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Register a new userMagnetic phases and reorientation transitions in antiferromagnetically coupled multilayers
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In antiferromagnetically coupled superlattices grown on (001) faces of cubic substrates, e.g. based on materials combinations as Co/Cu, Fe/Si, Co/Cr, or Fe/Cr, the magnetic states evolve under competing influence of bilinear and biquadratic exchange interactions, surface-enhanced four-fold in-plane anisotropy, and specific finite-size effects. Using phenomenological (micromagnetic) theory, a comprehensive survey of the magnetic states and reorientation transitions has been carried out for multilayer systems with even number of ferromagnetic sub-layers and magnetizations in the plane. In two-layer systems (N=2) the phase diagrams in dependence on components of the applied field in the plane include ``swallow-tail type regions of (metastable) multistate co-existence and a number of continuous and discontinuous reorientation transitions induced by radial and transversal components of the applied field. In multilayers (N ge 4) noncollinear states are spatially inhomogeneous with magnetization varying across the multilayer stack. For weak four-fold anisotropy the magnetic states under influence of an applied field evolve by a complex continuous reorientation into the saturated state. At higher anisotropy they transform into various inhomogeneous and asymmetric structures. The discontinuous transitions between the magnetic states in these two-layers and multilayers are characterized by broad ranges of multi-phase coexistence of the (metastable) states and give rise to specific transitional domain structures.
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Equilibrium spin configurations and their stability limits have been calculated for models of magnetic superlattices with a finite number of thin ferromagnetic layers coupled antiferromagnetically through (non-magnetic) spacers as Fe/Cr and Co/Ru multilayers. Depending on values of applied magnetic field and unaxial anisotropy, the system assumes collinear(antiferromagnetic, ferromagnetic, various ferrimagnetic) phases, or spatially inhomogeneous (symmetric spin-flop phase and asymmetric, canted and twisted, phases)via series of field induced continuous and discontinuous transitions. Contrary to semi-infinite systems a surface phase transition, so-called surface spin-flop, does not occur in the models with a finite number of layers. It is shown that discrete jumps observed in some Fe/Cr superlattices and interpreted as surface spin-flop transition are first-order volume transitions between different canted phases. Depending on the system several of these collinear and canted phases can exist as metastable states in broad ranges of the magnetic fields, which may cause severe hysteresis effects. The results explain magnetization processes in recent experiments on antiferromagnetic Fe/Cr superlattices.
In antiferromagnetically coupled multilayers with perpendicular anisotropy unusual multidomain textures can be stabilized due to a close competition between long-range demagnetization fields and short-range interlayer exchange coupling. In particular, the formation and evolution of specific topologically stable planar defects within the antiferromagnetic ground state, i.e. wall-like structures with a ferromagnetic configuration extended over a finite width, explain configurational hysteresis phenomena recently observed in [Co/Pt(Pd)]/Ru and [Co/Pt]/NiO multilayers. Within a phenomenological theory, we have analytically derived the equilibrium sizes of these ferroband defects as functions of the antiferromagnetic exchange, a bias magnetic field, and geometrical parameters of the multilayers. In the magnetic phase diagram, the existence region of the ferrobands mediates between the regions of patterns with sharp antiferromagnetic domain walls and regular arrays of ferromagnetic stripes. The theoretical results are supported by magnetic force microscopy images of the remanent states observed in [Co/Pt]/Ru.
The in-plane correlation lengths and magnetic disorder of magnetic domains in a transition metal multilayer have been studied using neutron scattering techniques. A new theoretical framework is presented connecting the observed scattering to the in-plane correlation length and the dispersion of the local magnetization vector about the mean macroscopic direction. The results unambiguously show the highly correlated nature of the antiferromagnetically coupled domain structure vertically throughout the multilayer. We are easily able to relate the neutron determined magnetic dispersion and domain correlations to magnetization and magnetotransport experiments.
A rich variety of specific multidomain textures recently observed in antiferromagnetically coupled multilayers with perpendicular anisotropy include regular (equilibrium) multidomain states as well as different types of topological magnetic defects. Within a phenomenological theory we have classified and analyzed the possible magnetic defects in the antiferromagnetic ground state and determine their structures. We have derived the optimal sizes of the defects as functions of the antiferromagnetic exchange, the applied magnetic field, and geometrical parameters of the multilayer. The calculated magnetic phase diagrams show the existence regions for all types of magnetic defects. Experimental investigations of the remanent states (observed after different magnetic pre-history) in [Co/Pt]/Ru multilayers with wedged Co layers reveal a corresponding succession of different magnetic defect domain types.
Antiferromagnetically coupled multilayers with perpendicular anisotropy, as [CoPt]/Ru, Co/Ir, Fe/Au, display ferromagnetic stripe phases as the ground states. It is theoretically shown that the antiferromagnetic interlayer exchange causes a relative shift of domains in adjacent layers. This ``exchange shift is responsible for several recently observed effects: an anomalous broadening of domain walls, the formation of so-called ``tiger-tail patterns, and a ``mixed state of antiferromagnetic and ferromagnetic domains in [CoPt]/Ru multilayers. The derived analitical relations between the values of the shift and the strength of antiferromagnetic coupling provide an effective method for a quantitative determination of the interlayer exchange interactions.
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