We investigate systematic errors associated with a common modulation technique used for phase sensitive detection of a coherent population trapping (CPT) resonance. In particular, we show that modification of the CPT resonance lineshape due to the presence of off-resonant fields leads to frequency shifts which may limit the stability of CPT-based atomic clocks. We also demonstrate that an alternative demodulation technique greatly reduces these effects.
Extra-laboratory atomic clocks are necessary for a wide array of applications (e.g. satellite-based navigation and communication). Building upon existing vapor cell and laser technologies, we describe an optical atomic clock, designed around a simple and manufacturable architecture, that utilizes the 778~nm two-photon transition in rubidium and yields fractional frequency instabilities of $3times10^{-13}/sqrt{tau (s)}$ for $tau$ from 1~s to 10000~s. We present a complete stability budget for this system and explore the required conditions under which a fractional frequency instability of $1times 10^{-15}$ can be maintained on long timescales. We provide precise characterization of the leading sensitivities to external processes including magnetic fields and fluctuations of the vapor cell temperature and 778~nm laser power. The system is constructed primarily from commercially-available components, an attractive feature from the standpoint of commercialization and deployment of optical frequency standards.
The coherent population trapping (CPT) atomic clock is very promising for use in next-generation spaceborne applications owing to its compactness and high performance. In this paper, we propose and implement a CPT atomic clock based on the direct modulation of a large-modulation-bandwidth and narrow-linewidth distributed Bragg reflector laser, which replaces the usually used external bulk modulator in the high-performance CPT clock. Our method retains the high performance while significantly reducing the size. Using this highly compact bichromatic light source and simplest CPT configuration, in which a circularly polarized bichromatic laser interrogates the ^{87}Rb atom system, a CPT signal of clock transition with a narrow linewidth and high contrast is observed. We then lock the local oscillator frequency to the CPT error signal and demonstrate a short-term frequency stability of 3.6 times 10^{-13} {tau}^{-1/2} (4 s le {tau} le 200 s). We attribute it to the ultralow laser frequency and intensity noise as well as to the high-quality-factor CPT signal. This study can pave the way for the development of compact high-performance CPT clocks based on our scheme.
We report modulation transfer spectroscopy on the D2 transitions in 85Rb and 87Rb using a simple home-built electro-optic modulator (EOM). We show that both the gradient and amplitude of modulation transfer spectroscopy signals, for the 87Rb F=2 to F=3 and the 85Rb F=3 to F=4 transitions, can be significantly enhanced by expanding the beams, improving the signals for laser frequency stabilization. The signal gradient for these transitions is increased by a factor of 3 and the peak to peak amplitude was increased by a factor of 2. The modulation transfer signal for the 85Rb F=2 to F transitions is also presented to highlight how this technique can generate a single, clear line for laser frequency stabilization even in cases where there are a number of closely spaced hyperfine transitions.
A general mechanism for the generation of frequency combs referenced to atomic resonances is put forward. The mechanism is based on the periodic phase control of a quantum systems dipole response. We develop an analytic description of the comb spectral structure, depending on both the atomic and the phase-control properties. We further suggest an experimental implementation of our scheme: Generating a frequency comb in the soft-x-ray spectral region, which can be realized with currently available techniques and radiation sources. The universality of this mechanism allows the generalization of frequency-comb technology to arbitrary frequencies, including the hard-x-ray regime by using reference transitions in highly charged ions.
The sensitivity of an atomic interferometer increases when the phase evolution of its quantum superposition state is measured over a longer interrogation interval. In practice, a limit is set by the measurement process, which returns not the phase, but its projection in terms of population difference on two energetic levels. The phase interval over which the relation can be inverted is thus limited to the interval $[-pi/2,pi/2]$; going beyond it introduces an ambiguity in the read out, hence a sensitivity loss. Here, we extend the unambiguous interval to probe the phase evolution of an atomic ensemble using coherence preserving measurements and phase corrections, and demonstrate the phase lock of the clock oscillator to an atomic superposition state. We propose a protocol based on the phase lock to improve atomic clocks under local oscillator noise, and foresee the application to other atomic interferometers such as inertial sensors.