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Register a new userEvidence for Braggoriton Excitations in Opal Photonic Crystals Infiltrated with Highly Polarizable Dyes
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N. Eradat
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We studied angle-dependent reflectivity spectra of opal photonic crystals infiltrated with cyanine dyes, which are highly polarizable media with very large Rabi frequency. We show that when resonance conditions between the exciton-polariton of the infiltrated dye and Bragg frequencies exist, then the Bragg stop band decomposes into two reflectivity bands with a semi-transparent spectral range in between that is due to light propagation inside the gap caused by the existence of braggoriton excitations. These novel excitations result from the interplay interaction between the Bragg gap with spatial modulation origin and the polariton gap due to the excitons, and may lead to optical communication traffic inside the gap of photonic crystals via channel waveguiding.
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Ordered binary and ternary photonic crystals, composed of different sized polymer-composite spheres with diameter ratios up to 120%, are generated using bending induced oscillatory shearing (BIOS). This viscoelastic system creates polydisperse equilibrium structures, producing mixed opaline colored films with greatly reduced requirements for particle monodispersity, and very different sphere size ratios, compared to other methods of nano-assembly.
The complete symmetry characterization of eigenstates in bare opal systems is obtained by means of group theory. This symmetry assignment has allowed us to identify several bands that cannot couple with an incident external plane wave. Our prediction is supported by layer-KKR calculations, which are also performed: the coupling coefficients between bulk modes and externally excited field tend to zero when symmetry properties mismatch.
Slow-light enhanced optical detection in liquid-infiltrated photonic crystals is theoretically studied. Using a scattering-matrix approach and the Wigner-Smith delay time concept, we show that optical absorbance benefits both from slow-light phenomena as well as a high filling factor of the energy residing in the liquid. Utilizing strongly dispersive photonic crystal structures, we numerically demonstrate how liquid-infiltrated photonic crystals facilitate enhanced light-matter interactions, by potentially up to an order of magnitude. The proposed concept provides strong opportunities for improving existing miniaturized absorbance cells for optical detection in lab-on-a-chip systems.
The dispersion properties of exciton polaritons in multiple-quantum-well based resonant photonic crystals are studied. In the case of structures with an elementary cell possessing a mirror symmetry with respect to its center, a powerful analytical method for deriving and analyzing dispersion laws of the respective normal modes is developed. The method is used to analyze band structure and dispersion properties of several types of resonant photonic crystals, which would not submit to analytical treatment by other approaches. These systems include multiple quantum well structures with an arbitrary periodic modulation of the dielectric function and structures with a complex elementary cell. Special attention was paid to determining conditions for superradiance (Bragg resonance) in these structures, and to the properties of the polariton stop band in the case when this condition is fulfilled (Bragg structures). The dependence of the band structure on the angle of propagation, the polarization of the wave, and the effects due to exciton homogeneous and inhomogeneous broadenings are considered, as well as dispersion properties of excitations in near-Bragg structures.
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