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Register a new userLocal electronic structure near oxygen dopants in BSCCO-2212: a window on the high-Tc pair mechanism?
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The cuprate material BSCCO-2212 is believed to be doped by a combination of cation switching and excess oxygen. The interstitial oxygen dopants are of particular interest because scanning tunnelling microscopy (STM) experiments have shown that they are positively correlated with the local value of the superconducting gap, and calculations suggest that the fundamental attraction between electrons is modulated locally. In this work, we use density functional theory to try to ascertain which locations in the crystal are energetically most favorable for the O dopant atoms, and how the surrounding cage of atoms deforms. Our results provide support for the identification of STM resonances at -1eV with dopant interstitial O atoms, and show how the local electronic structure is modified nearby.
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Unveiling the nature of the bosonic excitations that mediate the formation of Cooper pairs is a key issue for understanding unconventional superconductivity. A fundamen- tal step toward this goal would be to identify the relative weight of the electronic and phononic contributions to the overall frequency (Omega) dependent bosonic function, Pi(Omega). We perform optical spectroscopy on Bi2212 crystals with simultaneous time- and frequency-resolution; this technique allows us to disentangle the electronic and phononic contributions by their different temporal evolution. The strength of the interaction ({lambda}~1.1) with the electronic excitations and their spectral distribution fully account for the high critical temperature of the superconducting phase transition.
We report measurements of anamolously large dissipative conductivities in BiSrCaCuO(2212) at low temperatures. We have measured the complex conductivity of BSCCO thin films at 100-600 GHz as a function of doping from the underdoped to the overdoped state. At low temperatures there exists a residual dissipative conductivity which scales with the T=0 superfluid density as the doping is varied. This residual dissipative conductivity is larger than the possible contribution from a thermal population of quasiparticles at the d-wave gap nodes.
We have measured the complex conductivity of a BSCCO(2212) thin film between 0.2 and 1.0 THz. We find the conductivity in the superconducting state to be well described as the sum of contributions from quasiparticles, the condensate, and order parameter fluctuations which draw 30% of the spectral weight from the condensate. An analysis based on this decomposition yields a quasiparticle scattering rate on the order of k_(B)*T/(hbar) for temperatures below Tc.
We present results of density functional theory (DFT) calculation of the structural supermodulation in BSCCO-2212 structure, and show that the supermodulation is indeed a spontaneous symmetry breaking of the nominal crystal symmetry, rather than a phenomenon driven by interstitial O dopants. The structure obtained is in excellent quantitative agreement with recent x-ray studies, and reproduces several qualitative aspects of scanning tunnelling microscopy (STM) experiments as well. The primary structural modulation affecting the CuO_2 plane is found to be a buckling wave of tilted CuO_5 half-octahedra, with maximum tilt angle near the phase of the supermodulation where recent STM experiments have discovered an enhancement of the superconducting gap. We argue that the tilting of the half-octahedra and concommitant planar buckling are directly modulating the superconducting pair interaction.
We use scanning tunneling microscopy to visualize the atomic-scale electronic states induced by a pair of hole dopants in Ca2CuO2Cl2 parent Mott insulator of cuprates. We find that when the two dopants approach each other, the transfer of spectral weight from high energy Hubbard band to low energy in-gap state creates a broad peak and nearly V-shaped gap around the Fermi level. The peak position shows a sudden drop at distance around 4 a0 and then remains almost constant. The in-gap states exhibit peculiar spatial distributions depending on the configuration of the two dopants relative to the underlying Cu lattice. These results shed important new lights on the evolution of low energy electronic states when a few holes are doped into parent cuprates.
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