No Arabic abstract
While typical theories of atom-light interactions treat the atomic medium as being smooth, it is well-known that microscopic optical effects driven by atomic granularity, dipole-dipole interactions, and multiple scattering can lead to important effects. Recently, for example, it was experimentally observed that these ingredients can lead to a fundamental, density-dependent dephasing of optical spin waves in a disordered atomic medium. Here, we go beyond the short-time and dilute limits considered previously, to develop a comprehensive theory of dephasing dynamics for arbitrary times and atomic densities. In particular, we develop a novel, non-perturbative theory based on strong disorder renormalization group, in order to quantitatively predict the dominant role that near-field optical interactions between nearby neighbors has in driving the dephasing process. This theory also enables one to capture the key features of the many-atom dephasing dynamics in terms of an effective single-atom model. These results should shed light on the limits imposed by near-field interactions on quantum optical phenomena in dense atomic media, and illustrate the promise of strong disorder renormalization group as a method of dealing with complex microscopic optical phenomena in such systems.
Quantum light-matter interfaces, based upon ensembles of cold atoms or other quantum emitters, are a vital platform for diverse quantum technologies and the exploration of fundamental quantum phenomena. Most of our understanding and modeling of such systems are based upon macroscopic theories, wherein the atoms are treated as a smooth, quantum polarizable medium. Although it is known that such approaches ignore a number of microscopic details, such as the granularity of atoms, dipole-dipole interactions and multiple scattering of light, the consequences of such effects in practical settings are usually mixed with background macroscopic effects and difficult to quantify. In this work we demonstrate a time-domain method to measure microscopically-driven optical effects in a background-free fashion, by transiently suppressing the macroscopic dynamics. With the method, we reveal a microscopic dipolar dephasing mechanism that generally limits the lifetime of the optical spin-wave order in a random gas. Theoretically, we show the dephasing effect emerges from the strong resonant dipole interaction between close-by atomic pairs.
We propose a method for measuring parity violation in neutral atoms. It is an adaptation of a seminal work by Fortson [Phys. Rev. Lett. {bf 70}, 2383 (1993)], proposing a scheme for a single trapped ion. In our version, a large sample of neutral atoms should be localised in an optical lattice overlapping a grid of detection sites, all tailored as the single site in Fortsons work. The methodology is of general applicability, but as an example we estimate the achievable signal in an experiment probing a nuclear spin independent parity violation on the line $6mathrm{s},^2mathrm{S}_{1/2}$--$5mathrm{d},^2mathrm{D}_{3/2}$ in $^{133}$Cs. The projected result is based on realistic parameters and textit{ab initio} calculations of transition amplitudes, using the relativistic coupled-cluster method. The final result is a predicted spectroscopic signature, evidencing parity violation, of the order of 1 Hz, for a sample of $10^8$ atoms. We show that a total interrogation time of 30000 s should suffice for achieving a precision of the order of 0.1% --- surpassing previous determinations of the weak charge in Cs by at least a factor of five.
Long-lived storage of arbitrary transverse multimodes is important for establishing a high-channel-capacity quantum network. Most of the pioneering works focused on atomic diffusion as the dominant impact on the retrieved pattern in an atom-based memory. In this work, we demonstrate that the unsynchronized Larmor precession of atoms in the inhomogeneous magnetic field dominates the distortion of the pattern stored in a cold-atom-based memory. We find that this distortion effect can be eliminated by applying a strong uniform polarization magnetic field. By preparing atoms in magnetically insensitive states, the destructive interference between different spin-wave components is diminished, and the stored localized patterns are synchronized further in a single spin-wave component; then, an obvious enhancement in preserving patterns for a long time is obtained. The reported results are very promising for studying transverse multimode decoherence in storage and high-dimensional quantum networks in the future.
Molecules are many body systems with a substantial amount of entanglement between their electrons. Is there a way to break the molecular bond of a diatomic molecule and obtain two atoms in their ground state which are still entangled and form a Bell-like state? We present a scheme that allows for the preparation of such entangled atomic states from single oxygen molecules on femtosecond time scales. The two neutral oxygen atoms are entangled in the magnetic quantum number of their valence electrons. In a time-delayed probe step, we employ non-adiabatic tunnel ionization, which is a magnetic quantum number-sensitive mechanism. We then investigate correlations by comparing single and double ionization probabilities of the Bell-like state. The experimental results agree with the predictions for an entangled state.
The problem of photoionization of atomic hydrogen in a white-dwarf-strength magnetic field is revisited to understand the existing discrepancies in the positive-energy spectra obtained by a variety of theoretical approaches reported in the literature. Oscillator strengths for photoionization are calculated with the adiabatic-basis-expansion method developed by Mota-Furtado and OMahony [Phys. Rev. A {bf 76}, 053405 (2007)]. A comparative study is performed between the adiabatic-basis-expansion method and our previously developed coupled-channel theory [Phys. Rev. A {bf 94}, 033422 (2016)]. A detailed analysis of the positive-energy spectra obtained here and those from other theoretical approaches shows that the adiabatic-basis-expansion method can produce more accurate positive-energy spectra than other reported approaches for low field strengths.