Subscribe to the gold package and get unlimited access to Shamra Academy
Register a new userMetamagnetism and critical fluctuations in high quality single crystals of the bilayer ruthenate Sr3Ru2O7
85
0
0.0
(
0
)
Ask ChatGPT about the research
No Arabic abstract
We report the results of low temperature transport, specific heat and magnetisation measurements on high quality single crystals of the bilayer perovskite Sr3Ru2O7, which is a close relative of the unconventional superconductor Sr2RuO4. Metamagnetism is observed, and transport and thermodynamic evidence for associated critical fluctuations is presented. These relatively unusual fluctuations might be pictured as variations in the Fermi surface topography itself. No equivalent behaviour has been observed in the metallic state of Sr2RuO4.
rate research
Read More
The local spectroscopic signatures of metamagnetic criticality in Sr3Ru2O7 were explored using scanning tunneling microscopy (STM). Singular features in the tunneling spectrum were found close to the Fermi level, as would be expected in a Stoner picture of itinerant electron metamagnetism. These features showed a pronounced magnetic field dependence across the metamagnetic critical point, which cannot be understood in terms of a naive Stoner theory. In addition, a pseudo-gap structure was observed over several tens of meV, accompanied by a c(2x2) superstructure in STM images. This result represents a new electronic ordering at the surface in the absence of any measurable surface reconstruction.
The Ruthenium based perovskites exhibit a wide variety of interesting collective phenomena related to magnetism originating from the Ru 4d electrons. Much remains unknown concerning the nature of magnetic fluctuations and excitations in these systems. We present results of detailed inelastic neutron scattering measurements of Sr3Ru2O7 as a function of temperature, probing the ferromagnetic fluctuations of the bilayer structure. A magnetic response is clearly visible for a range of temperatures, T = 3.8 K up to T = 100 K, and for energy transfers between 2 and 14 meV. These measurements indicate that the ferromagnetic fluctuations manifest in the bilayer structure factor persist to surprisingly large temperatures. This behavior may be related to the proximity of the system in zero magnetic field to the metamagnetic/ferromagnetic transition.
It was suggested that the two consecutive metamagnetic transitions and the large residual resistivity discovered in Sr$_3$Ru$_2$O$_7$ can be understood via the nematic order and its domains in a single layer system. However, a recently reported anisotropy between two longitudinal resistivities induced by tilting the magnetic field away from the c-axis cannot be explained within the single layer nematic picture. To fill the gap in our understanding within the nematic order scenario, we investigate the effects of bilayer coupling and in-plane magnetic field on the electronic nematic phases in a bilayer system. We propose that the in-plane magnetic field in the bilayer system modifies the energetics of the domain formation, since it breaks the degeneracy of two different nematic orientations. Thus the system reveals a pure nematic phase with a resistivity anisotropy in the presence of an in-plane magnetic field. In addition to the nematic phase, the bilayer coupling opens a novel route to a hidden nematic phase that preserves the x-y symmetry of the Fermi surfaces.
We report a detailed investigation into the metamagnetism of Sr3Ru2O7 at low temperatures for the magnetic field parallel to the ruthenium oxygen planes. The metamagnetism is studied as a function of temperature, magnetic field and sample quality using magnetisation, magnetotransport and specific heat as probes. From hysteretic behaviour in the magnetisation, we confirm earlier work and observe a finite temperature critical point at (5 T, >0.25 K). In our highest quality samples two-step metamagnetic transitions are additionally observed at 5.8 T and at 6.3 T, which coincide with a range of broad maximum in the magnetoresistance. At low temperatures, these two metamagnetic features each further split in two. Such behaviour of the multiple transitions are qualitatively different from the first order transition at 5.1 T.
When the transition temperature of a continuous phase transition is tuned to absolute zero, new ordered phases and physical behaviour emerge in the vicinity of the resulting quantum critical point. Sr3Ru2O7 can be tuned through quantum criticality with magnetic field at low temperature. Near its critical field Bc it displays the hallmark T-linear resistivity and a T log(1/T) electronic heat capacity behaviour of strange metals. However, these behaviours have not been related to any critical fluctuations. Here we use inelastic neutron scattering to reveal the presence of collective spin fluctuations whose relaxation time and strength show a nearly singular variation with magnetic field as Bc is approached. The large increase in the electronic heat capacity and entropy near Bc can be understood quantitatively in terms of the scattering of conduction electrons by these spin-fluctuations. On entering the spin density wave (SDW) phase present near Bc, the fluctuations become stronger suggesting that the SDW order is stabilised through an order-by-disorder mechanism.
Log in to be able to interact and post comments
comments
Fetching comments
Sign in to be able to follow your search criteria
