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Register a new userThermodynamic evidence for the formation of a Fulde-Ferrell-Larkin-Ovchinnikov phase in the organic superconductor $lambda$-(BETS)$_2$GaCl$_4$
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In this work, the thermodynamic properties of the organic superconductor $lambda$-(BETS)$_2$GaCl$_4$ are investigated to study a high-field superconducting state known as the putative Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase. We observed a small thermodynamic anomaly in the field $H_{rm FFLO}$ $sim$ 10~T, which corresponds to the Pauli limiting field $H_{rm P}$. This anomaly probably originates from a transition from a uniform superconducting state to the FFLO state. $H_{rm FFLO}$ does not show a strong field-angular dependence due to a quasi-isotropic paramagnetic effect in $lambda$-(BETS)$_2$GaCl$_4$. The thermodynamic anomaly at $H_{rm FFLO}$ is smeared out and low-temperature upper critical field $H_{rm c2}$ changes significantly if fields are not parallel to the conducting plane even for a deviation of $sim$0.5$^{circ}$. This behavior indicates that the high-field state is very unstable, as it is influenced by the strongly anisotropic orbital effect. Our results are consistent with the theoretical predictions on the FFLO state, and show that the high-field superconductivity is probably an FFLO state in $lambda$-(BETS)$_2$GaCl$_4$ from a thermodynamic point of view.
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The specific heat of the layered organic superconductor $kappa$-% (BEDT-TTF)$_2$Cu(NCS)$_2$, where BEDT-TTF is bisethylenedithio-% tetrathiafulvalene, has been studied in magnetic fields up to 28 T applied perpendicular and parallel to the superconducting layers. In parallel fields above 21 T, the superconducting transition becomes first order, which signals that the Pauli-limiting field is reached. Instead of saturating at this field value, the upper critical field increases sharply and a second first-order transition line appears within the superconducting phase. Our results give strong evidence that the phase, which separates the homogeneous superconducting state from the normal state is a realization of a Fulde-Ferrell-Larkin-Ovchinnikov state.
We demonstrate that the vortex state in the Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase may be very different depending on the field orientation relative to the crystalline axes. We calculate numerically the upper critical field near the tricritical point taking into account the modulation of the order parameter along the magnetic field as well as the higher Landau levels. For s-wave superconductors with the anisotropy described by an elliptical Fermi surface we propose a general scheme of the analysis of the angular dependence of upper critical field at all temperatures on the basis of the exact solution for the order parameter. Our results show that the transitions (with tilting magnetic field) between different types of mixed states may be a salient feature of the FFLO phase. Moreover we discuss the reasons for the first-order phase transition into the FFLO state in the case of CeCoIn5 compound.
The Higgs mode associated with amplitude fluctuations of the superconducting gap in uniform superconductors usually is heavy, which makes its excitation and detection difficult. We report on the existence of a gapless Higgs mode in the Fulde-Ferrell-Larkin-Ovchinnikov states. This feature is originated from the Goldstone mode associated with the translation symmetry breaking. The existence of the gapless Higgs mode is demonstrated by using both a phenomenological model and microscopic Bardeen-Cooper-Schrieffer (BCS) theory. The gapless Higgs mode can avoid the decay into other low energy excitations, which renders it stable and detectable.
The Fulde-Ferrell-Larkin-Ovchinnikov (FFLO) phase is an unconventional superconducting state found under the influence of strong Zeeman field. This phase is identified by finite center-of-mass momenta in the Cooper pairs, causing the pairing amplitude to oscillate in real space. Repulsive correlations, on the other hand, smear out spatial inhomogeneities in d-wave superconductors. We investigate the FFLO state in a strongly correlated d-wave superconductor within a consolidated framework of Hartree-Fock-Bogoliubov theory and Gutzwiller approximation. We find that the profound effects of strong correlations lie in shifting the BCS-FFLO phase boundary towards a lower Zeeman field and thereby enlarging the window of the FFLO phase. In the FFLO state, our calculation features a sharp mid-gap peak in the density of states, indicating the formation of strongly localized Andreev bound states. We also find that the signatures of the FFLO phase survive even in the presence of an additional translational symmetry breaking competing order in the ground state. This is demonstrated by considering a broken symmetry ground state with a simultaneous presence of the d-wave superconducting order and a spin-density wave order, often found in unconventional superconductors.
We consider a two-component Fermi gas in the presence of spin imbalance, modeling the system in terms of a one-dimensional attractive Hubbard Hamiltonian initially in the presence of a confining trap potential. With the aid of the time-evolving block decimation method, we investigate the dynamics of the initial state when the trap is switched off. We show that the dynamics of a gas initially in the Fulde-Ferrel-Larkin-Ovchinnikov (FFLO) state is decomposed into the independent expansion of two fluids, namely the paired and the unpaired particles. In particular, the expansion velocity of the unpaired cloud is shown to be directly related to the FFLO momentum. This provides an unambiguous signature of the FFLO state in a remarkably simple way.
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