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Register a new userFinal excitation energy of fission fragments
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We study how the excitation energy of the fully accelerated fission fragments is built up. It is stressed that only the intrinsic excitation energy available before scission can be exchanged between the fission fragments to achieve thermal equilibrium. This is in contradiction with most models used to calculate prompt neutron emission where it is assumed that the total excitation energy of the final fragments is shared between the fragments by the condition of equal temperatures. We also study the intrinsic excitation-energy partition according to a level density description with a transition from a constant-temperature regime to a Fermi-gas regime. Complete or partial excitation-energy sorting is found at energies well above the transition energy.
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Two methods of the total excitation energy (TXE) partition between complementary fission fragments (FF) are compared: one based on the classical hypothesis of prompt neutron emission from fully accelerated FF with both fragments having the same residual nuclear temperature distribution,the second one on the systematic behavior of the experimental multiplicity ratio { u}H/({ u}L+{ u}H) as a function of the heavy fragment mass number AH,the complementary FF having different residual temperature distributions.These methods were applied on six fissioning systems: 233,235U(nth,f), 239Pu(nth,f), 237Np(n5.5MeV,f), 252Cf(SF), 248Cm(SF) and fragment excitation energies,level density parameters,fragment and fragment pair temperatures were compared.Limitations of the classical TXE partition method are shown.Residual temperature ratios RT=TL/TH versus AH,local and global parameterizations of RT(AH) for the neutron induced fissioning systems are obtained.Average values of quantities characterizing prompt neutron emission are discussed.A linear decrease of <RT> with the mass number of the fissioning nucleus and a linear decrease of the average C parameter with the fissility parameter is obtained.Point by Point (PbP) model calculations validate the RT(AH) parameterizations.The multi-parametric matrix { u}(A,TKE) as well as prompt neutron and gamma-ray emission quantities as a function of fragment mass,total average prompt neutron multiplicity and spectrum and prompt neutron multiplicity distribution P({ u}) were calculated.The global RT(AH) parameterization extends the use of the PbP model to predict prompt neutron emission quantities for fissioning systems without experimental data.An explanation of the less pronounced sawtooth shape of { u}(A) and the increase of { u}(A) with incident neutron energy only for heavy fragments is given and exemplified by quantitative results of the PbP model.
The isospin properties of primary and secondary fragments produced in multifragmentation of Fe + Ni and Fe + Fe systems with respect to Ni + Ni system are analyzed within the statistical multifragmentation model framework. The reduced neutron and proton densities show an asymmetry in the primary fragments, that is lessened after secondary decay. with increasing isospin (N/Z) this effect increases, while the sensitivity of fragment isospin towards excitation energy and N/Z of the primary fragments remains unchanged.
A simplified, though realistic, model describing two receding and accelerating fission fragments, due to their mutual Coulomb repulsion, shows that fission fragments share excitation energy well after they ceased to exchange nucleons. This mechanism leads to a lower total kinetic energy of the fission fragments, particularly if the pygmy resonances in the fission fragments are excited. Even though the emphasis here is on fission, similar arguments apply to fragments in heavy-ion reactions.
The energy loss of heavy ions in thin Mylar and nickel foils was measured accurately using fission fragments from $^{239}Pu(n_{th},f)$, mass and energy separated by the Lohengrin separator at ILL. The detection setup, placed at the focal plane of the Lohengrin separator enabled to measure precisely the kinetic energy difference of selected fragments after passing through the sample. From these data, the stopping powers in Mylar and nickel layers were extracted and compared to calculations. Whereas large deviations are observed with SRIM-2013 for Mylar, fairly good agreements are obtained with the semi-empirical approach of Knyazheva et al. and the calculations contained within the DPASS database. In nickel, SRIM-2013 and Knyazheva model are in agreement with our data within about 10 %, while large deviations are observed with DPASS. We used our data to provide updated parameters for the Knyazheva et al. model and rescale DPASS database for nickel and Mylar.
A correlation between the production and kinematic properties of the fragments issued of fission and multifragmentation is established in the study of the reaction 136Xe+hydrogen at 1 GeV per nucleon, measured in inverse kinematics at the FRagment Separator (GSI, Darmstadt). Such observables are analysed in a comprehensive study, selected as a function of the decay mode, and related to the isotopic properties of the fragments in the intermediate-mass region. Valuable information can be deduced on the characteristics of the heaviest product in the reaction, which has been considered a fundamental observable for tagging the thermodynamic properties of finite nuclear systems.
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