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Register a new userSystematics on production of superheavy nuclei $Z = 119-122$ in fusion-evaporation reactions
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The fusion dynamics on the formation of superheavy nuclei is investigated thoroughly within the dinuclear system model. The Monte Carlo approach is implemented into the nucleon transfer process for including all possible orientations, at which the dinuclear system is assumed to be formed at the touching configuration of dinuclear fragments. The production cross sections of superheavy nuclei Cn, Fl, Lv, Ts and Og are calculated and compared with the available data from Dubna. The evaporation residue excitation functions in the channels of pure neutrons and charged particles are analyzed systematically. The combinations with $^{44}$Sc, $^{48,50}$Ti, $^{49,51}$V, $^{52,54}$Cr, $^{58,62}$Fe and $^{62,64}$Ni bombarding the actinide nuclides $^{238}$U, $^{244}$Pu, $^{248}$Cm, $^{247,249}$Bk, $^{249,251}$Cf, $^{252}$Es and $^{243}$Am are calculated for producing the superheavy elements with Z=119-122. It is found that the production cross sections sensitively depend on the neutron richness of reaction system. The structure of evaporation residue excitation function is related to the neutron separation energy and fission barrier of compound nucleus.
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Within the framework of the dinuclear system model, production cross sections of proton-rich nuclei with charged numbers of Z=84-90 are investigated systematically. Possible combinations with the $^{28}$Si, $^{32}$S, $^{40}$Ar bombarding the target nuclides $^{165}$Ho, $^{169}$Tm, $^{170-174}$Yb, $^{175,176}$Lu, $^{174,176-180}$Hf and $^{181}$Ta are analyzed thoroughly. The optimal excitation energies and evaporation channels are proposed to produce the proton-rich nuclei. The systems are feasible to be constructed in experiments. It is found that the neutron shell closure of N=126 is of importance during the evaporation of neutrons. The experimental excitation functions in the $^{40}$Ar induced reactions can be nicely reproduced. The charged particle evaporation is comparable with neutrons in cooling the excited proton-rich nuclei, in particular for the channels with $alpha$ and proton evaporation. The production cross section increases with the mass asymmetry of colliding systems because of the decrease of the inner fusion barrier. The channels with pure neutron evaporation depend on the isotopic targets. But it is different for the channels with charged particles and more sensitive to the odd-even effect.
In this manuscript, we analyze the structural properties of $Z=119$ superheavy nuclei in the mass range of 284 $le$ A $le$ 375 within the framework of deformed relativistic mean field theory (RMF) and calculate the binding energy, radii, quadrupole deformation parameter, separation energies and density profile. Further, a competition between possible decay modes such as $alpha-$decay, $beta-$decay and spontaneous fission (SF) of the isotopic chain of $Z=119$ superheavy nuclei under study is systematically analyzed within self-consistent relativistic mean field model. Moreover, our analysis confirmed that $alpha-$decay is restricted within the mass range 284 $leq$ A $leq$ 296 and thus being the dominant decay channel in this mass range. However, for the mass range 297 $leq$ A $leq$ 375 the nuclei are unable to survive fission and hence SF is the principal mode of decay for these isotopes. There is no possibility of $beta-$decay for the considered isotopic chain. In addition, we forecasted the mode of decay $^{284-296}$119 as one $alpha$ chain from $^{284}$119 and $^{296}$119, two consistent $alpha$ chains from $^{285}$119 and $^{295}$119, three consistent $alpha$ chains from $^{286}$119 and $^{294}$119, four consistent alpha chains from $^{287}$119, six consistent alpha chains from $^{288-293}$119. Also from our analysis we inferred that for the isotopes $^{264-266,269}$Bh both $alpha$ decay and SF are equally competent and can decay via either of these two modes. Thus, such studies can be of great significance to the experimentalists in very near future for synthesizing $Z=119$ superheavy nuclei.
The fusion probability for the production of superheavy nuclei in cold fusion reactions was investigated and compared with recent experimental results for $^{48}$Ca, $^{50}$Ti, and $^{54}$Cr incident on a $^{208}$Pb target. Calculations were performed within the fusion-by-diffusion model (FbD) using new nuclear data tables by Jachimowicz et al. It is shown that the experimental data could be well explained within the framework of the FbD model. The saturation of the fusion probability at bombarding energies above the interaction barrier is reproduced. It emerges naturally from the physical effect of the suppression of contributions of higher partial waves in fusion reactions and is related to the critical angular momentum. The role of the difference in values of the rotational energies in the fusion saddle point and contact (sticking) configuration of the projectile-target system is discussed.
The production cross sections of heaviest isotopes of superheavy nuclei with charge numbers 112--118 are predicted in the $xn$--, $pxn$--, and $alpha xn$--evaporation channels of the $^{48}$Ca-induced complete fusion reactions for future experiments. The estimates of synthesis capabilities are based on a uniform and consistent set of input nuclear data. Nuclear masses, deformations, shell corrections, fission barriers, and decay energies are calculated within the macroscopic-microscopic approach for even-even, odd-Z, and odd-N nuclei. For odd systems, the blocking procedure is used. To find, the ground states via minimization and saddle points using Immersion Water flow technique, multidimensional deformation spaces, containing non-axially are used. As shown, current calculations based on a new set of mass and barriers, agree very well with experimentally known cross-sections, especially in the $3n$--evaporation channel. The dependencies of these predictions on the mass/fission barriers tables and fusion models are discussed. A way is shown to produce directly unknown superheavy isotopes in the $1n$-- or $2n$--evaporation channels. The synthesis of new superheavy isotopes unattainable in reactions with emission of neutrons is proposed in the promising channels with emission of protons ($sigma_{pxn} simeq 10-200$ fb) and alphas ($sigma_{alpha xn} simeq 5-500$ fb).
Structural properties and the decay modes of the superheavy elements Z $=$ 122, 120, 118 are studied in a microscopic framework. We evaluate the binding energy, one- and two- proton and neutron separation energy, shell correction and density profile of even and odd isotopes of Z $=$ 122, 120, 118 (284 $leq$ A $leq$ 352) which show a reasonable match with FRDM results and the available experimental data. Equillibrium shape and deformation of the superheavy region are predicted. We investigate the possible decay modes of this region specifically $alpha$-decay, spontaneous fission (SF) and the $beta$-decay and evaluate the probable $alpha$-decay chains. The phenomena of bubble like structure in the charge density is predicted in $^{330}$122, $^{292,328}$120 and $^{326}$118 with significant depletion fraction around 20-24$%$ which increases with increasing Coulomb energy and diminishes with increasing isospin (N$-$Z) values exhibiting the fact that the coloumb forces are the main driving force in the central depletion in superheavy systems.
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