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Register a new userExperimental evidence of chiral symmetry breaking in Kekule-ordered graphene
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The low-energy excitations of graphene are relativistic massless Dirac fermions with opposite chiralities at valleys K and K. Breaking the chiral symmetry could lead to gap opening in analogy to dynamical mass generation in particle physics. Here we report direct experimental evidences of chiral symmetry breaking (CSB) from both microscopic and spectroscopic measurements in a Li-intercalated graphene. The CSB is evidenced by gap opening at the Dirac point, Kekule-O type modulation, and chirality mixing near the gap edge. Our work opens up opportunities for investigating CSB related physics in a Kekule-ordered graphene.
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While graphene shows a characteristic conical dispersion with a vanishing density of states (DOS) near the Fermi energy E$_F$, it has been suggested that under extremely-high doping ($sim$ 1/4), the extended flat band can be shifted to near E$_F$, resulting in a diverging DOS with strong many-body interactions and electronic instabilities. Although such highly-doped graphene has attracted tremendous research interests, so far the experimental demonstration of doping-induced flat band as well as its associated intriguing phenomena remains rather limited. Here, we report the observation of an extended flat band around the M point in a Li-intercalated graphene, in which the Li ions not only dope graphene with a high electron concentration, but also induce a Kekule order which breaks the chiral symmetry. At such high electron doping, pronounced electron-phonon and electron-electron interactions are clearly identified by the notable kinks in the band dispersion and a strong reduction of the band width. Moreover, by following the evolution of the band structure upon Li intercalation, we find that the flat band and the Kekule order, with the characteristic flat band near M and folded Dirac cones near $Gamma$ respectively, emerge simultaneously, which indicates that they are strongly coupled. Our work identifies Li-intercalated graphene as a fertile platform for investigating the unique physics of the extended flat band, strong many-body interactions as well as the Kekule order.
Electron-phonon interaction and related self-energy are fundamental to both the equilibrium properties and non-equilibrium relaxation dynamics of solids. Although electron-phonon interaction has been suggested by various time-resolved measurements to be important for the relaxation dynamics of graphene, the lack of energy- and momentum-resolved self-energy dynamics prohibits direct identification of the role of specific phonon modes in the relaxation dynamics. Here by performing time- and angle-resolved photoemission spectroscopy measurements on a Kekule-ordered graphene with folded Dirac cones at the $Gamma$ point, we have succeeded in resolving the self-energy effect induced by coupling of electrons to two phonons at $Omega_1$ = 177 meV and $Omega_2$ = 54 meV and revealing its dynamical change in the time domain. Moreover, these strongly coupled phonons define energy thresholds, which separate the hierarchical relaxation dynamics from ultrafast, fast to slow, thereby providing direct experimental evidence for the dominant role of mode-specific phonons in the relaxation dynamics
Based on the spontaneous breaking of chiral symmetry, chiral perturbation theory (ChPT) is believed to approximate confinement scale QCD. Dedicated and increasingly accurate experiments and improving lattice calculations are confirming this belief, and we are entering a new era in which we can test confinement scale QCD in some well chosen reactions. This is demonstrated with an overview of low energy experimental tests of ChPT predictions of $pipi$ scattering, pion properties, $pi$N scattering and electromagnetic pion production. These predictions have been shown to be consistent with QCD in the meson sector by increasingly accurate lattice calculations. At present there is good agreement between experiment and ChPT calculations, including the $pipi$ and $pi$N s wave scattering lengths and the $pi^{0}$ lifetime. Recent, accurate pionic atom data are in agreement with chiral calculations once isospin breaking effects due to the mass difference of the up and down quarks are taken into account, as was required to extract the $pipi$ scattering lengths. In addition to tests of the theory, comparisons between $pipi$ and $pi$N interactions based on general chiral principles are discussed. Lattice calculations are now providing results for the fundamental, long and inconclusively studied, $pi$N $sigma$ term and the contribution of the strange quark to the mass of the proton. Increasingly accurate experiments in electromagnetic pion production experiments from the proton which test ChPT calculations (and their energy region of validity) are presented. These experiments are also beginning to measure the final state $pi$N interaction. This paper is based on the concluding remarks made at the Chiral Dynamics Workshop CD12 held at Jefferson Lab in Aug. 2012.
A Kekule bond texture in graphene modifies the electronic band structure by folding the Brillouin zone and bringing the two inequivalent Dirac points to the center. This can result, in the opening of a gap (Kek-O) or the locking of the valley degree of freedom with the direction of motion (Kek-Y). We analyze the effects of uniaxial strain on the band structure of Kekule-distorted graphene for both textures. Using a tight-binding approach, we introduce strain by considering the hopping renormalization and corresponding geometrical modifications of the Brillouin zone. We numerically evaluate the dispersion relation and present analytical expressions for the low-energy limit. Our results indicate the emergence of a Zeeman-like term due to the coupling of the pseudospin with the pseudomagnetic strain potential which separates the valleys by moving them in opposite directions away from the center of the Brillouin zone. For the Kek-O phase, this results in a competition between the Kekule parameter that opens a gap and the magnitude of strain which closes it. While for the Kek-Y phase, in a superposition of two shifted Dirac cones. As the Dirac cones are much closer in the supperlattice reciprocal space that in pristine graphene, we propose strain as a control parameter for intervalley scattering.
The quantum Hall effect near the charge neutrality point in bilayer graphene is investigated in high magnetic fields of up to 35 T using electronic transport measurements. In the high field regime, the eight-fold degeneracy in the zero energy Landau level is completely lifted, exhibiting new quantum Hall states corresponding filling factors $ u=$0, 1, 2, & 3. Measurements of the activation energy gap in tilted magnetic fields suggest that the Landau level splitting at the newly formed $ u=$1, 2, & 3 filling factors are independent of spin, consistent with the formation of a quantum Hall ferromagnet. In addition, measurements taken at the $ u$ = 0 charge neutral point show that, similar to single layer graphene, the bilayer becomes insulating at high fields.
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