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Experimental verification of the work fluctuation-dissipation relation for information-to-work conversion

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 Added by David Barker
 Publication date 2021
  fields Physics
and research's language is English




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We study experimentally work fluctuations in a Szilard engine that extracts work from information encoded as the occupancy of an electron level in a semiconductor quantum dot. We show that as the average work extracted per bit of information increases towards the Landauer limit $k_BT ln 2$, the work fluctuations decrease in accordance with the work fluctuation-dissipation relation. We compare the results to a protocol without measurement and feedback and show that when no information is used, the work output and fluctuations vanish simultaneously contrasting the information-to-energy conversion case where increasing amount of work is produced with decreasing fluctuations. Our work highlights the importance of fluctuations in the design of information-to-work conversion processes.



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In recent years, the study of heat to work conversion has been re-invigorated by nanotechnology. Steady-state devices do this conversion without any macroscopic moving parts, through steady-state flows of microscopic particles such as electrons, photons, phonons, etc. This review aims to introduce some of the theories used to describe these steady-state flows in a variety of mesoscopic or nanoscale systems. These theories are introduced in the context of idealized machines which convert heat into electrical power (heat-engines) or convert electrical power into a heat flow (refrigerators). In this sense, the machines could be categorized as thermoelectrics, although this should be understood to include photovoltaics when the heat source is the sun. As quantum mechanics is important for most such machines, they fall into the field of quantum thermodynamics. In many cases, the machines we consider have few degrees of freedom, however the reservoirs of heat and work that they interact with are assumed to be macroscopic. This review discusses different theories which can take into account different aspects of mesoscopic and nanoscale physics, such as coherent quantum transport, magnetic-field induced effects (including topological ones such as the quantum Hall effect), and single electron charging effects. It discusses the efficiency of thermoelectric conversion, and the thermoelectric figure of merit. More specifically, the theories presented are (i) linear response theory with or without magnetic fields, (ii) Landauer scattering theory in the linear response regime and far from equilibrium, (iii) Green-Kubo formula for strongly interacting systems within the linear response regime, (iv) rate equation analysis for small quantum machines with or without ..... (SEE THE PDF FOR THE REST OF THIS ABSTRACT)
Performances of work-to-work conversion are studied for a dissipative nonlinear quantum system with two isochromatic phase-shifted drives. It is shown that for weak Ohmic damping simultaneous maximization of efficiency with finite power yield and low power fluctuations can be achieved. Optimal performances of these three quantities are accompanied by a shortfall of the trade-off bound recently introduced for classical thermal machines. This bound can be undercut down to zero for sufficiently low temperature and weak dissipation, where the non-Markovian quantum nature dominates. Analytic results are given for linear thermodynamics. These general features can persist in the nonlinear driving regime near to a maximum of the power yield and a minimum of the power fluctuations. This broadens the scope to a new operation field beyond linear response.
Research on the out-of-equilibrium dynamics of quantum systems has so far produced important statements on the thermodynamics of small systems undergoing quantum mechanical evolutions. Key examples are provided by the Crooks and Jarzynski relations: taking into account fluctuations in non-equilibrium dynamics, such relations connect equilibrium properties of thermodynamical relevance with explicit non-equilibrium features. Although the experimental verification of such fundamental relations in the classical domain has encountered some success, their quantum mechanical version requires the assessment of the statistics of work performed by or onto an evolving quantum system, a step that has so far encountered considerable difficulties in its implementation due to the practical difficulty to perform reliable projective measurements of instantaneous energy states. In this paper, by exploiting a radical change in the characterization of the work distribution at the quantum level, we report the first experimental verification of the quantum Jarzynski identity and the Tasaki-Crooks relation following a quantum process implemented in a Nuclear Magnetic Resonance (NMR) system. Our experimental approach has enabled the full characterisation of the out-of-equilibrium dynamics of a quantum spin in a statistically significant way, thus embodying a key step towards the grounding of quantum-systems thermodynamics.
Universal phenomena far from equilibrium exhibit additional independent scaling exponents and functions as compared to thermal universal behavior. For the example of an ultracold Bose gas we simulate nonequilibrium transport processes in a universal scaling regime and show how they lead to the breaking of the fluctuation-dissipation relation. As a consequence, the scaling of spectral functions (commutators) and statistical correlations (anticommutators) between different points in time and space become linearly independent with distinct dynamic scaling exponents. As a macroscopic signature of this phenomenon we identify a transport peak in the statistical two-point correlator, which is absent in the spectral function showing the quasiparticle peaks of the Bose gas.
We propose a setup for a quantitative test of the quantum fluctuation theorem. It consists of a quantum conductor, driven by an external voltage source, and a classical inductor-capacitor circuit. The work done on the system by the voltage source can be expressed by the classical degrees of freedom of the LC circuit, which are measurable by conventional techniques. In this way the circuit acts as a classical detector to perform measurements of the quantum conductor. We prove that this definition is consistent with the work fluctuation theorem. The system under consideration is effectively described by a Langevin equation with non-Gaussian white noise. Our analysis extends the proof of the fluctuation theorem to this situation.
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