No Arabic abstract
Magnetic properties under the external field are investigated in low-carrier two-band systems, which may explain the nontrivial phase boundary found in temperature vs. magnetic field diagram discovered in some materials, such as filled-skutterudite compound CeOs$_{4}$Sb$_{12}$. Analysis is made both for the periodic Anderson model with the small-dispersive $f$ band and the simplified two parabolic band model in the vicinity of the Fermi level. The magnetic susceptibilities are calculated by using the random phase approximation. It is shown that the maximum value of the magnetic susceptibility perpendicular to the external field is enhanced and yields the anomalous phase boundary. By applying the magnetic field, the phase boundary shifts to higher temperature region in the insulating state with a small band gap. On the other hand, the similar phase boundary also appears in the semi-metallic states, in which the structure of the density of states in the vicinity of the Fermi level and the finite temperature effect are essential.
Specific heat for single crystalline samples of Ce1-xLaxOs4Sb12 at zero-field and magnetic fields to 14 T is reported. Our results confirm enhanced value of the electronic specific heat coefficient in the paramagnetic state. They provide arguments for the intrinsic origin of the 1.1 K anomaly. This transition leads to opening of the gap at the Fermi surface. This low temperature state of CeOs4Sb12 is extremely sensitive to chemical impurities. 2% of La substituted for Ce suppresses the transition and reduces the electronic specific heat coefficient. The magnetic field response of the specific heat is also anomalous.
What is so unique in TlCuCl3 which drives so many unique magnetic features in this compound? To study these properties, here we employ a combination of ab-initio band structure, tight-binding model, and an effective quantum field theory. Within a density-functional theory (DFT) calculation, we find an unexpected bulk Dirac cone without spin-orbit coupling (SOC). Tracing back to its origin, we identify, for the first time, the presence of a Su-Schrieffer-Heeger (SSH) like dimerized Cu chain lying in the 3D crystal structure. The SSH chain, combined with SOC, stipulates an anisotropic 3D Dirac cone where chiral and helical states are intertwined. As a Heisenberg interaction is introduced, we show that the dimerized Cu sublattices of the SSH chain condensate into spin-singlet, dimerized magnets. In the magnetic ground state, we also find a topological phase, distinguished by the axion angle. Finally, to study how the topological axion term couples to magnetic excitations, we derive a Chern-Simons-Ginzburg-Landau action from the 3D SSH Hamiltonian. We find that axion term provides an additional mass term to the Higgs mode, and a lifetime to paramagnons, which are independent of the quantum critical physics. The axion-Higgs interplay can be probed with electric and magnetic field applied parallel or anti-parallel to each other.
Using the dynamical mean-field approximation we investigate formation of excitonic condensate in the two-band Hubbard model in the vicinity of the spin-state transition. With temperature and band filling as the control parameters we realize all symmetry allowed spin-triplet excitonic phases, some exhibiting a ferromagnetic polarization. While the transitions are first-order at low temperatures, at elevated temperatures continuous transitions are found that give rise to a multi-critical point. Rapid but continuous transition between ferromagnetic and non-magnetic excitonic phases allows switching of uniform magnetization by small changes of chemical potential.
We investigate the magnetism of a previously unexplored distorted spin-1/2 kagome model consisting of three symmetry-inequivalent nearest-neighbor antiferromagnetic Heisenberg couplings and uncover a rich ground state phase diagram even at the classical level. Using analytical arguments and numerical techniques we identify a collinear $vec{Q} = 0$ magnetic phase, two unusual non-collinear coplanar $vec{Q} = (1/3,1/3)$ phases and a classical spin liquid phase with a degenerate manifold of non-coplanar ground states, resembling the jammed spin liquid phase found in the context of a bond-disordered kagome antiferromagnet. We further show with density functional theory calculations that the recently synthesized Y-kapellasite $text{Y}_{text{3}}text{Cu}_{text{9}}text{(OH)}_{text{19}}text{Cl}_{text{8}}$ is a realization of this model and predict its ground state to lie in the region of $vec{Q} = (1/3,1/3)$ order, which remains stable even after inclusion of quantum fluctuation effects within variational Monte Carlo and pseudofermion functional renormalization group. Interestingly, the excitation spectrum of Y-kapellasite lies between that of an underlying triangular lattice of hexagons and a kagome lattice of trimers. The presented model opens a new direction in the study of kagome antiferromagnets.
We report complex metamagnetic transitions in single crystals of the new low carrier Kondo antiferromagnet YbRh3Si7. Electrical transport, magnetization, and specific heat measurements reveal antiferromagnetic order at T_N = 7.5 K. Neutron diffraction measurements show that the magnetic ground state of YbRh3Si7 is a collinear antiferromagnet where the moments are aligned in the ab plane. With such an ordered state, no metamagnetic transitions are expected when a magnetic field is applied along the c axis. It is therefore surprising that high field magnetization, torque, and resistivity measurements with H||c reveal two metamagnetic transitions at mu_0H_1 = 6.7 T and mu_0H_2 = 21 T. When the field is tilted away from the c axis, towards the ab plane, both metamagnetic transitions are shifted to higher fields. The first metamagnetic transition leads to an abrupt increase in the electrical resistivity, while the second transition is accompanied by a dramatic reduction in the electrical resistivity. Thus, the magnetic and electronic degrees of freedom in YbRh3Si7 are strongly coupled. We discuss the origin of the anomalous metamagnetism and conclude that it is related to competition between crystal electric field anisotropy and anisotropic exchange interactions.