No Arabic abstract
We have studied the spin anisotropy in spin-singlet ground state compounds and the magnetic chirality, as measured by inelastic polarized neutron scattering techniques, in the chain-sublattice of Sr14Cu24O41. In-plane and out of plane magnetic fluctuations are measured to be anisotropic and further discussed in the light of the current hypothesis of spin-orbit coupling. We show that under appropriate conditions of magnetic field and neutron polarization, the textit{trivial} magnetic chirality selects only one of the Zeeman splitted triplet states for scattering and erases the other one that posses opposite helicity. Our analysis pertains to previous studies on dynamical magnetic chirality and chiral critical exponents, where the ground state is chiral itself, the so-called textit{non-trivial} dynamical magnetic chirality. As it turns out, both textit{trivial} and textit{non-trivial} dynamical magnetic chirality have identical selection rules for inelastic polarized neutron scattering experiments and it is not at all evident that they can be distinguished in a paramagnetic compound.
Non-coplanar spin textures with scalar spin chirality can generate effective magnetic field that deflects the motion of charge carriers, resulting in topological Hall effect (THE), a powerful probe of the ground state and low-energy excitations of correlated systems. However, spin chirality fluctuation in two-dimensional ferromagnets with perpendicular anisotropy has not been considered in prior studies. Herein, we report direct evidence of universal spin chirality fluctuation by probing the THE above the transition temperatures in two different ferromagnetic ultra-thin films, SrRuO$_3$ and V doped Sb$_2$Te$_3$. The temperature, magnetic field, thickness, and carrier type dependences of the THE signal, along with our Monte-Carlo simulations, unambiguously demonstrate that the spin chirality fluctuation is a universal phenomenon in two-dimensional Ising ferromagnets. Our discovery opens a new paradigm of exploring the spin chirality with topological Hall transport in two-dimensional magnets and beyond
We probed the local electronic properties of the mixed-valent Co(+4-x) triangular-lattice in Na{x}CoO{2}-yH{2}O by 59-Co NMR. We observed two distinct types of Co sites for x>=1/2, but the valence seems averaged out for x~1/3. Local spin fluctuations exhibit qualitatively the same trend down to ~100 K regardless of the carrier-concentration x, and hence the nature of the electronic ground state. A canonical Fermi-liquid behavior emerges below ~100 K only for x~1/3.
Quantum criticality in iron pnictides involves both the nematic and antiferromagnetic degrees of freedom, but the relationship between the two types of fluctuations has yet to be clarified. Here we study this problem in the presence of a small external uniaxial potential, which breaks the $C_4$-symmetry in the B$_{1g}$ sector. We establish an identity that connects the spin excitation anisotropy, which is the difference of the dynamical spin susceptibilities at $vec{Q}_1=left(pi,0right)$ and $vec{Q}_2=left(0,piright)$, with the dynamical magnetic susceptibility and static nematic susceptibility. Using this identity, we introduce a scaling procedure to determine the dynamical nematic susceptibility in the quantum critical regime, and illustrate the procedure for the case of the optimally Ni-doped BaFe$_2$As$_2$[Y. Song textit{et al.}, Phys. Rev. B 92, 180504 (2015)]. The implications of our results for the overall physics of the iron-based superconductors are discussed.
We use the state-of-the-art tensor network state method, specifically, the finite projected entangled pair state (PEPS) algorithm, to simulate the global phase diagram of spin-$1/2$ $J_1$-$J_2$ Heisenberg model on square lattices up to $24times 24$. We provide very solid evidences to show that the nature of the intermediate nonmagnetic phase is a gapless quantum spin liquid (QSL), whose spin-spin and dimer-dimer correlations both decay with a power law behavior. There also exists a valence-bond solid (VBS) phase in a very narrow region $0.56lesssim J_2/J_1leq0.61$ before the system enters the well known collinear antiferromagnetic phase. We stress that our work gives rise to the first solid PEPS results beyond the well established density matrix renormalization group (DMRG) through one-to-one direct benchmark for small system sizes. Thus our numerical evidences explicitly demonstrate the huge power of PEPS for solving long-standing 2D quantum many-body problems. The physical nature of the discovered gapless QSL and potential experimental implications are also addressed.
The magnetoelectric (ME) effects are investigated in a cubic compound SrCuTe2O6, in which uniform Cu2+ (S=1/2) spin chains with considerable spin frustration exhibit a concomitant antiferromagnetic transition and dielectric constant peak at TN=5.5 K. Pyroelectric Jp(T) and magnetoelectric current JME(H) measurements in the presence of a bias electric field are used to reveal that SrCuTe2O6 shows clear variations of Jp(T) across TN at constant magnetic fields. Furthermore, isothermal measurements of JME(H) also develop clear peaks at finite magnetic fields, of which traces are consistent with the spin-flop transitions observed in the magnetization studies. As a result, the anomalies observed in Jp(T) and JME(H) curves well match with the field-temperature phase diagram constructed from magnetization and dielectric constant measurements, demonstrating that SrCuTe2O6 is a new magnetoelectric compound with S=1/2 spin chains.