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Dragging of light by moving dielectrics was predicted by Fresnel and verified by Fizeaus celebrated experiments with flowing water. This momentous discovery is among the experimental cornerstones of Einsteins special relativity and is well understood in the context of relativistic kinematics. In contrast, experiments on dragging photons by an electron flow in solids are riddled with inconsistencies and so far eluded agreement with the theory. Here we report on the electron flow dragging surface plasmon polaritons (SPPs): hybrid quasiparticles of infrared photons and electrons in graphene. The drag is visualized directly through infrared nano-imaging of propagating plasmonic waves in the presence of a high-density current. The polaritons in graphene shorten their wavelength when launched against the drifting carriers. Unlike the Fizeau effect for light, the SPP drag by electrical currents defies the simple kinematics interpretation and is linked to the nonlinear electrodynamics of the Dirac electrons in graphene. The observed plasmonic Fizeau drag enables breaking of time-reversal symmetry and reciprocity at infrared frequencies without resorting to magnetic fields or chiral optical pumping.
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Fizeau demonstrated in 1850 that the speed of light can be modified when it is propagating in moving media. Can we achieve such control of the light speed efficiently with a fast-moving electron media by passing electrical current? Because the strong electromagnetic coupling between the electron and light leads to the collective excitation of plasmon polaritons, it will manifest as the plasmonic Doppler effect. Experimental observation of the plasmonic Doppler effect in electronic system has been challenge because the plasmon propagation speed is much faster than the electron drift velocity in conventional noble metals. Here, we report direct observation of Fizeau drag of plasmon polaritons in strongly biased graphene by exploiting the high electron mobility and the slow plasmon propagation of massless Dirac electrons. The large bias current in graphene creates a fast drifting Dirac electron medium hosting the plasmon polariton. It results in nonreciprocal plasmon propagation, where plasmons moving with the drifting electron media propagate at an enhanced speed. We measure the Doppler-shifted plasmon wavelength using a cryogenic near-field infrared nanoscopy, which directly images the plasmon polariton mode in the biased graphene at low temperature. We observe a plasmon wavelength difference up to 3.6% between plasmon moving along and against the drifting electron media. Our findings on the plasmonic Doppler effect open new opportunities for electrical control of non-reciprocal surface plasmon polaritons in nonequilibrium systems.
The optical response of graphene micro-structures, such as micro-ribbons and disks, is dominated by the localized plasmon resonance in the far infrared (IR) spectral range. An ensemble of such structures is usually involved and the effect of the coupling between the individual structures is expected to play an important role. In this paper, the plasmonic coupling of graphene microstructures in different configurations is investigated. While a relatively weak coupling between graphene disks on the same plane is observed, the coupling between vertically stacked graphene disks is strong and a drastic increase of the resonance frequency is demonstrated. The plasmons in a more complex structure can be treated as the hybridization of plasmons from more elementary structures. As an example, the plasmon resonances of graphene micro-rings are presented, in conjunction with their response in a magnetic field. Finally, the coupling of the plasmon and the surface polar phonons of SiO2 substrate is demonstrated by the observation of a new hybrid resonance peak around 500cm-1.
Plasmon in graphene possesses many unique properties. It originates from the collective motion of massless Dirac fermions and the carrier density dependence is distinctively different from conventional plasmons. In addition, graphene plasmon is highly tunable and shows strong energy confinement capability. Most intriguing, as an atom-thin layer, graphene and its plasmon are very sensitive to the immediate environment. Graphene plasmons strongly couple to polar phonons of the substrate, molecular vibrations of the adsorbates, and lattice vibrations of other atomically thin layers. In this review paper, well present the most important advances in grapene plasmonics field. The topics include terahertz plasmons, mid-infrared plasmons, plasmon-phonon interactions and potential applications. Graphene plasmonics opens an avenue for reconfigurable metamaterials and metasurfaces. Its an exciting and promising new subject in the nanophotonics and plasmonics research field.
Plasmonics has established itself as a branch of physics which promises to revolutionize data processing, improve photovoltaics, increase sensitivity of bio-detection. A widespread use of plasmonic devices is notably hindered (in addition to high losses) by the absence of stable and inexpensive metal films suitable for plasmonic applications. This may seem surprising given the number of metal compounds to choose from. Unfortunately, most of them either exhibit a strong damping of surface plasmons or easily oxidize and corrode. To this end, there has been continuous search for alternative plasmonic materials that are, unlike gold, the current metal of choice in plasmonics, compatible with complementary metal oxide semiconductor technology. Here we show that copper and silver protected by graphene are viable candidates. Copper films covered with one to a few graphene layers show excellent plasmonics characteristics surpassing those of gold films. They can be used to fabricate plasmonic devices and survive for at least a year, even in wet and corroding conditions. As a proof of concept, we use the graphene-protected copper to demonstrate dielectric loaded plasmonic waveguides and test sensitivity of surface plasmon resonances. Our results are likely to initiate a wide use of graphene-protected plasmonics.
Using a novel structure, consisting of two, independently contacted graphene single layers separated by an ultra-thin dielectric, we experimentally measure the Coulomb drag of massless fermions in graphene. At temperatures higher than 50 K, the Coulomb drag follows a temperature and carrier density dependence consistent with the Fermi liquid regime. As the temperature is reduced, the Coulomb drag exhibits giant fluctuations with an increasing amplitude, thanks to the interplay between coherent transport in the graphene layer and interaction between the two layers.
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