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Test of nuclear level density inputs for Hauser-Feshbach model calculations

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 Added by Alexander Voinov dr
 Publication date 2007
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and research's language is English




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The energy spectra of neutrons, protons, and alpha-particles have been measured from the d+59Co and 3He+58Fe reactions leading to the same compound nucleus, 61$Ni. The experimental cross sections have been compared to Hauser-Feshbach model calculations using different input level density models. None of them have been found to agree with experiment. It manifests the serious problem with available level density parameterizations especially those based on neutron resonance spacings and density of discrete levels. New level densities and corresponding Fermi-gas parameters have been obtained for reaction product nuclei such as 60Ni,60Co, and 57Fe.



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The Hauser-Feshbach fission fragment decay model, $mathtt{HF^3D}$, which calculates the statistical decay of fission fragments, has been expanded to include multi-chance fission, up to neutron incident energies of 20 MeV. The deterministic decay takes as input pre-scission quantities - fission probabilities and the average energy causing fission - and post-scission quantities - yields in mass, charge, total kinetic energy, spin, and parity. From these fission fragment initial conditions, the full decay is followed through both prompt and delayed particle emissions, allowing for the calculation of prompt neutron and $gamma$ properties, such as multiplicity and energy distributions, both independent and cumulative fission yields, and delayed neutron observables. In this work, we describe the implementation of multi-chance fission into the $mathtt{HF^3D}$ model, and show an example of prompt and delayed quantities beyond first-chance fission, using the example of neutron-induced fission on $^{235}$U. This expansion represents significant progress in consistently modeling the emission of prompt and delayed particles from fissile systems.
We present a probable experimental signature of collective enhancement in the nuclear level density (NLD) by measuring the neutron and the giant dipole resonance (GDR) $gamma$ rays emitted from the rare earth $^{169}$Tm compound nucleus populated at 26.1 MeV excitation energy. An enhanced yield is observed in both neutron and $gamma$ ray spectra corresponding to the same excitation energy in the daughter nuclei. The enhancement could only be reproduced by including a collective enhancement factor in the Fermi gas model of NLD to explain the neutron and GDR spectra simultaneously. The experimental results show that the relative enhancement factor is of the order of 10 and the fadeout occurs at $sim$ 14 MeV excitation energy, much before the commonly accepted transition from deformed to spherical shape. We also explain how the collective enhancement contribution changes the inverse level density parameter ($k$) from 8 to 9.5 MeV observed recently in several deformed nuclei.
The nuclear level density and the gamma-ray strength function have been determined for 43Sc in the energy range up to 2 MeV below the neutron separation energy using the Oslo method with the 46Ti(p,alpha)43Sc reaction. A comparison to 45Sc shows that the level density of 43Sc is smaller by an approximately constant factor of two. This behaviour is well reproduced in a microscopical/combinatorial model calculation. The gamma-ray strength function is showing an increase at low gamma-ray energies, a feature which has been observed in several nuclei but which still awaits theoretical explanation.
We present the first application of a new approach, proposed in [Journal of Physics G: Nuclear and Particle Physics, 43, 04LT01 (2016)] to derive coupling constants of the Skyrme energy density functional (EDF) from ab initio Hamiltonian. By perturbing the ab initio Hamiltonian with several functional generators defining the Skyrme EDF, we create a set of metadata that is then used to constrain the coupling constants of the functional. We use statistical analysis to obtain such an ab initio-equivalent Skyrme EDF. We find that the resulting functional describes properties of atomic nuclei and infinite nuclear matter quite poorly. This may point out to the necessity of building up the ab initio-equivalent functionals from more sophisticated generators. However, we also indicate that the current precision of the ab initio calculations may be insufficient for deriving meaningful nuclear EDFs.
The isospin dependence of nuclear level density has been investigated by analyzing the spectra of evaporated neutrons from excited $^{116}$Sn and $^{116}$Te nuclei. These nuclei are populated via $p$ + $^{115}$In and $^{4}$He + $^{112}$Sn reactions in the excitation energy range of 18 - 26 MeV. Because of low excitation energy, the neutron spectra are predominantly contributed by the first-chance decay leading to the $beta$-stable $^{115}$Sn and neutron-deficient $^{115}$Te as residues for the two cases. Theoretical analysis of the experimental spectra have been performed within the Hauser-Feshbach formalism by employing different models of the level density parameter. It is observed that the data could only be explained by the level density parameter that decreases monotonically when the proton number deviates from the $beta$-stable value. This is also confirmed by performing a microscopic shell-model calculation with the Wood-Saxon mean field. The results have strong implication on the estimation of the level density of unstable nuclei, and calculation of astrophysical reaction rates relevant to $r$- and $rp$-processes.
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