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Register a new userA multiexcitonic quantum dot in an optical microcavity
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We theoretically study the coupled modes of a medium-size quantum dot, which may confine a maximum of ten electron-hole pairs, and a single photonic mode of an optical microcavity. Ground-state and excitation energies, exciton-photon mixing in the wave functions and the emission of light from the microcavity are computed as functions of the pair-photon coupling strength, photon detuning, and polariton number.
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Mean-field evolution equations for the exciton and photon populations and polarizations (Bloch-Lamb equations) are written and numerically solved in order to describe the dynamics of electronic states in a quantum dot coupled to the photon field of a microcavity. The equations account for phase space filling effects and Coulomb interactions among carriers, and include also (in a phenomenological way) incoherent pumping of the quantum dot, photon losses through the microcavity mirrors, and electron-hole population decay due to spontaneous emission of the dot. When the dot may support more than one electron-hole pair, asymptotic oscillatory states, with periods between 0.5 and 1.5 ps, are found almost for any values of the system parameters.
We propose and characterize a two-photon emitter in a highly polarised, monochromatic and directional beam, realized by means of a quantum dot embedded in a linearly polarized cavity. In our scheme, the cavity frequency is tuned to half the frequency of the biexciton (two excitons with opposite spins) and largely detuned from the excitons thanks to the large biexciton binding energy. We show how the emission can be Purcell enhanced by several orders of magnitude into the two-photon channel for available experimental systems.
The Jaynes-Cummings model, describing the interaction between a single two-level system and a photonic mode, has been used to describe a large variety of systems, ranging from cavity quantum electrodynamics, trapped ions, to superconducting qubits coupled to resonators. Recently there has been renewed interest in studying the quantum strong-coupling (QSC) regime, where states with photon number greater than one are excited. This regime has been recently achieved in semiconductor nanostructures, where a quantum dot is trapped in a planar microcavity. Here we study the quantum strong-coupling regime by calculating its photoluminescence (PL) properties under a pulsed excitation. We discuss the changes in the PL as the QSC regime is reached, which transitions between a peak around the cavity resonance to a doublet. We particularly examine the variations of the PL in the time domain, under regimes of short and long pulse times relative to the microcavity decay time.
We demonstrate that the spin of a Cr atom in a quantum dot (QD) can be controlled optically and we discuss the main properties of this single spin system. The photoluminescence of individual Cr-doped QDs and their evolution in magnetic field reveal a large magnetic anisotropy of the Cr spin induced by local strain. This results in a splitting of the Cr spin states and in a thermalization on the lower energy states states S$_z$=0 and S$_z$=$pm$1. The magneto-optical properties of Cr-doped QDs can be modelled by an effective spin Hamiltonian including the spin to strain coupling and the influence of the QD symmetry. We also show that a single Cr spin can be prepared by resonant optical pumping. Monitoring the intensity of the resonant fluorescence of the QD during this process permits to probe the dynamics of the optical initialization of the spin. Hole-Cr flip-flops induced by an interplay of the hole-Cr exchange interaction and the coupling with acoustic phonons are the main source of relaxation that explains the efficient resonant optical pumping. The Cr spin relaxation time is measured in the $mu s$ range. We evidence that a Cr spin couples to non-equilibrium acoustic phonons generated during the optical excitation inside or near the QD). Finally we show that the energy of any spin state of an individual Cr atom can be independently tuned by a resonant single mode laser through the optical Stark effect. All these properties make Cr-doped QDs very promising for the development of hybrid spin-mechanical systems where a coherent mechanical driving of an individual spin in an oscillator is required.
We review the practical conditions required to achieve a non-equilibrium BEC driven by quantum dynamics in a system comprising a microcavity field mode and a distribution of localised two-level systems driven to a step-like population inversion profile. A candidate system based on eight 3.8nm layers of In(0.23)Ga(0.77)As in GaAs shows promising characteristics with regard to the total dipole strength which can be coupled to the field mode.
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