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Register a new userTemperature dependent scattering rate and optical mass of ferromagnetic metallic manganites
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We report on the optical properties of the hole-doped manganites La_0.7Ca_0.3MnO_3 and La_0.7Ca_0.3MnO_3. Transmission and reflection of thin films are measured in the infrared at temperatures from 10 - 150 K using Fourier-transform spectroscopy. The scattering rate and optical mass are obtained by fitting the far-infrared transmission to a Drude model. The scattering rate shows a T^2 dependence with temperature. The optical mass enhancement differs only slightly from specific heat results. In addition, we compare the infrared spectral weight to band structure calculations [M. Quijada et al., Phys. Rev. B 58, 16093 (1998)].
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Ferromagnetic (FM) manganites, a group of likely half-metallic oxides, are of special interest not only because they are a testing ground of the classical doubleexchange interaction mechanism for the colossal magnetoresistance, but also because they exhibit an extraordinary arena of emergent phenomena. These emergent phenomena are related to the complexity associated with strong interplay between charge, spin, orbital, and lattice. In this review, we focus on the use of inelastic neutron scattering to study the spin dynamics, mainly the magnon excitations in this class of FM metallic materials. In particular, we discussed the unusual magnon softening and damping near the Brillouin zone boundary in relatively narrow band compounds with strong Jahn-Teller lattice distortion and charge/orbital correlations. The anomalous behaviors of magnons in these compounds indicate the likelihood of cooperative excitations involving spin, lattice, as well as orbital degrees of freedom.
What happens to ferromagnetism at the surfaces and interfaces of manganites? With the competition between charge, spin, and orbital degrees of freedom, it is not surprising that the surface behavior may be profoundly different than that of the bulk. Using a powerful combination of two surface probes, tunneling and polarized x-ray interactions, this paper reviews our work on the nature of the electronic and magnetic states at manganite surfaces and interfaces. The general observation is that ferromagnetism is not the lowest energy state at the surface or interface, which results in a suppression or even loss of ferromagnetic order at the surface. Two cases will be discussed ranging from the surface of the quasi-2D bilayer manganite (La$_{2-2x}$Sr$_{1+2x}$Mn$_2$O$_7$) to the 3D Perovskite (La$_{2/3}$Sr$_{1/3}$MnO$_3$)/SrTiO$_3$ interface. For the bilayer manganite, that is, ferromagnetic and conducting in the bulk, these probes present clear evidence for an intrinsic insulating non-ferromagnetic surface layer atop adjacent subsurface layers that display the full bulk magnetization. This abrupt intrinsic magnetic interface is attributed to the weak inter-bilayer coupling native to these quasi-two-dimensional materials. This is in marked contrast to the non-layered manganite system (La$_{2/3}$Sr$_{1/3}$MnO$_3$/SrTiO$_3$), whose magnetization near the interface is less than half the bulk value at low temperatures and decreases with increasing temperature at a faster rate than the bulk.
Using the Lanczos method in linear chains we study the double exchange model in the low concentration limit, including an antiferromagnetic super-exchange K. In the strong coupling limit we find that the ground state contains ferromagnetic polarons whose length is very sensitive to the value of K/t. We investigate the dispersion relation, the trapping by impurities, and the interaction between these polarons. As the overlap between polarons increases, by decreasing K/t, the effective interaction between them changes from antiferromagnetic to ferromagnetic. The scaling to the thermodynamic limit suggests an attractive interaction in the strong coupling regime (J_h > t) and no binding in the weak limit (J_h simeq t).
We report measurements of the resistivity in the ferromagnetic state of epitaxial thin films of La_{1-x}Ca_{x}MnO_{3} and the low temperature specific heat of a polycrystalline La_{0.8}Ca_{0.2}MnO_{3}. The resistivity below 100 K can be well fitted by rho - rho_{o} = E omega_{s}/sinh^{2}(hbar omega_{s}/2k_{B}T) with hbar omega_{s}/k_{B} simeq 100 K and E being a constant. Such behavior is consistent with small-polaron coherent motion which involves a relaxation due to a soft optical phonon mode. The specific heat data also suggest the existence of such a phonon mode. The present results thus provide evidence for small-polaron metallic conduction in the ferromagnetic state of manganites.
We argue that in lightly hole doped perovskite-type Mn oxides the holes (Mn$^{4+}$ sites) are surrounded by nearest neighbor Mn$^{3+}$ sites in which the occupied $3d$ orbitals have their lobes directed towards the central hole (Mn$^{4+}$) site and with spins coupled ferromagnetically to the central spin. This composite object, which can be viewed as a combined orbital-spin-lattice polaron, is accompanied by the breathing type (Mn$^{4+}$) and Jahn-Teller type (Mn$^{3+}$) local lattice distortions. We present calculations which indicate that for certain doping levels these orbital polarons may crystallize into a charge and orbitally ordered ferromagnetic insulating state.
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