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Register a new userManipulation of collective spin correlations in semiconductors with polarization squeezed vacuum
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We calculate the transfer rate of correlations from polarization entangled photons to the collective spin of a many-electron state in a two-band system. It is shown that when a semiconductor absorbs pairs of photons from a two-mode squeezed vacuum, certain fourth order electron-photon processes correlate the spins of the excited electron pairs of different quasi-momenta. Different distributions of the quantum Stokes vector of the light lead to either enhancement or reduction of the collective spin correlations, depending on the symmetry of the distribution. We find that as the squeezing of the light becomes non-classical, the spin correlations exhibit a crossover from being positive with a $sim N^2$ ($N$ is average photon number) scaling, to being negative with $sim N$ scaling, even when $N$ is not small. Negative spin correlations mean a preponderance of spin singlets in the optically generated state. We discuss the possibility to measure the collective spin correlations in a combined measurement of the Faraday rotation fluctuation spectrum and excitation density in a steady-state configuration.
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The effect of hyperfine interaction on the room-temperature defect-enabled spin filtering effect in GaNAs alloys is investigated both experimentally and theoretically through a master equation approach based on the hyperfine and Zeeman interaction between electron and nuclear spin of the spin filtering defect. We show that the nuclear spin polarization can be tuned through the optically induced spin polarization of conduction band electrons.
We report on theoretical and experimental study of the spin polarization recovery and Hanle effect for the charge carriers interacting with the fluctuating nuclear spins in the semiconductor structures. We start the theoretical description from the simplest model of static and isotropic nuclear spin fluctuations. Then we describe the modification of the polarization recovery and Hanle curves due to the anisotropy of the hyperfine interaction, finite nuclear spin correlation time, and the strong pulsed spin excitation. For the latter case, we describe the resonance spin amplification effect in the Faraday geometry and discuss the manifestations of the quantum Zeno effect. The set of the experimental results for various structures and experimental conditions is chosen to highlight the specific effects predicted theoretically. We show that the spin polarization recovery is a very valuable tool for addressing carrier spin dynamics in semiconductors and their nanostructures.
We consider a semiconductor quantum-well placed in a wave guide microcavity and interacting with the broadband squeezed vacuum radiation, which fills one mode of the wave guide with a large average occupation. The wave guide modifies the optical density of states so that the quantum well interacts mostly with the squeezed vacuum. The vacuum is squeezed around the externally controlled central frequency $om_0$, which is tuned above the electron-hole gap $E_g$, and induces fluctuations in the interband polarization of the quantum-well. The power spectrum of scattered light exhibits a peak around $om_0$, which is moreover non-Lorentzian and is a result of both the squeezing and the particle-hole continuum. The squeezing spectrum is qualitatively different from the atomic case. We discuss the possibility to observe the above phenomena in the presence of additional non-radiative (e-e, phonon) dephasing.
Photon-number correlation measurements are performed on bright squeezed vacuum states using a standard Bell-test setup, and quantum correlations are observed for conjugate polarization-frequency modes. We further test the entanglement witnesses for these states and demonstrate the violation of the separability criteria, which infers that all the macroscopic Bell states, containing typically $10^6$ photons per pulse, are polarization entangled. The study also reveals the symmetry of macroscopic Bell states with respect to local polarization transformations.
The resonance energy and the transition rate of atoms, molecules and solids were understood as their intrinsic properties in classical electromagnetism. With the development of quantum electrodynamics, it is realized that these quantities are linked to the coupling of the transition dipole and the quantum vacuum. Such effects can be greatly amplified in macroscopic many-body systems from virtual photon exchange between dipoles, but are often masked by inhomogeneity and pure dephasing, especially in solids. Here, we observe an exceptionally large renormalization of exciton resonance and radiative decay rate in transition metal dichalcogenides monolayers due to interactions with the vacuum in both absorption and emission spectroscopy. Tuning the vacuum energy density near the monolayer, we demonstrate control of cooperative Lamb shift, radiative decay, and valley polarization as well as control of the charged exciton emission. Our work establishes a simple and robust experimental system for vacuum engineering of cooperative matter-light interactions.
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