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Register a new userPressure dependence of magnetism in URu2Si2
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Neutron-scattering and specific-heat measurements of the heavy-fermion superconductor URu2Si2 under hydrostatic pressure and with Rh-doping [U(Ru{0.98}Rh{0.02})2Si2] show the existence of two magnetic phase transitions. At the second-order phase transition Tm ≈ 17.5 K, a tiny ordered moment is established, while at TM < Tm, a first-order phase transition (under pressure or doping) gives rise to a large moment. The results can be understood in terms of a hidden OP Psi coupled to the ordered moment m, where m and Psi have the same symmetry.
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CeRhIn$_5$ provides a textbook example of quantum criticality in a heavy fermion system: Pressure suppresses local-moment antiferromagnetic (AFM) order and induces superconductivity in a dome around the associated quantum critical point (QCP) near $p_{c} approx 23,$kbar. Strong magnetic fields also suppress the AFM order at a field-induced QCP at $B_{rm c}approx 50,$T. In its vicinity, a nematic phase at $B^*approx 28,$T characterized by a large in-plane resistivity anisotropy emerges. Here, we directly investigate the interrelation between these phenomena via magnetoresistivity measurements under high pressure. As pressure increases, the nematic transition shifts to higher fields, until it vanishes just below $p_{rm c}$. While pressure suppresses magnetic order in zero field as $p_{rm c}$ is approached, we find magnetism to strengthen under strong magnetic fields due to suppression of the Kondo effect. We reveal a strongly non-mean-field-like phase diagram, much richer than the common local-moment description of CeRhIn$_5$ would suggest.
Resistivity and specific heat measurements were performed in the low carrier unconventional superconductor URu2Si2 on various samples with very different qualities. The superconducting transition temperature (TSC) and the hidden order transition temperature (THO) of these crystals were evaluated as a function of the residual resistivity ratio (RRR). In high quality single crystals the resistivity does not seem to follow a T2 dependence above TSC, indicating that the Fermi liquid regime is restricted to low temperatures. However, an analysis of the isothermal longitudinal magnetoresistivity points out that the T2 dependence may be spoiled by residual inhomogeneous superconducting contribution. We discuss a possible scenario concerning the distribution of TSC related with the fact that the hidden order phase is very sensitive to the pressure inhomogeneity.
We report 29Si nuclear magnetic resonance measurements of single crystals and aligned powders of URu2Si2 under pressure in the hidden order and paramagnetic phases. We find that the Knight shift decreases with applied pressure, consistent with previous measurements of the static magnetic susceptibility. Previous measurements of the spin lattice relaxation time revealed a partial suppression of the density of states below 30 K. This suppression persists under pressure, and the onset temperature is mildly enhanced.
The pressure-temperature phase diagram of the heavy-electron superconductor URu2Si2 has been reinvestigated by ac-susceptibility and elastic neutron-scattering (NS) measurements performed on a small single-crystalline rod (2 mm in diameter, 6 mm in length) in a Cu-Be clamp-type high-pressure cell (P < 1.1 GPa). At ambient pressure, this sample shows the weakest antiferromagnetic (AF) Bragg reflections reported so far, corresponding to the volume-averaged staggered moment of mord ~ 0.011 mB/U. Under applied pressure, the AF scattering intensity exhibits a sharp increase at P ~ 0.7 GPa at low temperatures. The saturation value of the AF scattering intensity above 0.7 GPa corresponds to mord ~ 0.41 mB/U, which is in good agreement with that (~ 0.39 mB/U) observed above 1.5 GPa in our previous NS measurements. The superconductivity is dramatically suppressed by the evolution of AF phase, indicating that the superconducting state coexists only with the hidden order phase. The presence of parasitic ferro- and/or antiferromagnetic phases with transition temperatures T1star =120(5) K, T2star = 36(3) K and T3star = 16.5(5) K and their relationship to the low-T ordered phases are also discussed.
We describe here recent inelastic neutron scattering experiments on the heavy fermion compound URu2Si2 realized in order to clarify the nature of the hidden order (HO) phase which occurs below T_0 = 17.5 K at ambient pressure. The choice was to measure at a given pressure P where the system will go, by lowering the temperature, successively from paramagnetic (PM) to HO and then to antiferromagnetic phase (AF). Furthermore, in order to verify the selection of the pressure, a macroscopic detection of the phase transitions was also achieved in situ via its thermal expansion response detected by a strain gauge glued on the crystal. Just above P_x = 0.5 GPa, where the ground state switches from HO to AF, the Q_0 = (1, 0, 0) excitation disappears while the excitation at the incommensurate wavevector Q_1 = (1.4, 0, 0) remains. Thus, the Q_0 = (1, 0, 0) excitation is intrinsic only in the HO phase. This result is reinforced by studies where now pressure and magnetic field $H$ can be used as tuning variable. Above P_x, the AF phase at low temperature is destroyed by a magnetic field larger than H_AF (collapse of the AF Q_0 = (1, 0, 0) Bragg reflection). The field reentrance of the HO phase is demonstrated by the reappearance of its characteristic Q_0 = (1, 0, 0) excitation. The recovery of a PM phase will only be achieved far above H_AF at H_M approx 35 T. To determine the P-H-T phase diagram of URu2Si2, macroscopic measurements of the thermal expansion were realized with a strain gauge. The reentrant magnetic field increases strongly with pressure. Finally, to investigate the interplay between superconductivity (SC) and spin dynamics, new inelastic neutron scattering experiments are reported down to 0.4 K, far below the superconducting critical temperature T_SC approx 1.3 K as measured on our crystal by diamagnetic shielding.
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