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Superchemistry: dynamics of coupled atomic and molecular Bose-Einstein condensates

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 Added by Kheruntsyan
 Publication date 2001
  fields Physics
and research's language is English




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We analyze the dynamics of a dilute, trapped Bose-condensed atomic gas coupled to a diatomic molecular Bose gas by coherent Raman transitions. This system is shown to result in a new type of `superchemistry, in which giant collective oscillations between the atomic and molecular gas can occur. The phenomenon is caused by stimulated emission of bosonic atoms or molecules into their condensate phases.



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We explored the dynamics of how a Bose-Einstein condensate collapses and subsequently explodes when the balance of forces governing the size and shape of the condensate is suddenly altered. A condensates equilibrium size and shape is strongly affected by the inter-atomic interactions. Our ability to induce a collapse by switching the interactions from repulsive to attractive by tuning an externally-applied magnetic field yields a wealth of detailed information on the violent collapse process. We observe anisotropic atom bursts that explode from the condensate, atoms leaving the condensate in undetected forms, spikes appearing in the condensate wave function, and oscillating remnant condensates that survive the collapse. These all have curious dependencies on time, the strength of the interaction, and the number of condensate atoms. Although ours would seem to be a simple well-characterized system, our measurements reveal many interesting phenomena that challenge theoretical models.
149 - S. Choi , B. Sundaram 2009
An atomic Bose-Einstein condensate (BEC) is often described as a macroscopic object which can be approximated by a coherent state. This, on the surface, would appear to indicate that its behavior should be close to being classical. In this paper, we clarify the extent of how classical a BEC is by exploring the semiclassical equations for BECs under the mean field Gaussian approximation. Such equations describe the dynamics of a condensate in the classical limit in terms of the variables < x > and < p > as well as their respective variances. We compare the semiclassical solution with the full quantum solution based on the Gross-Pitaevskii Equation (GPE) and find that the interatomic interactions which generate nonlinearity make the system less classical. On the other hand, many qualitative features are captured by the semiclassical equations, and the equations to be solved are far less computationally intensive than solving the GPE which make them ideal for providing quick diagnostics, and for obtaining new intuitive insight.
The structure and stability of vortices in hybrid atomic-molecular Bose-Einstein condensates is analyzed in the framework of a two-component Gross-Pitaevskii-type model that describes the stimulated Raman-induced photoassociation process. New types of topological vortex states are predicted to exist in the coherently coupled two-component condensates even without a trap, and their nontrivial dynamics in the presence of losses is demonstrated.
We study stationary clusters of vortices and antivortices in dilute pancake-shaped Bose-Einstein condensates confined in nonrotating harmonic traps. Previous theoretical results on the stability properties of these topologically nontrivial excited states are seemingly contradicting. We clarify this situation by a systematic stability analysis. The energetic and dynamic stability of the clusters is determined from the corresponding elementary excitation spectra obtained by solving the Bogoliubov equations. Furthermore, we study the temporal evolution of the dynamically unstable clusters. The stability of the clusters and the characteristics of their destabilizing modes only depend on the effective strength of the interactions between particles and the trap anisotropy. For certain values of these parameters, there exist several dynamical instabilities, but we show that there are also regions in which some of the clusters are dynamically stable. Moreover, we observe that the dynamical instability of the clusters does not always imply their structural instability, and that for some dynamically unstable states annihilation of the vortices is followed by their regeneration, and revival of the cluster.
Motivated by recent observations of phase-segregated binary Bose-Einstein condensates, we propose a method to calculate the excess energy due to the interface tension of a trapped configuration. By this method one should be able to numerically reproduce the experimental data by means of a simple Thomas-Fermi approximation, combined with interface excess terms and the Laplace equation. Using the Gross-Pitaevskii theory, we find expressions for the interface excesses which are accurate in a very broad range of the interspecies and intraspecies interaction parameters. We also present finite-temperature corrections to the interface tension which, aside from the regime of weak segregation, turn out to be small.
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