break both inversion and mirror symmetries. They host interesting phenomena such as the quantized circular photogalvanic effect (CPGE) and the chiral magnetic effect. In this work, we report a comprehensive theoretical and experimental analysis of the linear and non-linear optical responses of the chiral topological semimetal RhSi, which is known to host multifold fermions. We show that the characteristic features of the optical conductivity, which display two distinct quasi-linear regimes above and below 0.4 eV, can be linked to excitations of different kinds of multifold fermions. The characteristic features of the CPGE, which displays a sign change at 0.4 eV and a large non-quantized response peak of around 160 $mu textrm{A V}^{-2}$ at 0.7 eV, are explained by assuming that the chemical potential crosses a flat hole band at the Brillouin zone center. Our theory predicts that, in order to observe a quantized CPGE in RhSi, it is necessary to increase the chemical potential as well as the quasiparticle lifetime. More broadly our methodology, especially the development of the broadband terahertz emission spectroscopy, could be widely applied to study photo-galvanic effects in noncentrosymmetric materials and in topological insulators in a contact-less way and accelerate the technological development of efficient infrared detectors based on topological semimetals.
We identify the existence of nonlinear optical (NLO) activity in a number of novel $ABX_3$-type metal-free perovskites, where $A$ is a highly tuneable organic cation, $B$ is a NH$_4$ cation and $X$ a halide anion. Through systematic first-principles calculations, we identify important trends to chart the second-harmonic generation of this class of materials. We study three perovskites MDABCO-NH$_4$I$_3$, CNDABCO-NH$_4$I$_3$ and ODABCO-NH$_4$I$_3$ for use as deep-UV second-harmonic generation materials. We identify the role of the dipole moment imparted by the organic group on the $A$ cation as an important parameter to tune the NLO properties of these materials. We apply this knowledge functionalising the organic group DABCO with the highly polar cyanide CN$^-$ group, and we demonstrate a significant improvement of the NLO response in this family of materials. These findings can accelerate the application of metal free perovskites as inexpensive, non-toxic, earth-abundant materials for the next generation of optical communication applications.
It is shown that stationary vortex structures can be excited in a ferrite film. This is the first proposal for creating vortex structures in the important cm and mm wavelength ranges. It is shown that both linear and nonlinear structures can be excited using a three-beam interaction created with circular antennae. These give rise to a special phase distribution created by linear and nonlinear mixing. An interesting set of three clockwise rotating vortices joined by one counter-rotating one presents itself in the linear regime: a scenario that is only qualitatively changed by the onset of nonlinearity. It is pointed out that control of the vortex structure, through parametric coupling, based upon a microwave resonator, is possible and that there are many interesting possibilities for applications.
LiOsO3 is one of the first materials identified in a recent literature as a polar metal, a class of materials that are simultaneously noncentrosymmetric and metallic. In this work, the linear and nonlinear optical susceptibility of LiOsO3 is studied by means of ellipsometry and optical second harmonic generation (SHG). Strong optical birefringence is observed using spectroscopic ellipsometry. The nonlinear optical susceptibility extracted from SHG polarimetry reveals that the tensor components are of the same magnitude as in isostructural insulator LiNbO3, except the component along the polar axis d33, which is suppressed by an order of magnitude. Temperature-dependent SHG measurements in combination with Raman spectroscopy indicate a continuous order-disorder type polar phase transition at 140 K. Linear and nonlinear optical microscopy techniques reveal 109 deg/71 deg ferroelastic domain walls, like in other trigonal ferroelectrics. No 180 deg polar domain walls are observed to emerge across the phase transition.
comments
Fetching comments Fetching comments
mircosoft-partner

هل ترغب بارسال اشعارات عن اخر التحديثات في شمرا-اكاديميا