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Register a new userThe Quasi-Molecular Stage of Ternary Fission
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We developed a three-center phenomenological model,able to explain qualitatively the recently obtained experimental results concerning the quasimolecular stage of a light-particle accompanied fission process. It was derived from the liquid drop model under the assumption that the aligned configuration, with the emitted particle between the light and heavy fragment, is reached by increasing continuously the separation distance, while the radii of the heavy fragment and of the light particle are kept constant. In such a way,a new minimum of a short-lived molecular state appears in the deformation energy at a separation distance very close to the touching point. This minimum allows the existence of a short-lived quasi-molecular state, decaying into the three final fragments.The influence of the shell effects is discussed. The half-lives of some quasimolecular states which could be formed in the $^{10}$Be and $^{12}$C accompanied fission of $^{252}$Cf are roughly estimated to be the order of 1 ns, and 1 ms, respectively.
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We consider the collinear ternary fission which is a sequential ternary decay with a very short time between the ruptures of two necks connecting the middle cluster of the ternary nuclear system and outer fragments. In particular, we consider the case where the Coulomb field of the first massive fragment separated during the first step of the fission produces a lower pre-scission barrier in the second step of the residual part of the ternary system. In this case, we obtain a probability of about $10^{-3}$ for the yield of massive clusters such as uclide[70]{Ni}, uclide[80-82]{Ge}, uclide[86]{Se}, and uclide[94]{Kr} in the ternary fission of uclide[252]{Cf}. These products appear together with the clusters having mass numbers of $A = 132$--$140$. The results show that the yield of a heavy cluster such as uclide[68-70]{Ni} would be followed by a product of $A = 138$--$148$ with a large probability as observed in the experimental data obtained with the FOBOS spectrometer at the Joint Institute for Nuclear Research. The third product is not observed. The landscape of the potential energy surface shows that the configuration of the Ni + Ca + Sn decay channel is lower about 12 MeV than that of the Ca + Ni + Sn channel. This leads to the fact, that the yield of Ni and Sn is large. The analysis on the dependence of the velocity of the middle fragment on mass numbers of the outer products leads to the conclusion that, in the collinear tripartition channel of uclide[252]{Cf}, the middle cluster has a very small velocity, which does not allow it to be found in experiments.
For the first time, we apply the temperature dependent relativistic mean field (TRMF) model to study the ternary fission of heavy nucleus using level density approach. The probability of yields of a particular fragment is obtained by evaluating the convolution integrals which employ the excitation energy and the level density parameter for a given temperature calculated within the TRMF formalism. To illustrate, we have considered the ternary fissions in 252Cf, 242Pu and 236U with fixed third fragment A3 = 48Ca, 20O and 16O respectively. The relative yields are studied for the temperatures T = 1, 2 and 3 MeV. For the comparison, the relative yields are also calculated from the single particle energies of the finite range droplet model (FRDM). In general, the larger phase space for the ternary fragmentation is observed indicating that such fragmentations are most probable ones. For T = 2 and 3 MeV, the Sn + Ni + Ca is the most probable combination for the nucleus 252Cf. However, for the nuclei 242Pu and 236U, the maximum fragmentation yields at T = 2 MeV differ from those at T = 3 MeV. For T = 3 MeV, the closed shell (Z = 8) light mass fragments with its corresponding partners has larger yield values. But, at T = 2 MeV Si/P/S are favorable fragments with the corresponding partners. It is noticed that the symmetric binary fragmentation along with the fixed third fragment for 242Pu and 236U are also favored at T = 1 MeV. The temperature dependence of the nuclear shape and the single particle energies are also discussed.
Ternary fission of actinides probes the state of the nucleus at scission. Light clusters are produced in space and time very close to the scission point. Within the nonequilibrium statistical operator method, a generalized Gibbs distribution is constructed from the information given by the observed yields of isotopes. Using this relevant statistical operator, yields are calculated taking excited states and continuum correlations into account, in accordance with the virial expansion of the equation of state. Clusters with mass number $A le 10$ are well described using the nonequilibrium generalizations of temperature and chemical potentials. Improving the virial expansion, in-medium effects may become of importance in determining the contribution of weakly bound states and continuum correlations to the intrinsic partition function. Yields of larger clusters, which fail to reach this quasi-equilibrium form of the relevant distribution, are described by nucleation kinetics, and a saddle-to-scission relaxation time of about 7000 fm/c is inferred. Light charged particle emission, described by reaction kinetics and virial expansions, may therefore be regarded as a very important tool to probe the nonequilibrium time evolution of actinide nuclei during fission.
The quasi-fission mechanism hinders fusion of heavy systems because of a mass flow between the reactants, leading to a re-separation of more symmetric fragments in the exit channel. A good understanding of the competition between fusion and quasi-fission mechanisms is expected to be of great help to optimize the formation and study of heavy and superheavy nuclei. Quantum microscopic models, such as the time-dependent Hartree-Fock approach, allow for a treatment of all degrees of freedom associated to the dynamics of each nucleon. This provides a description of the complex reaction mechanisms, such as quasi-fission, with no parameter adjusted on reaction mechanisms. In particular, the role of the deformation and orientation of a heavy target, as well as the entrance channel magicity and isospin are investigated with theoretical and experimental approaches.
The yields of light elements ($Z=1,2$) obtained from spontaneous ternary fission of $^{252}$Cf are treated within a nonequilibrium approach, and the contribution of unstable nuclei and excited bound states is taken into account. These light cluster yields may be used to probe dense matter, and to infer in-medium corrections. Continuum correlations are calculated from scattering phase shifts using the Beth-Uhlenbeck formula, and the effect of medium modification is estimated. The relevant distribution is reconstructed from the measured yields of isotopes. This describes the state of the nucleon system at scission and cluster formation, using only three Lagrange parameters which are the nonequilibrium counterparts of the temperature and chemical potentials, as defined in thermodynamic equilibrium. We concluded that a simple nuclear statistical equilibrium model neglecting continuum correlations and medium effects is not able to describe the measured distribution of H and He isotopes. Moreover, the freeze-out concept may serve as an important ingredient to the nonequilibrium approach using the relevant statistical operator concept.
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