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Register a new userA study of the phase transition in the usual statistical model for nuclear multifragmentation
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We use a simplified model which is based on the same physics as inherent in most statistical models for nuclear multifragmentation. The simplified model allows exact calculations for thermodynamic properties of systems of large number of particles. This enables us to study a phase transition in the model. A first order phase transition can be tracked down. There are significant differences between this phase transition and some other well-known cases.
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The agreement between the fragments internal and kinetic temperatures with the breakup temperature is investigated using a Statistical Multifragmentation Model which makes no a priori as- sumption on the relationship between them. We thus examine the conditions for obtaining such agreement and find that, in the framework of our model, this holds only in a relatively narrow range of excitation energy. The role played by the qualitative shape of the fragments state densities is also examined. Our results suggest that the internal temperature of the light fragments may be affected by this quantity, whose behavior may lead to constant internal temperatures over a wide excitation energy range. It thus suggests that the nuclear thermometry may provide valuable information on the nuclear state density.
A great many observables seen in intermediate energy heavy ion collisions can be explained on the basis of statistical equilibrium. Calculations based on statistical equilibrium can be implemented in microcanonical ensemble (energy and number of particles in the system are kept fixed), canonical ensemble (temperature and number of particles are kept fixed) or grand canonical ensemble (fixed temperature and a variable number of particles but with an assigned average). This paper deals with calculations with canonical ensembles. A recursive relation developed recently allows calculations with arbitrary precision for many nuclear problems. Calculations are done to study the nature of phase transition in intermediate energy heavy ion collision, to study the caloric curves for nuclei and to explore the possibility of negative specific heat because of the finiteness of nuclear systems. The model can also be used for detailed calculations of other observables not connected with phase transitions, such as populations of selected isotopes in a heavy ion collision. The model also serves a pedagogical purpose. For the problems at hand, both the canonical and grand canonical solutions are obtainable with arbitrary accuracy hence we can compare the values of observables obtained from the canonical calculations with those from the grand canonical. Sometimes, very interesting discrepancies are found. To illustrate the predictive power of the model, calculated observables are com$data from the central collisions of Sn isotopes.
The cumulant ratios up to fourth order of the $Z$ distributions of the largest fragment in spectator fragmentation following $^{107,124}$Sn+Sn and $^{124}$La+Sn collisions at 600 MeV/nucleon have been investigated. They are found to exhibit the signatures of a second-order phase transition established with cubic bond percolation and previously observed in the ALADIN experimental data for fragmentation of $^{197}$Au projectiles at similar energies. The deduced pseudocritical points are found to be only weakly dependent on the $A/Z$ ratio of the fragmenting spectator source. The same holds for the corresponding chemical freeze-out temperatures of close to 6 MeV. The experimental cumulant distributions are quantitatively reproduced with the Statistical Multifragmentation Model and parameters used to describe the experimental fragment multiplicities, isotope distributions and their correlations with impact-parameter related observables in these reactions. The characteristic coincidence of the zero transition of the skewness with the minimum of the kurtosis excess appears to be a generic property of statistical models and is found to coincide with the maximum of the heat capacity in the canonical thermodynamic fragmentation model.
This review article is focused on the tremendous progress realized during the last fifteen years in the understanding of multifragmentation and its relationship to the liquid-gas phase diagram of nuclei and nuclear matter. The explosion of the whole nucleus, early predicted by Bohr [N. Bohr, Nature 137 (1936) 351], is a very complex and rich subject which continues to fascinate nuclear physicists as well as theoreticians who extend the thermodynamics of phase transitions to finite systems.
The Statistical Multifragmentation Model is modified to incorporate the Helmholtz free energies calculated in the finite temperature Thomas-Fermi approximation using Skyrme effective interactions. In this formulation, the density of the fragments at the freeze-out configuration corresponds to the equilibrium value obtained in the Thomas-Fermi approximation at the given temperature. The behavior of the nuclear caloric curve at constant volume is investigated in the micro-canonical ensemble and a plateau is observed for excitation energies between 8 and 10 MeV per nucleon. A kink in the caloric curve is found at the onset of this gas transition, indicating the existence of a small excitation energy region with negative heat capacity. In contrast to previous statistical calculations, this situation takes place even in this case in which the system is constrained to fixed volume. The observed phase transition takes place at approximately constant entropy. The charge distribution and other observables also turn out to be sensitive to the treatment employed in the calculation of the free energies and the fragments volumes at finite temperature, specially at high excitation energies. The isotopic distribution is also affected by this treatment, which suggests that this prescription may help to obtain information on the nuclear equation of state.
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