No Arabic abstract
An optical antenna can convert a propagative optical radiation into a localized excitation, and reciprocally. Although optical antennas can be readily created using resonant nanoparticles (metallic or dielectric) as elementary building blocks, the realization of antennas sustaining multiple resonances over a broad range of frequencies remains a challenging task. Here, we use aluminum self-similar, fractal-like structures as broadband optical antennas. Using electron energy loss spectroscopy, we experimentally evidence that a single aluminum Cayley tree, a simple self-similar structure, sustains multiple plasmonic resonances. The spectral position of these resonances is scalable over a broad spectral range spanning two decades, from ultraviolet to mid-infrared. Such multi-resonant structures are highly desirable for applications ranging from non-linear optics to light harvesting and photodetection, as well as surface-enhanced infrared absorption spectroscopy.
Recent progress in nanotechnology has enabled us to fabricate subwavelength architectures that function as antennas for improving the exchange of optical energy with nanoscale matter. We describe the main features of optical antennas for enhancing quantum emitters and review designs that increase the spontaneous emission rate by orders of magnitude from the ultraviolet up to the near-infrared spectral range. To further explore how optical antennas may lead to unprecedented regimes of light-matter interaction, we draw a relationship between metal nanoparticles, radio-wave antennas and optical resonators. Our analysis points out how optical antennas may function as nanoscale resonators and how these may offer unique opportunities with respect to state-of-the-art microcavities.
Plasmonics aims to interface photonics and electronics. Finding optical, near-field analogues of much used electro-technical components is crucial to the success of such a platform. Here we present the plasmonic analogue of a non-reciprocal antenna. For non-reciprocality in a plasmonic context, the optical excitation and emission resonances of the antenna need to be an orthogonal set. We show that nonlinear excitation of metal nanoantennas creates a sufficient shift between excitation and emission wavelengths that they can be interpreted as decoupled, allowing for independent tuning of excitation and emission properties along different spatial dimensions. This leads, for given excitation wavelength and polarization, to independent optimization of emission intensity, frequency spectrum, polarization and angular spectrum. Non-reciprocal optical antennas of both gold and aluminum are characterized and shown to be useful as e.g. nonlinear signal transducers or nanoscale sources of widely tunable light.
The functionalities of a wide range of optical and opto-electronic devices are based on resonance effects and active tuning of the amplitude and wavelength response is often essential. Plasmonic nanostructures are an efficient way to create optical resonances, a prominent example is the extraordinary optical transmission (EOT) through arrays of nanoholes patterned in a metallic film. Tuning of resonances by heating, applying electrical or optical signals has proven to be more elusive, due to the lack of materials that can induce modulation over a broad spectral range and/or at high speeds. Here we show that nanopatterned metals combined with phase change materials (PCMs) can overcome this limitation due to the large change in optical constants which can be induced thermally or on an ultrafast timescale. We demonstrate resonance wavelength shifts as large as 385 nm - an order of magnitude higher than previously reported - by combining properly designed Au EOT nanostructures with Ge2Sb2Te5 (GST). Moreover, we show, through pump probe measurements, repeatable and reversible, large amplitude modulations in the resonances, especially at telecommunication wavelengths, over ps time scales and at powers far below those needed to produce a permanent phase transition. Our findings open a pathway to the design of hybrid metal PCM nanostructures with ultrafast and widely tuneable resonance responses, which hold potential impact on active nanophotonic devices such as tuneable optical filters, smart windows, biosensors and reconfigurable memories.
The design of nano-antennas is so far mainly inspired by radio-frequency technology. However, material properties and experimental settings need to be reconsidered at optical frequencies, which entails the need for alternative optimal antenna designs. Here a checkerboard-type, initially random array of gold cubes is subjected to evolutionary optimization. To illustrate the power of the approach we demonstrate that by optimizing the near-field intensity enhancement the evolutionary algorithm finds a new antenna geometry, essentially a split-ring/two-wire antenna hybrid which surpasses by far the performance of a conventional gap antenna by shifting the n=1 split-ring resonance into the optical regime.
The emission rate of a point dipole can be strongly increased in presence of a well-designed optical antenna. Yet, optical antenna design is largely based on radio-frequency rules, ignoring e.g.~ohmic losses and non-negligible field penetration in metals at optical frequencies. Here we combine reciprocity and Poyntings theorem to derive a set of optical-frequency antenna design rules for benchmarking and optimizing the performance of optical antennas driven by single quantum emitters. Based on these findings a novel plasmonic cavity antenna design is presented exhibiting a considerably improved performance compared to a reference two-wire antenna. Our work will be useful for the design of high-performance optical antennas and nanoresonators for diverse applications ranging from quantum optics to antenna-enhanced single-emitter spectroscopy and sensing.