No Arabic abstract
Using a microscopic numerical approach suitable to describe disordered antiferromagnets, with application to $Fe_{x}Zn_{1-x}F_{2}$, it is shown that the characteristics of the spin glass phase found for $x=0.25$ is much in agreement with the scenario predicted by the scaling theory of the droplet model.
We use high temperature series expansions to study the $pm J$ Ising spin-glass in a magnetic field in $d$-dimensional hypercubic lattices for $d=5, 6, 7$ and $8$, and in the infinite-range Sherrington-Kirkpatrick (SK) model. The expansions are obtained in the variable $w=tanh^2{J/T}$ for arbitrary values of $u=tanh^2{h/T}$ complete to order $w^{10}$. We find that the scaling dimension $Delta$ associated with the ordering-field $h^2$ equals $2$ in the SK model and for $dge 6$. However, in agreement with the work of Fisher and Sompolinsky, there is a violation of scaling in a finite field, leading to an anomalous $h$-$T$ dependence of the Almeida-Thouless (AT) line in high dimensions, while scaling is restored as $d to 6$. Within the convergence of our series analysis, we present evidence supporting an AT line in $dge 6$. In $d=5$, the exponents $gamma$ and $Delta$ are substantially larger than mean-field values, but we do not see clear evidence for the AT line in $d=5$.
We study the quenched disordered magnetic system, which is obtained from the 2D SO(3) quantum Heisenberg model, on a square lattice, with nearest neighbors interaction, by taking a Gaussian random distribution of couplings centered in an antiferromagnetic coupling, $bar J>0$ and with a width $Delta J$. Using coherent spin states we can integrate over the random variables and map the system onto a field theory, which is a generalization of the SO(3) nonlinear sigma model with different flavors corresponding to the replicas, coupling parameter proportional to $bar J$ and having a quartic spin interaction proportional to the disorder ($Delta J$). After deriving the CP$^1$ version of the system, we perform a calculation of the free energy density in the limit of zero replicas, which fully includes the quantum fluctuations of the CP$^1$ fields $z_i$. We, thereby obtain the phase diagram of the system in terms of ($T, bar J, Delta J$). This presents an ordered antiferromagnetic (AF) phase, a paramagnetic (PM) phase and a spin-glass (SG) phase. A critical curve separating the PM and SG phases ends at a quantum critical point located between the AF and SG phases, at T=0. The Edwards-Anderson order parameter, as well as the magnetic susceptibilities are explicitly obtained in each of the three phases as a function of the three control parameters. The magnetic susceptibilities show a Curie-type behavior at high temperatures and exhibit a clear cusp, characteristic of the SG transition, at the transition line. The thermodynamic stability of the phases is investigated by a careful analysis of the Hessian matrix of the free energy. We show that all principal minors of the Hessian are positive in the limit of zero replicas, implying in particular that the SG phase is stable.
We present a mean-field solution for a quantum, short-range interacting, disordered, SO(3) Heisenberg spin model, in which the Gaussian distribution of couplings is centered in an AF coupling $bar J>0$, and which, for weak disorder, can be treated as a perturbation of the pure AF Heisenberg system. The phase diagram contains, apart from a Neel phase at T=0, spin-glass and paramagnetic phases whose thermodynamic stability is demonstrated by an analysis of the Hessian matrix of the free-energy. The magnetic susceptibilities exhibit the typical cusp of a spin-glass transition.
The nickelate Pr4Ni3O8 features quasi-two-dimensional layers consisting of three stacked square-planar NiO2 planes, in a similar way to the well-known cuprate superconductors. The mixed-valent nature of Ni and its metallic properties makes it a candidate for potentially unconventional superconductivity. We have synthesized Pr4Ni3O8 by topotactic reduction of Pr4Ni3O10 in 10 percent hydrogen gas, and report on measurements of powder-neutron diffraction, magnetization and muon-spin rotation (uSR). We find that Pr4Ni3O8 shows complicated spin-glass behavior with a distinct magnetic memory effect in the temperature range from 2 to 300 K and a freezing temperature T_s ~ 68 K. Moreover, the analysis of uSR spectra indicates two magnetic processes characterized by remarkably different relaxation rates: a slowly-relaxing signal, resulting from paramagnetic fluctuations of Pr/Ni ions, and a fast-relaxing signal, whose relaxation rate increases substantially below ~ 70 K which can be ascribed to the presence of short-range correlated regions. We conclude that the complex spin-freezing process in Pr4Ni3O8 is governed by these multiple magnetic interactions. It is possible that the complex magnetism in Pr4Ni3O8 is detrimental to the occurrence of superconductivity.
$Ni Cl_2$-$4SC(NH_2)_2$ (known as DTN) is a spin-1 material with a strong single-ion anisotropy that is regarded as a new candidate for Bose-Einstein condensation (BEC) of spin degrees of freedom. We present a systematic study of the low-energy excitation spectrum of DTN in the field-induced magnetically ordered phase by means of high-field electron spin resonance measurements at temperatures down to 0.45 K. We argue that two gapped modes observed in the experiment can be consistently interpreted within a four-sublattice antiferromagnet model with a finite interaction between two tetragonal subsystems and unbroken axial symmetry. The latter is crucial for the interpretation of the field-induced ordering in DTN in terms of BEC.