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Stopping power of fission fragments in thin Mylar and nickel foils

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 Added by Thomas Materna
 Publication date 2021
  fields Physics
and research's language is English




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The energy loss of heavy ions in thin Mylar and nickel foils was measured accurately using fission fragments from $^{239}Pu(n_{th},f)$, mass and energy separated by the Lohengrin separator at ILL. The detection setup, placed at the focal plane of the Lohengrin separator enabled to measure precisely the kinetic energy difference of selected fragments after passing through the sample. From these data, the stopping powers in Mylar and nickel layers were extracted and compared to calculations. Whereas large deviations are observed with SRIM-2013 for Mylar, fairly good agreements are obtained with the semi-empirical approach of Knyazheva et al. and the calculations contained within the DPASS database. In nickel, SRIM-2013 and Knyazheva model are in agreement with our data within about 10 %, while large deviations are observed with DPASS. We used our data to provide updated parameters for the Knyazheva et al. model and rescale DPASS database for nickel and Mylar.



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We study how the excitation energy of the fully accelerated fission fragments is built up. It is stressed that only the intrinsic excitation energy available before scission can be exchanged between the fission fragments to achieve thermal equilibrium. This is in contradiction with most models used to calculate prompt neutron emission where it is assumed that the total excitation energy of the final fragments is shared between the fragments by the condition of equal temperatures. We also study the intrinsic excitation-energy partition according to a level density description with a transition from a constant-temperature regime to a Fermi-gas regime. Complete or partial excitation-energy sorting is found at energies well above the transition energy.
208 - X.B. Ma , F.Lu , L.Z. Wang 2014
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A correlation between the production and kinematic properties of the fragments issued of fission and multifragmentation is established in the study of the reaction 136Xe+hydrogen at 1 GeV per nucleon, measured in inverse kinematics at the FRagment Separator (GSI, Darmstadt). Such observables are analysed in a comprehensive study, selected as a function of the decay mode, and related to the isotopic properties of the fragments in the intermediate-mass region. Valuable information can be deduced on the characteristics of the heaviest product in the reaction, which has been considered a fundamental observable for tagging the thermodynamic properties of finite nuclear systems.
We report a measurement of the spin-flip probabilities for ultracold neutrons interacting with surfaces coated with nickel phosphorus. For 50~$mu$m thick nickel phosphorus coated on stainless steel, the spin-flip probability per bounce was found to be $beta_{rm NiP;on;SS} = (3.3^{+1.8}_{-5.6}) times 10^{-6}$. For 50~$mu$m thick nickel phosphorus coated on aluminum, the spin-flip probability per bounce was found to be $beta_{rm NiP;on;Al} = (3.6^{+2.1}_{-5.9}) times 10^{-6}$. For the copper guide used as reference, the spin flip probability per bounce was found to be $beta_{rm Cu} = (6.7^{+5.0}_{-2.5}) times 10^{-6}$. The results on the nickel phosphorus-coated surfaces may be interpreted as upper limits, yielding $beta_{rm NiP;on;SS} < 6.2 times 10^{-6}$ (90% C.L.) and $beta_{rm NiP;on;Al} < 7.0 times 10^{-6}$ (90% C.L.) for 50~$mu$m thick nickel phosphorus coated on stainless steel and 50~$mu$m thick nickel phosphorus coated on aluminum, respectively. Nickel phosphorus coated stainless steel or aluminum provides a solution when low-cost, mechanically robust, and non-depolarizing UCN guides with a high-Fermi-potential are needed.
The simultaneous measurement of the isotopic fission-fragment yields and fission-fragment velocities of $^{239}$U has been performed for the first time. The $^{239}$U fissioning system was produced in one-neutron transfer reactions between a $^{238}$U beam at 5.88 MeV/nucleon and a $^{9}$Be target. The combination of inverse kinematics at low energy and the use of the VAMOS++ spectrometer at the GANIL facility allows the isotopic identification of the full fission-fragment distribution and their velocity in the reference frame of the fissioning system. The proton and neutron content of the fragments at scission, their total kinetic and total excitation energy, as well as the neutron multiplicity were determined. Information from the scission point configuration is obtained from these observables and the correlation between them. The role of the octupole-deformed proton and neutron shells in the fission-fragment production is discussed.
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