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Bound spinons in an antiferromagnetic S=1/2 chain with a staggered field

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 Added by Michel Kenzelmann
 Publication date 2003
  fields Physics
and research's language is English




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Inelastic neutron scattering was used to measure the magnetic field dependence of spin excitations in the antiferromagnetic S=1/2 chain CuCl_2 2(dimethylsulfoxide) (CDC) in the presence of uniform and staggered fields. Dispersive bound states emerge from a zero-field two-spinon continuum with different finite energy minima at wave numbers q=pi and q_i approx pi (1-2<S_z>). The ratios of the field dependent excitation energies are in excellent agreement with predictions for breather and soliton solutions to the quantum sine-Gordon model, the proposed low-energy theory for S=1/2 chains in a staggered field. The data are also consistent with the predicted soliton and n=1,2 breather polarizations and scattering cross sections.

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We report an experimental and theoretical study of the antiferromagnetic S=1/2 chain subject to uniform and staggered fields. Using inelastic neutron scattering, we observe a novel bound-spinon state at high energies in the linear chain compound CuCl2 * 2((CD3)2SO). The excitation is explained with a mean-field theory of interacting S=1/2 fermions and arises from the opening of a gap at the Fermi surface due to confining spinon interactions. The mean-field model also describes the wave-vector dependence of the bound-spinon states, particularly in regions where effects of the discrete lattice are important. We calculate the dynamic structure factor using exact diagonalization of finite length chains, obtaining excellent agreement with the experiments.
94 - N. Shibata , K. Ueda 2001
Thermodynamic properties of the S=1/2 Heisenberg chain in transverse staggered magnetic field H^y_s and uniform magnetic field H^x perpendicular to the staggered field is studied by the finite-temperature density-matrix renormalization-group method. The uniform and staggered magnetization and specific heat are calculated from zero temperature to high temperatures up to T/J=4 under various strength of magnetic fields from H^y_s/J, H^x/J=0 to 2.4. The specific heat and magnetization of the effective Hamiltonian of the Yb_4As_3 are also presented, and field induced gap formation and diverging magnetic susceptibility at low temperature are shown.
We investigate the low-temperature magnetic properties of the molecule-based chiral spin chain [Cu(pym)(H$_2$O)$_4$]SiF$_6cdot$H$_2$O (pym = pyrimidine). Electron-spin resonance, magnetometry and heat capacity measurements reveal the presence of staggered $g$ tensors, a rich low-temperature excitation spectrum, a staggered susceptibility and a spin gap that opens on the application of a magnetic field. These phenomena are reminiscent of those previously observed in non-chiral staggered chains, which are explicable within the sine-Gordon quantum-field theory. In the present case, however, although the sine-Gordon model accounts well for the form of the temperature-dependence of the heat capacity, the size of the gap and its measured linear field dependence do not fit with the sine-Gordon theory as it stands. We propose that the differences arise due to additional terms in the Hamiltonian resulting from the chiral structure of [Cu(pym)(H$_2$O)$_4$]SiF$_6cdot$H$_2$O, particularly a uniform Dzyaloshinskii-Moriya coupling and a four-fold periodic staggered field.
Anderson localization is a general phenomenon of wave physics, which stems from the interference between multiple scattering paths1,2. It was originally proposed for electrons in a crystal, but later was also observed for light3-5, microwaves6, ultrasound7,8, and ultracold atoms9-12. Actually, in a crystal, besides electrons there may exist other quasiparticles such as magnons and spinons. However the search for Anderson localization of these magnetic excitations is rare so far. Here we report the first observation of spinon localization in copper benzoate, an ideal compound of spin-1/2 antiferromagnetic Heisenberg chain, by ultra-low-temperature specific heat and thermal conductivity measurements. We find that while the spinon specific heat Cs displays linear temperature dependence down to 50 mK, the spinons thermal conductivity ks only manifests the linear temperature dependence down to 300 mK. Below 300 mK, ks/T decreases rapidly and vanishes at about 100 mK, which is a clear evidence for Anderson localization. Our finding opens a new window for studying such a fundamental phenomenon in condensed matter physics.
We have investigated the zero and finite temperature behaviors of the anisotropic antiferromagnetic Heisenberg XXZ spin-1/2 chain in the presence of a transverse magnetic field (h). The attention is concentrated on an interval of magnetic field between the factorizing field (h_f) and the critical one (h_c). The model presents a spin-flop phase for 0<h<h_f with an energy scale which is defined by the long range antiferromagnetic order while it undergoes an entanglement phase transition at h=h_f. The entanglement estimators clearly show that the entanglement is lost exactly at h=h_f which justifies different quantum correlations on both sides of the factorizing field. As a consequence of zero entanglement (at h=h_f) the ground state is known exactly as a product of single particle states which is the starting point for initiating a spin wave theory. The linear spin wave theory is implemented to obtain the specific heat and thermal entanglement of the model in the interested region. A double peak structure is found in the specific heat around h=h_f which manifests the existence of two energy scales in the system as a result of two competing orders before the critical point. These results are confirmed by the low temperature Lanczos data which we have computed.
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