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Register a new userSearch for the Production of Element 112 in the 48Ca + 238U Reaction
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W. Loveland
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We have searched for the production of element 112 in the reaction of 231 MeV 48Ca with 238U. We have not observed any events with a one event upper limit cross section of 1.6 pb for EVR-fission events and 1.8 pb for EVR-alpha events.
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The 48Ca({gamma},n) cross section was measured using {gamma}-ray beams of energies between 9.5 and 15.3 MeV generated at the Triangle Universities Nuclear Laboratory (TUNL) high-intensity {gamma}-ray source (HI{gamma}S). Prior to this experiment, no direct measurements had been made with {gamma}-ray beams of sufficiently low energy spread to observe structure in this energy range. The cross sections were measured at thirty-four different {gamma}-ray energies with an enriched 48Ca target. Neutron emission is the dominant decay mechanism in the measured energy range that spans from threshold, across the previously identified M1 strength, and up the low-energy edge of the E1 giant dipole resonance (GDR). This work found B(M 1) = 6.8 pm 0.5 {mu}N2 for the 10.23 MeV resonance, a value greater than previously measured. Structures in the cross section commensurate with extended random-phase approximation (ERPA) calculations have also been observed whose magnitudes are in agreement with existing data.
Fission fragments from 1 A GeV 238U projectiles irradiating a hydrogen target were investigated by using the fragment separator FRS for magnetic selection of reaction products including ray-tracing and DE-ToF techniques. The momentum spectra of 733 identified fragments were analysed to provide isotopic production cross sections, fission-fragment velocities and recoil momenta of the fissioning parent nuclei. Besides their general relevance, these quantities are also demanded for applications. Calculations and simulations with codes commonly used and recently developed or improved are compared to the data.
We investigated the 238U(d,p) reaction as a surrogate for the n + 238U reaction. For this purpose we measured for the first time the gamma-decay and fission probabilities of 239U* simultaneously and compared them to the corresponding neutron-induced data. We present the details of the procedure to infer the decay probabilities, as well as a thorough uncertainty analysis, including parameter correlations. Calculations based on the continuum-discretized coupled-channels and distorted-wave Born approximations were used to correct our data from detected protons originating from elastic and inelastic deuteron breakup. In the region where the fission and gamma-decay probabilities compete, the corrected fission probability is in agreement with neutron-induced data, whereas the gamma-decay probability is much higher than the neutron-induced data. The performed statistical-model calculations are not able to explain these results.
During the slow neutron capture process in massive stars, reactions on light elements can both produce and absorb neutrons thereby influencing the final heavy element abundances. At low metallicities, the high neutron capture rate of 16-O can inhibit s-process nucleosynthesis unless the neutrons are recycled via the 17O(a,n)20Ne reaction. The efficiency of this neutron recycling is determined by competition between the 17O(a,n)20Ne and 17O(a,g)21Ne reactions. While some experimental data are available on the former reaction, no data exist for the radiative capture channel at the relevant astrophysical energies. The 17O(a,g)21Ne reaction has been studied directly using the DRAGON recoil separator at the TRIUMF Laboratory. The reaction cross section has been determined at energies between 0.6 and 1.6 MeV Ecm, reaching into the Gamow window for core helium burning for the first time. Resonance strengths for resonances at 0.63, 0.721, 0.81 and 1.122 MeV Ecm have been extracted. The experimentally based reaction rate calculated represents a lower limit, but suggests that significant s-process nucleosynthesis occurs in low metallicity massive stars.
The reaction mechanisms best suited for the production of neutron-rich nuclei, fragmentation and fission, are discussed. Measurements of the production cross sections of reaction residues together with model calculations allow to conclude about the expected production rates of neutron-rich isotopes in future facilities.
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