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Vortex motion in tilted magnetic fields in highly layered electron-doped superconductor Nd2-xCexCuO4

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 Added by Mikhail Popov
 Publication date 2021
  fields Physics
and research's language is English




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The carrier transport and the motion of a vortex system in a mixed state of an electron-doped high-temperature superconductors Nd2-xCexCuO4 were investigated. To study the anisotropy of galvanomagnetic effects of highly layered NdCeCuO system we have synthesized Nd2-xCexCuO4/SrTiO3 epitaxial films with non-standart orientations of the c-axis and conductive CuO2 layers relative to the substrate. The variation ofe the angle of inclination of the magnetic field B, relative to the current J, reveals that the behavior of both the in-plane r_xx(B) and the out-plane r_xy(B) resistivities in the mixed state is mainly determined by the perpendicular to J component of B, that indicates the crucial role of the Lorentz force F_L~[JxB] and defines the motion of Josephson vortices across the CuO2 layers.



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The carrier transport and the motion of a vortex system in the electron-doped high-temperature superconductors Nd2-xCexCuO4 in underdoped and optimally doped (x = 0135, 0.145, 0.15) regions, in the area of the evolution from antiferromagnetic to superconducting order were investigated. To study the anisotropy of the transport properties of highly layered NdCeCuO system we have synthesized Nd2-xCexCuO4/SrTiO3 epitaxial films of three types with different orientations of the c-axis and conductive CuO2 layers relative to the substrate. Such a set of samples allowed us to study the processes of both standard (in the CuO2 layers) and lateral (across the CuO2 layers) carrier transfer in the normal and the mixed states of a superconductor. In a flux-flow regime, in magnetic field B, the dynamics of Abrikosov (B||c-axis) and Josephson (B||ab-plane) vortices are thoroughly investigated and analyzed which is perspective for scientific purposes and for practical applications in measurement technology.
In cuprate high-temperature superconductors, an antiferromagnetic Mott insulating state can be destabilized toward unconventional superconductivity by either hole- or electron-doping. In addition to these two electronic phases there is now a copious amount of evidence that supports the presence of a charge ordering (CO) instability competing with superconductivity inside the pseudogap state of the hole-doped (p-type) cuprates, but so far there has been no evidence of a similar CO in their electron-doped (n-type) counterparts. Here we report resonant x-ray scattering (RXS) measurements which demonstrate the presence of charge ordering in the n-type cuprate Nd2-xCexCuO4 near optimal doping. Remarkably we find that the CO in Nd2-xCexCuO4 occurs with similar periodicity, and along the same direction, as the CO in p-type cuprates. However, in contrast to the latter, the CO onset in Nd2-xCexCuO4 is higher than the pseudogap temperature, and is actually in the same temperature range where antiferromagnetic fluctuations are first detected -- thereby showing that CO and antiferromagnetic fluctuations are likely coupled in n-type cuprates. Overall our discovery uncovers a missing piece of the cuprate phase diagram and opens a parallel path to the study of CO and its relationship to other phenomena, such as antiferromagnetism (AF) and high-temperature superconductivity.
The aim of this work is to investigate the temperature dependencies both in CuO2-plane and out-of plane resistivities in electron-doped Nd2-xCexCuO4 for x from 0.135 up to 0.15 in order to analyze the anisotropy of the electrical transport in the process of the evolution from antiferromagnetic (AF) order in underdoped region to superconducting (SC) order in optimally doped region.
Extensive X-ray and neutron scattering experiments and additional transmission electron microscopy results reveal the partial decomposition of Nd2-xCexCuO4 (NCCO) in a low-oxygen-fugacity environment such as that typically realized during the annealing process required to create a superconducting state. Unlike a typical situation in which a disordered secondary phase results in diffuse powder scattering, a serendipitous match between the in-plane lattice constant of NCCO and the lattice constant of one of the decomposition products, (Nd,Ce)2O3, causes the secondary phase to form an oriented, quasi-two-dimensional epitaxial structure. Consequently, diffraction peaks from the secondary phase appear at rational positions (H,K,0) in the reciprocal space of NCCO. Additionally, because of neodymium paramagnetism, the application of a magnetic field increases the low-temperature intensity observed at these positions via neutron scattering. Such effects may mimic the formation of a structural superlattice or the strengthening of antiferromagnetic order of NCCO, but the intrinsic mechanism may be identified through careful and systematic experimentation. For typical reduction conditions, the (Nd,Ce)2O3 volume fraction is ~1%, and the secondary-phase layers exhibit long-range order parallel to the NCCO CuO2 sheets and are 50-100 angstromsthick. The presence of the secondary phase should also be taken into account in the analysis of other experiments on NCCO, such as transport measurements.
Measurements of the high-frequency complex resistivity in superconductors are a tool often used to obtain the vortex parameters, such as the vortex viscosity, the pinning constant and the depinning frequency. In anisotropic superconductors, the extraction of these quantities from the measurements faces new difficulties due to the tensor nature of the electromagnetic problem. The problem is specifically intricate when the magnetic field is tilted with respect to the crystallographic axes. Partial solutions exist in the free-flux-flow (no pinning) and Campbell (pinning dominated) regimes. In this paper we develop a full tensor model for the vortex motion complex resistivity, including flux-flow, pinning, and creep. We give explicit expressions for the tensors involved. We obtain that, despite the complexity of the physics, some parameters remain scalar in nature. We show that under specific circumstances the directly measured quantities do not reflect the true vortex parameters, and we give procedures to derive the true vortex parameters from measurements taken with arbitrary field orientations. Finally, we discuss the applicability of the angular scaling properties to the measured and transformed vortex parameters and we exploit these properties as a tool to unveil the existence of directional pinning.
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