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Register a new userPlasma formation from ultracold Rydberg gases
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Recent experiments have demonstrated the spontaneous evolution of a gas of ultracold Rydberg atoms into an expanding ultracold plasma, as well as the reverse process of plasma recombination into highly excited atomic states. Treating the evolution of the plasma on the basis of kinetic equations, while ionization/excitation and recombination are incorporated using rate equations, we have investigated theoretically the Rydberg-to-plasma transition. Including the influence of spatial correlations on the plasma dynamics in an approximate way we find that ionic correlations change the results only quantitatively but not qualitatively.
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We report on the behaviour of the ionization avalanche in an ensemble of ultracold 87Rb atoms coupled to a high lying Rydberg state and investigate extensions to the current model by including the effects of three-body recombination and plasma expansion. To separate the two effects we study the time dependence of the plasma formation at various densities as well as for different nS and nD states. At medium densities and low n we observe the onset of the avalanche as has been reported in other experiments, as well as a subsequent turn-off of the avalanche for longer excitation times, which we associate with plasma expansion. At higher densities and for higher lying Rydberg states we observe a disappearance of the avalanche signature, which we attribute to three-body recombination.
In plasmas at very low temperatures formation of neutral atoms is dominated by collisional three-body recombination, owing to the strong ~ T^(-9/2) scaling of the corresponding recombination rate with the electron temperature T. While this law is well established at high temperatures, the unphysical divergence as T -> 0 clearly suggest a breakdown in the low-temperature regime. Here, we present a combined molecular dynamics-Monte-Carlo study of electron-ion recombination over a wide range of temperatures and densities. Our results reproduce the known behavior of the recombination rate at high temperatures, but reveal significant deviations with decreasing temperature. We discuss the fate of the kinetic bottleneck and resolve the divergence-problem as the plasma enters the ultracold, strongly coupled domain.
An ensemble of excited atoms can synchronize emission of light collectively in a process known as superradiance when its characteristic size is smaller than the wavelength of emitted photons. The underlying superradiance depends strongly on electromagnetic (photon) fields surrounding the atomic ensemble. High mode densities of microwave photons from $300,$K blackbody radiation (BBR) significantly enhance decay rates of Rydberg states to neighbouring states, enabling superradiance that is not possible with bare vacuum induced spontaneous decay. Here we report observations of the superradiance of ultracold Rydberg atoms embedded in a bath of room-temperature photons. The temporal evolution of the Rydberg $|nDrangle$ to $|(n+1)Prangle$ superradiant decay of Cs atoms ($n$ the principal quantum number) is measured directly in free space. Theoretical simulations confirm the BBR enhanced superradiance in large Rydberg ensembles. We demonstrate that the van der Waals interactions between Rydberg atoms change the superradiant dynamics and modify the scaling of the superradiance. In the presence of static electric fields, we find that the superradiance becomes slow, potentially due to many-body interaction induced dephasing. Our study provides insights into many-body dynamics of interacting atoms coupled to thermal BBR, and might open a route to the design of blackbody thermometry at microwave frequencies via collective, dissipative photon-atom interactions.
Double-resonant photoexcitation of nitric oxide in a molecular beam creates a dense ensemble of $50f(2)$ Rydberg states, which evolves to form a plasma of free electrons trapped in the potential well of an NO$^+$ spacecharge. The plasma travels at the velocity of the molecular beam, and, on passing through a grounded grid, yields an electron time-of-flight signal that gauges the plasma size and quantity of trapped electrons. This plasma expands at a rate that fits with an electron temperature as low as 5 K, colder that typically observed for atomic ultracold plasmas. The recombination of molecular NO$^+$ cations with electrons forms neutral molecules excited by more than twice the energy of the NO chemical bond, and the question arises whether neutral fragmentation plays a role in shaping the redistribution of energy and particle density that directs the short-time evolution from Rydberg gas to plasma. To explore this question, we adapt a coupled rate-equations model established for atomic ultracold plasmas to describe the energy-grained avalanche of electron-Rydberg and electron-ion collisions in our system. Adding channels of Rydberg predissociation and two-body, electron- cation dissociative recombination to the atomic formalism, we investigate the kinetics by which this relaxation distributes particle density and energy over Rydberg states, free electrons and neutral fragments. The results of this investigation suggest some mechanisms by which molecular fragmentation channels can affect the state of the plasma.
We characterize the two-photon excitation of an ultracold gas of Rubidium atoms to Rydberg states analysing the induced atomic losses from an optical dipole trap. Extending the duration of the Rydberg excitation to several ms, the ground state atoms are continuously coupled to the formed positively charged plasma. In this regime we measure the $n$-dependence of the blockade effect and we characterise the interaction of the excited states and the ground state with the plasma. We also investigate the influence of the quasi-electrostatic trapping potential on the system, confirming the validity of the ponderomotive model for states with $20leq nleq 120$.
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