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Dissociation of Feshbach Molecules into Different Partial Waves

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 Added by Stephan Duerr
 Publication date 2005
  fields Physics
and research's language is English




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Ultracold molecules can be associated from ultracold atoms by ramping the magnetic field through a Feshbach resonance. A reverse ramp dissociates the molecules. Under suitable conditions, more than one outgoing partial wave can be populated. A theoretical model for this process is discussed here in detail. The model reveals the connection between the dissociation and the theory of multichannel scattering resonances. In particular, the decay rate, the branching ratio, and the relative phase between the partial waves can be predicted from theory or extracted from experiment. The results are applicable to our recent experiment in 87Rb, which has a d-wave shape resonance.



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We study the spontaneous dissociation of diatomic molecules produced in cold atomic gases via magnetically tunable Feshbach resonances. We provide a universal formula for the lifetime of these molecules that relates their decay to the scattering length and the loss rate constant for inelastic spin relaxation. Our universal treatment as well as our exact coupled channels calculations for $^{85}$Rb dimers predict a suppression of the decay over several orders of magnitude when the scattering length is increased. Our predictions are in good agreement with recent measurements of the lifetime of $^{85}$Rb$_2$.
We present measurements of the loss-rate coefficients K_am and K_mm caused by inelastic atom-molecule and molecule-molecule collisions. A thermal cloud of atomic 87Rb is prepared in an optical dipole trap. A magnetic field is ramped across the Feshbach resonance at 1007.4 G. This associates atom pairs to molecules. A measurement of the molecule loss at 1005.8 G yields K_am=2 10^-10 cm^3/s. Additionally, the atoms can be removed with blast light. In this case, the measured molecule loss yields K_mm=3 10^-10 cm^3/s.
We analyze the temporal behavior of the survival probability of an unstable $^6$Li Feshbach molecule close to the BCS-BEC crossover. We find different instances of nonexponential decay as the magnetic field approaches the resonance value, at which the molecule becomes stable. We observe a transition from an exponential decay towards a regime dominated by a stretched-exponential law.
We investigate the phase diagram of a two-species Bose-Hubbard model describing atoms and molecules on a lattice, interacting via a Feshbach resonance. We identify a region where the system exhibits an exotic super-Mott phase and regions with phases characterized by atomic and/or molecular condensates. Our approach is based on a recently developed exact quantum Monte Carlo algorithm: the Stochastic Green Function algorithm with tunable directionality. We confirm some of the results predicted by mean-field studies, but we also find disagreement with these studies. In particular, we find a phase with an atomic but no molecular condensate, which is missing in all mean-field phase diagrams.
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