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The formation, deformation, and break-up of liquid interfaces are ubiquitous phenomena in nature. In the present article we discuss the deformation of a liquid interface produced by optical radiation forces. Usually, the bending of such an interface by the radiation pressure of a c.w. laser beam is weak. However, the effect can be enhanced significantly if one works with a near-critical phase-separated liquid mixture, whereby the surface tension becomes weak. The bending may in this way become as large as several tenths of micrometers, even with the use of only moderate laser power. This near-criticality is a key element in our experimental investigations as reviewed in the article. The effect is achieved by working with a micellar phase of microemulsions, at room temperature. We give a brief survey of the theory of electromagnetic forces on continuous matter, and survey earlier experiments in this area, such as the Ashkin-Dziedzic optical radiation force experiment on a water/air surface (1973), the Zhang-Chang experiment on the laser-induced deformation of a micrometer-sized spherical water droplet (1988), and the experiment of Sakai et al. measuring surface tensions of interfaces in a non-contact manner (2001). Thereafter, we survey results we obtained in recent years by performing experiments on near-critical interfaces, such as interface bending in the linear regime, stationary large deformations of liquid interfaces, asymmetric pressure effects on interfaces under intense illumination, nonlinear deformations, and laser-sustained liquid columns.
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Recent experimental developments showed that the use of the radiation pressure, induced by a continuous laser wave, to control fluid-fluid interface deformations at the microscale, represents a very promising alternative to electric or magnetic actuation. In this article, we solve numerically the dynamics and steady state of the fluid interface under the effects of buoyancy, capillarity, optical radiation pressure and viscous stress. A precise quantitative validation is shown by comparison with experimental data. New results due to the nonlinear dependence of the optical pressure on the angle of incidence are presented, showing different morphologies of the deformed interface going from needle-like to finger-like shapes, depending on the refractive index contrast. In the transient regime, we show that the viscosity ratio influences the time taken for the deformation to reach steady state.
Fluctuations of the interface between coexisting colloidal fluid phases have been measured with confocal microscopy. Due to a very low surface tension, the thermal motions of the interface are so slow, that a record can be made of the positions of the interface. The theory of the interfacial height fluctuations is developed. For a host of correlation functions, the experimental data are compared with the theoretical expressions. The agreement between theory and experiment is remarkably good.
We report on a new class of electromagnetically-driven fluid interface instability. Using the optical radiation pressure of a cw laser to bend a very soft near-critical liquid-liquid interface, we show that it becomes unstable for sufficiently large beam power P, leading to the formation of a stationary beam-centered liquid micro-jet. We explore the behavior of the instability onset by tuning the interface softness with temperature and varying the size of the exciting beam. The instability mechanism is experimentally demonstrated. It simply relies on total reflection of light at the deformed interface whose condition provides the universal scaling relation for the onset Ps of the instability.
Deformations of horizontal liquid interfaces by optical radiation pressure are generally expected to display similar behaviors whatever the direction of propagation of the exciting laser beam is. In the present experiment we find this expectation to be borne out, as long as the cw laser illumination is moderate in strength. However, as a striking contrast in the case of high field strengths, we find that either a large stable tether can be formed, or else that a break-up of the interface can occur, depending on whether the laser beam is upward or downward directed. Physically, the reason for this asymmetry can be traced to whether total reflection can occur or not. We also present two simple theoretical models, one based on geometrical optics, the other on wave optics, that are able to illustrate the essence of the effect. In the case leading to interface disruption our experimental results are compared with those obtained by Zhang and Chang for water droplets under intense laser pulses [Opt. Lett. textbf{13}, 916 (1988)]. A key point in our experimental investigations is to work with a near-critical liquid/liquid interface. The surface tension becomes therefore significantly reduced, which thus enhances the magnitude of the stationary deformations induced.
The influence of a fluid-fluid interface on self-phoresis of chemically active, axially symmetric, spherical colloids is analyzed. Distinct from the studies of self-phoresis for colloids trapped at fluid interfaces or in the vicinity of hard walls, here we focus on the issue of self-phoresis close to a fluid-fluid interface. In order to provide physically intuitive results highlighting the role played by the interface, the analysis is carried out for the case that the symmetry axis of the colloid is normal to the interface; moreover, thermal fluctuations are not taken into account. Similarly to what has been observed near hard walls, we find that such colloids can be set into motion even if their whole surface is homogeneously active. This is due to the anisotropy along the direction normal to the interface owing to the partitioning by diffusion, among the coexisting fluid phases, of the product of the chemical reaction taking place at the colloid surface. Different from results corresponding to hard walls, in the case of a fluid interface the direction of motion, i.e., towards the interface or away from it, can be controlled by tuning the physical properties of one of the two fluid phases. This effect is analyzed qualitatively and quantitatively, both by resorting to a far-field approximation and via an exact, analytical calculation which provides the means for a critical assessment of the approximate analysis.
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