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Register a new userThermodynamics of Two Dimensional Magnetic Nanoparticles
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A two dimensional magnetic particle in the presence of an external magnetic field is studied. Equilibrium thermodynamical properties are derived by evaluating analytically the partition function. When the external field is applied perpendicular to the anisotropy axis the system exhibits a second order phase transition with order parameter being the magnetization parallel to the field. In this case the system is isomorph to a mechanical system consisting in a particle moving without friction in a circle rotating about its vertical diameter. Contrary to a paramagnetic particle, equilibrium magnetization shows a maximum at finite temperature. We also show that uniaxial anisotropy in a system of noninteracting particles can be missinterpreted as a ferromagnetic or antiferromagnetic coupling among the magnetic particles depending on the angle between anisotropy axis and magnetic field.
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We report on theoretical investigation of the magnetization reversal in two-dimensional arrays of ferromagnetic nano-particles with parameters of cobalt. The system was optimized for achieving the lowest coercivity in an array of particles located in the nodes of triangular, hexagonal and square grids. Based on the numerical solution of the non-stochastic Landau-Lifshitz-Gilbert equation we show that each particle distribution type is characterized with a proper optimal distance, allowing to lower the coercivity values for approximately 30% compared with the reference value obtained for a single nano-particle. It was shown that the reduction of coercivity occurs even if the particle position in the array is not very precise. In particular, the triangular particle arrangement maintained the same optimal distance between the particles under up to 20% random displacements of their position within the array.
Interstellar iron in the form of metallic iron nanoparticles may constitute a component of the interstellar dust. We compute the stability of iron nanoparticles to sublimation in the interstellar radiation field, finding that iron clusters can persist down to a radius of $simeq 4.5,$AA, and perhaps smaller. We employ laboratory data on small iron clusters to compute the photoelectric yields as a function of grain size and the resulting grain charge distribution in various interstellar environments, finding that iron nanoparticles can acquire negative charges particularly in regions with high gas temperatures and ionization fractions. If $gtrsim 10%$ of the interstellar iron is in the form of ultrasmall iron clusters, the photoelectric heating rate from dust may be increased by up to tens of percent relative to dust models with only carbonaceous and silicate grains.
This chapter is intended as a pedagogical introduction to the dynamics of optically levitated nanoparticles with a focus on the study of single particle thermodynamics. Much of the work studying thermodynamics with nano- and micro-particles has taken place in liquid, and this chapter will avoid reviewing this impressive body of work, focussing instead on studies of thermodynamics with nanoparticles levitated in a gas. For a recent literature review we refer the reader to Gieseler & Millen Entropy 20, 326 (2018). The authors will discuss extensions into the quantum regime where relevant throughout the chapter.
Using emph{in situ} measurements on a quasi two-dimensional, harmonically trapped $^{87}$Rb gas, we infer various equations of state for the equivalent homogeneous fluid. From the dependence of the total atom number and the central density of our clouds with the chemical potential and temperature, we obtain the equations of state for the pressure and the phase-space density. Then using the approximate scale invariance of this two-dimensional system, we determine the entropy per particle. We measure values as low as $0.06,kB$ in the strongly degenerate regime, which shows that a 2D Bose gas can constitute an efficient coolant for other quantum fluids. We also explain how to disentangle the various contributions (kinetic, potential, interaction) to the energy of the trapped gas using a time-of-flight method, from which we infer the reduction of density fluctuations in a non fully coherent cloud.
We study the thermodynamics of short-range interacting, two-dimensional bosons constrained to the lowest Landau level. When the temperature is higher than other energy scales of the problem, the partition function reduces to a multidimensional complex integral that can be handled by classical Monte Carlo techniques. This approach takes the quantization of the lowest Landau level orbits fully into account. We observe that the partition function can be expressed in terms of a function of a single combination of thermodynamic variables, which allows us to derive exact thermodynamic relations. We determine the asymptotic behavior of this function and compute some thermodynamic observables numerically.
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