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The Cassini-Huygens mission measured the chemical abundances of the major components of Titans atmosphere, and analyses of the data revealed several as-yet unexplained anomalies in the methane and hydrogen profiles. We model the deceleration and ablation of meteors in Titans atmosphere to examine whether meteor energy deposition could explain, in part, two of these anomalies. Our simulations vary meteor entry mass, trajectory angle, and velocity, and follow changes in all three as our meteors descend into a realistic Titan atmosphere. For the smallest particles, which deliver the most mass and therefore energy to Titan, we find that the altitudes where energy deposition peaks correspond to those of the observed chemical anomalies. In the region directly above the anomalies, energy deposition by meteors is greater than energy deposition from ultraviolet photons, which are typically responsible for methane dissociation. Finally, we calculate the total amount of energy available for chemical reactions in question. Total meteor energy deposited is swamped by daytime ultraviolet light, but of course is the dominant source of energy for atmospheric chemistry at the relevant altitudes during the night.
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Titan harbors a dense, organic-rich atmosphere primarily composed of N$_2$ and CH$_4$, with lesser amounts of hydrocarbons and nitrogen-bearing species. As a result of high sensitivity observations by the Atacama Large Millimeter/submillimeter Array (ALMA) in Band 6 ($sim$230-272 GHz), we obtained the first spectroscopic detection of CH$_3$C$_3$N (methylcyanoacetylene or cyanopropyne) in Titans atmosphere through the observation of seven transitions in the $J = 64rightarrow63$ and $J = 62rightarrow61$ rotational bands. The presence of CH$_3$C$_3$N on Titan was suggested by the Cassini Ion and Neutral Mass Spectrometer detection of its protonated form: C$_4$H$_3$NH$^+$, but the atmospheric abundance of the associated (deprotonated) neutral product is not well constrained due to the lack of appropriate laboratory reaction data. Here, we derive the column density of CH$_3$C$_3$N to be (3.8-5.7)$times10^{12}$ cm$^{-2}$ based on radiative transfer models sensitive to altitudes above 400 km Titans middle atmosphere. When compared with laboratory and photochemical model results, the detection of methylcyanoacetylene provides important constraints for the determination of the associated production pathways (such as those involving CN, CCN, and hydrocarbons), and reaction rate coefficients. These results also further demonstrate the importance of ALMA and (sub)millimeter spectroscopy for future investigations of Titans organic inventory and atmospheric chemistry, as CH$_3$C$_3$N marks the heaviest polar molecule detected spectroscopically in Titans atmosphere to date.
Vinyl cyanide (C$_2$H$_3$CN) is theorized to form in Titans atmosphere via high-altitude photochemistry and is of interest regarding the astrobiology of cold planetary surfaces due to its predicted ability to form cell membrane-like structures (azotosomes) in liquid methane. In this work, we follow up on the initial spectroscopic detection of C$_2$H$_3$CN on Titan by Palmer et al. (2017) with the detection of three new C$_2$H$_3$CN rotational emission lines at submillimeter frequencies. These new, high-resolution detections have allowed for the first spatial distribution mapping of C$_2$H$_3$CN on Titan. We present simultaneous observations of C$_2$H$_5$CN, HC$_3$N, and CH$_3$CN emission, and obtain the first (tentative) detection of C$_3$H$_8$ (propane) at radio wavelengths. We present disk-averaged vertical abundance profiles, two-dimensional spatial maps, and latitudinal flux profiles for the observed nitriles. Similarly to HC$_3$N and C$_2$H$_5$CN, which are theorized to be short-lived in Titans atmosphere, C$_2$H$_3$CN is most abundant over the southern (winter) pole, whereas the longer-lived CH$_3$CN is more concentrated in the north. This abundance pattern is consistent with the combined effects of high-altitude photochemical production, poleward advection, and the subsequent reversal of Titans atmospheric circulation system following the recent transition from northern to southern winter. We confirm that C$_2$H$_3$CN and C$_2$H$_5$CN are most abundant at altitudes above 200 km. Using a 300 km step model, the average abundance of C$_2$H$_3$CN is found to be $3.03pm0.29$ ppb, with a C$_2$H$_5$CN/C$_2$H$_3$CN abundance ratio of $2.43pm0.26$. Our HC$_3$N and CH$_3$CN spectra can be accurately modeled using abundance gradients above the tropopause, with fractional scale-heights of $2.05pm0.16$ and $1.63pm0.02$, respectively.
Simulations of Titans atmospheric transmission and surface reflectivity have been developed in order to estimate how Titans atmosphere and surface properties could affect performances of the Cassini radar experiment. In this paper we present a selection of models for Titans haze, vertical rain distribution, and surface composition implemented in our simulations. We collected dielectric constant values for the Cassini radar wavelength ($sim 2.2$ cm) for materials of interest for Titan: liquid methane, liquid mixture of methane-ethane, water ice and light hydrocarbon ices. Due to the lack of permittivity values for Titans haze particles in the microwave range, we performed dielectric constant ($varepsilon_r$) measurements around 2.2 cm on tholins synthesized in laboratory. We obtained a real part of $varepsilon_r$ in the range of 2-2.5 and a loss tangent between $10^{-3}$ and $5.10^{-2}$. By combining aerosol distribution models (with hypothetical condensation at low altitudes) to surface models, we find the following results: (1) Aerosol-only atmospheres should cause no loss and are essentially transparent for Cassini radar, as expected by former analysis. (2) However, if clouds are present, some atmospheric models generate significant attenuation that can reach $-50 dB$, well below the sensitivity threshold of the receiver. In such cases, a $13.78 GHz$ radar would not be able to measure echoes coming from the surface. We thus warn about possible risks of misinterpretation if a textquotedblleft wet atmospheretextquotedblright $ $is not taken into account. (3) Rough surface scattering leads to a typical response of $sim -17 dB$. These results will have important implications on future Cassini radar data analysis.
We have searched for the presence of simple P and S-bearing molecules in Titans atmosphere, by looking for the characteristic signatures of phosphine and hydrogen sulfide in infrared spectra obtained by Cassini CIRS. As a result we have placed the first upper limits on the stratospheric abundances, which are 1 ppb (PH3) and 330 ppb (H2S), at the 2-sigma significance level.
Simulation results are presented from a new general circulation model (GCM) of Titan, the Titan Atmospheric Model (TAM), which couples the Flexible Modeling System (FMS) spectral dynamical core to a suite of external/sub-grid-scale physics. These include a new non-gray radiative transfer module that takes advantage of recent data from Cassini-Huygens, large-scale condensation and quasi-equilibrium moist convection schemes, a surface model with bucket hydrology, and boundary layer turbulent diffusion. The model produces a realistic temperature structure from the surface to the lower mesosphere, including a stratopause, as well as satisfactory superrotation. The latter is shown to depend on the dynamical cores ability to build up angular momentum from surface torques. Simulated latitudinal temperature contrasts are adequate, compared to observations, and polar temperature anomalies agree with observations. In the lower atmosphere, the insolation distribution is shown to strongly impact turbulent fluxes, and surface heating is maximum at mid-latitudes. Surface liquids are unstable at mid- and low-latitudes, and quickly migrate poleward. The simulated humidity profile and distribution of surface temperatures, compared to observations, corroborate the prevalence of dry conditions at low latitudes. Polar cloud activity is well represented, though the observed mid-latitude clouds remain somewhat puzzling, and some formation alternatives are suggested.
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