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Register a new userRare-event induced binding transition of heteropolymers
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Sequence heterogeneity broadens the binding transition of a polymer onto a linear or planar substrate. This effect is analyzed in a real-space renormalization group scheme designed to capture the statistics of rare events. In the strongly disordered regime, binding initiates at an exponentially rare set of ``good contacts. Renormalization of the contact potential yields a Kosterlitz-Thouless type transition in any dimension. This and other predictions are confirmed by extensive numerical simulations of a directed polymer interacting with a columnar defect.
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We propose an atomistic model for correlated particle dynamics in liquids and glasses predicting both slow stretched-exponential relaxation (SER) and fast compressed-exponential relaxation (CER). The model is based on the key concept of elastically interacting local relaxation events. SER is related to slowing down of dynamics of local relaxation events as a result of this interaction, whereas CER is related to the avalanche-like dynamics in the low-temperature glass state. The model predicts temperature dependence of SER and CER seen experimentally and recovers the simple, Debye, exponential decay at high temperature. Finally, we reproduce SER to CER crossover across the glass transition recently observed in metallic glasses.
Understanding the physics of glass formation remains one of the major unsolved challenges of condensed matter science. As a material solidifies into a glass, it exhibits a spectacular slowdown of the dynamics upon cooling or compression, but at the same time undergoes only minute structural changes. Among the numerous theories put forward to rationalize this complex behavior, Mode-Coupling Theory (MCT) stands out as the only framework that provides a fully first-principles-based description of glass phenomenology. This review outlines the key physical ingredients of MCT, its predictions, successes, and failures, as well as recent improvements of the theory. We also discuss the extension and application of MCT to the emerging field of non-equilibrium active soft matter
A theoretical treatment of deeply supercooled liquids is difficult because their properties emerge from spatial inhomogeneities that are self-induced, transient, and nanoscopic. I use computer simulations to analyse self-induced static and dynamic heterogeneity in equilibrium systems approaching the experimental glass transition. I characterise the broad sample-to-sample fluctuations of salient dynamic and thermodynamic properties in elementary mesoscopic systems. Findings regarding local lifetimes and distributions of dynamic heterogeneity are in excellent agreement with recent single molecule studies. Surprisingly broad thermodynamic fluctuations are also found, which correlate well with dynamics fluctuations, thus providing a local test of the thermodynamic origin of slow dynamics.
As in the preceding paper we aim at identifying the effective theory that describes the fluctuations of the local overlap with an equilibrium reference configuration close to a putative thermodynamic glass transition. We focus here on the case of finite-dimensional glass-forming systems, in particular supercooled liquids. The main difficulty for going beyond the mean-field treatment comes from the presence of diverging point-to-set spatial correlations. We introduce a variational low-temperature approximation scheme that allows us to account, at least in part, for the effect of these correlations. The outcome is an effective theory for the overlap fluctuations in terms of a random-field + random-bond Ising model with additional, power-law decaying, pair and multi-body interactions generated by the point-to-set correlations. This theory is much more tractable than the original problem. We check the robustness of the approximation scheme by applying it to a fully connected model already studied in the companion paper. We discuss the physical implications of this mapping for glass-forming liquids and the possibility it offers to determine the presence or not of a finite-temperature thermodynamic glass transition.
A wave function exposed to measurements undergoes pure state dynamics, with deterministic unitary and probabilistic measurement induced state updates, defining a quantum trajectory. For many-particle systems, the competition of these different elements of dynamics can give rise to a scenario similar to quantum phase transitions. To access it despite the randomness of single quantum trajectories, we construct an $n$-replica Keldysh field theory for the ensemble average of the $n$-th moment of the trajectory projector. A key finding is that this field theory decouples into one set of degrees of freedom that heats up indefinitely, while $n-1$ others can be cast into the form of pure state evolutions generated by an effective non-Hermitian Hamiltonian. This decoupling is exact for free theories, and useful for interacting ones. In particular, we study locally measured Dirac fermions in $(1+1)$ dimensions, which can be bosonized to a monitored interacting Luttinger liquid at long wavelengths. For this model, the non-Hermitian Hamiltonian corresponds to a quantum Sine-Gordon model with complex coefficients. A renormalization group analysis reveals a gapless critical phase with logarithmic entanglement entropy growth, and a gapped area law phase, separated by a Berezinskii-Kosterlitz-Thouless transition. The physical picture emerging here is a pinning of the trajectory wave function into eigenstates of the measurement operators upon increasing the monitoring rate.
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