No Arabic abstract
Magnetization and neutron diffraction measurements indicate long-range antiferromagnetic ordering below TN=4 K in the 2D, S=1/2 Heisenberg antiferromagnet K2V3O8. The ordered state exhibits ``weak ferromagnetism and novel, field-induced spin reorientations. These experimental observations are well described by a classical, two-spin Heisenberg model incorporating Dzyaloshinskii-Moriya interactions and an additional c-axis anisotropy. This additional anisotropy can be accounted for by inclusion of the symmetric anisotropy term recently described by Kaplan, Shekhtman, Entin-Wohlman, and Aharony. This suggests that K2V3O8 may be a very unique system where the qualitative behavior relies on the presence of this symmetric anisotropy.
The ferrimagnetic spinel MnCr2S4 shows a variety of magnetic-field-induced phase transitions owing to bond frustration and strong spin-lattice coupling. However, the site-resolved magnetic properties at the respective field-induced phases in high magnetic fields remain elusive. Our soft x-ray magnetic circular dichroism studies up to 40 T directly evidence element-selective magnetic-moment reorientations in the field-induced phases. The complex magnetic structures are further supported by entropy changes extracted from magnetocaloric-effect measurements. Moreover, thermodynamic experiments reveal an unusual tetracritical point in the H-T phase diagram of MnCr2S4 due to strong spin-lattice coupling.
Orthorhombic single crystals of TbMn0.5Fe0.5O3 are found to exhibit spin-reorientation, magnetization reversal and weak ferromagnetism. Strong anisotropy effects are evident in the temperature dependent magnetization measurements along the three crystallographic axes a, b and c. A broad magnetic transition is visible at T_N (Fe/Mn) = 286 K due to paramagnetic to AxGyCz ordering. A sharp transition is observed at T_SR (Fe/Mn) = 28 K, which is pronounced along c axis in the form of a sharp jump in magnetization where the spins reorient to GxAyFz configuration. The negative magnetization observed below TSR Fe/Mn along c axis is explained in terms of domain wall pinning. A component of weak ferromagnetism is observed in field-scans along c-axis but below 28 K. Field-induced steps-like transitions are observed in hysteresis measurement along b axis below 28 K. It is noted that no sign of Tb-order is discernible down to 2 K. TbMn0.5Fe0.5O3 could be highlighted as a potential candidate to evaluate its magneto-dielectric effects across the magnetic transitions.
We have studied a EuFe2As2 single crystal by neutron diffraction under magnetic fields up to 3.5 T and temperatures down to 2 K. A field induced spin reorientation is observed in the presence of a magnetic field along both the a and c axes, respectively. Above critical field, the ground state antiferromagnetic configuration of Eu$^{2+}$ moments transforms into a ferromagnetic structure with moments along the applied field direction. The magnetic phase diagram for Eu magnetic sublattice in EuFe2As2 is presented. A considerable strain ($sim$0.9%) is induced by the magnetic field, caused by the realignment of the twinning structure. Furthermore, the realignment of the twinning structure is found to be reversible with the rebound of magnetic field, which suggested the existence of magnetic shape-memory effect. The Eu moment ordering exhibits close relationship with the twinning structure. We argue that the Zeeman energy in combined with magnetic anisotropy energy is responsible for the observed spin-lattice coupling.
We investigate a model of excitonic ordering (i.e electron-hole pair condensation) appropriate for the divalent hexaborides. We show that the inclusion of imperfectly nested electron hole Fermi surfaces can lead to the formation of an undoped excitonic metal phase. In addition, we find that weak ferromagnetism with compensated moments arises as a result of gapless excitations. We study the effect of the low lying excitations on the density of states, Fermi surface topology and optical conductivity and compare to available experimental data.
Weak itinerant ferromagnetism in YCo9Si4 below about 25 K is studied by means of magnetisation, specific heat, and resistivity measurements. Single crystal X-ray Rietveld refinements at room temperature reveal a fully ordered distribution of Y, Co and Si atoms within the tetragonal space group I4/mcm isostructural with LaCo9Si4. The latter exhibits itinerant electron metamagnetism with an induced moment of about 1 mu_B/f.u. above 6 T, whereas YCo9Si4 exhibits a spontaneous magnetisation M0~12 Am^2/kg at 2 K which corresponds to an ordered moment of about 1.6 mu_B/f.u. indicating weak itinerant ferromagnetism.