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Register a new userSecond-harmonic generation and the conservation of spatiotemporal orbital angular momentum of light
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Light with spatiotemporal orbital angular momentum (ST-OAM) is a recently discovered type of structured and localized electromagnetic field. This field carries characteristic space-time spiral phase structure and transverse intrinsic OAM. In this work, we present the generation and characterization of the second-harmonic of ST-OAM pulses. We uncovered the conservation of transverse OAM in a second-harmonic generation process, where the space-time topological charge of the fundamental field is doubled along with the optical frequency. Our experiment thus suggests a general ST-OAM nonlinear scaling rule - analogous to that in conventional OAM of light. Furthermore, we observe that the topology of a second-harmonic ST-OAM pulse can be modified by complex spatiotemporal astigmatism, giving rise to multiple phase singularities separated in space and time. Our study opens a new route for nonlinear conversion and scaling of light carrying ST-OAM with the potential for driving other secondary ST-OAM sources of electromagnetic fields and beyond.
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We experimentally study the behavior of orbital angular momentum (OAM) of light in a noncollinear second harmonic generation (SHG) process. The experiment is performed by using a type I BBO crystal under phase matching conditions with femtosecond pumping fields at 830 nm. Two specular off-axis vortex beams carrying fractional orbital angular momentum at the fundamental frequency (FF) are used. We analyze the behavior of the OAM of the SH signal when the optical vortex of each input field at the FF is displaced from the beams axis. We obtain different spatial configurations of the SH field, always carrying the same zero angular momentum.
Optical vortices are currently one of the most intensively studied topics in optics. These light beams, which carry orbital angular momentum (OAM), have been successfully utilized in the visible and infrared in a wide variety of applications. Moving to shorter wavelengths may open up completely new research directions in the areas of optical physics and material characterization. Here, we report on the generation of extreme-ultraviolet optical vortices with femtosecond duration carrying a controllable amount of OAM. From a basic physics viewpoint, our results help to resolve key questions such as the conservation of angular momentum in highly-nonlinear light-matter interactions, and the disentanglement and independent control of the intrinsic and extrinsic components of the photons angular momentum at short-wavelengths. The methods developed here will allow testing some of the recently proposed concepts such as OAM-induced dichroism, magnetic switching in organic molecules, and violation of dipolar selection rules in atoms.
Spin and orbital angular momentum of an optical beam are two independent parameters that exhibit distinct effects on mechanical objects. However, when laser beams with angular momentum interact with plasmas, one can observe the interplay between the spin and the orbital angular momentum. Here, by measuring the helical phase of the second harmonic 2{omega} radiation generated in an underdense plasma using a known spin and orbital angular momentum pump beam, we verify that the total angular momentum of photons is conserved and observe the conversion of spin to orbital angular momentum. We further determine the source of the 2{omega} photons by analyzing near field intensity distributions of the 2{omega} light. The 2{omega} images are consistent with these photons being generated near the largest intensity gradients of the pump beam in the plasma as predicted by the combined effect of spin and orbital angular momentum when Laguerre-Gaussian beams are used.
The interplay between spin and orbital angular momentum in the up-conversion process allows us to control the macroscopic wave front of high harmonics by manipulating the microscopic polarizations of the driving field. We demonstrate control of orbital angular momentum in high harmonic generation from both solid and gas phase targets using the selection rules of spin angular momentum. The gas phase harmonics extend the control of angular momentum to extreme-ultraviolet wavelength. We also propose a bi-color scheme to produce spectrally separated extreme-ultraviolet radiation carrying orbital angular momentum.
Manipulation of orbital angular momentum (OAM) of light is essential in OAM-based optical systems. Especially, OAM divider, which can convert the incoming OAM mode into one or several new smaller modes in proportion at different spatial paths, is very useful in OAM-based optical networks. However, this useful tool was never reported yet. For the first time, we put forward a passive OAM divider based on coordinate transformation. The device consists of a Cartesian to log-polar coordinate converter and an inverse converter. The first converter converts the OAM light into a rectangular-shaped plane light with a transverse phase gradient. And the second converter converts the plane light into multiple diffracted light. The OAM of zeroth-order diffracted light is the product of the input OAM and the scaling parameter. The residual light is output from other diffracted orders. Furthermore, we extend the scheme to realize equal N-dividing of OAM and arbitrary dividing of OAM. The ability of dividing OAM shows huge potential for OAM-based classical and quantum information processing.
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