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High-energy Cu spin excitations in PrBa2Cu3O6+x

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 Added by Andrew Boothroyd
 Publication date 2005
  fields Physics
and research's language is English




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This paper describes high-energy neutron inelastic scattering measurements of propagating magnetic excitations in PrBa2Cu3O6+x (x approx 0.2 and 0.93). The measurements probe the acoustic and optic modes of the antiferromagnetically-ordered copper--oxygen bilayers in the energy range 50-150 meV. The observed magnon dispersion can be described satisfactorily in this energy range by a spin wave model including intra- and inter-layer nearest-neighbour exchange constants J_parallel and J_perp. We find J_parallel = 127 +/- 10 meV and J_perp = 5.5 +/- 0.9 meV. The value of J_parallel is virtually the same as that found in YBa2Cu3O6.2, but J_perp is a factor of two smaller. To within experimental error the values of J_parallel and J_perp for PrBa2Cu3O6+x do not vary with oxygen doping.

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Low-energy electron excitation spectra were measured on a single crystal of a typical iron-based superconductor PrFeAsO$_{0.7}$ using resonant inelastic X-ray scattering (RIXS) at the Fe-$L_3$ edge. Characteristic RIXS features are clearly observed around 0.5, 1-1.5 and 2-3 eV energy losses. These excitations are analyzed microscopically with theoretical calculations using a 22-orbital model derived from first-principles electronic structure calculation. Based on the agreement with the experiment, the RIXS features are assigned to Fe-$d$ orbital excitations which, at low energies, are accompanied by spin flipping and dominated by Fe $d_{yz}$ and $d_{xz}$ orbital characters. Furthermore, our calculations suggest dispersive momentum dependence of the RIXS excitations below 0.5 eV, and predict remarkable splitting and merging of the lower-energy excitations in momentum space. Those excitations, which were not observed in the present experiment, highlight the potential of RIXS with an improved energy resolution to unravel new details of the electronic structure of the iron-based superconductors.
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