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Register a new userRevealing three-dimensional quantum criticality by Sr-substitution in Han Purple
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Classical and quantum phase transitions (QPTs), with their accompanying concepts of criticality and universality, are a cornerstone of statistical thermodynamics. An exemplary controlled QPT is the field-induced magnetic ordering of a gapped quantum magnet. Although numerous quasi-one-dimensional coupled spin-chain and -ladder materials are known whose ordering transition is three-dimensional (3D), quasi-2D systems are special for several physical reasons. Motivated by the ancient pigment Han Purple (BaCuSi$_{2}$O$_{6}$), a quasi-2D material displaying anomalous critical properties, we present a complete analysis of Ba$_{0.9}$Sr$_{0.1}$CuSi$_{2}$O$_{6}$. We measure the zero-field magnetic excitations by neutron spectroscopy and deduce the magnetic Hamiltonian. We probe the field-induced transition by combining magnetization, specific-heat, torque and magnetocalorimetric measurements with low-temperature nuclear magnetic resonance studies near the QPT. By a Bayesian statistical analysis and large-scale Quantum Monte Carlo simulations, we demonstrate unambiguously that observable 3D quantum critical scaling is restored by the structural simplification arising from light Sr-substitution in Han Purple.
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We present a route to grow single crystals of Ba$_{0.9}$Sr$_{0.1}$CuSi$_{2}$O$_{6}$ suitable for inelastic neutron studies via the floating zone technique. Neutron single crystal diffraction was utilized to check their bulk quality and orientation. Finally, the high quality of the grown crystals was proven by X-ray diffraction and magnetic susceptibility.
This review summarizes recent developments in the study of fermionic quantum criticality, focusing on new progress in numerical methodologies, especially quantum Monte Carlo methods, and insights that emerged from recently large-scale numerical simulations. Quantum critical phenomena in fermionic systems have attracted decades of extensive research efforts, partially lured by their exotic properties and potential technology applications and partially awaked by the profound and universal fundamental principles that govern these quantum critical systems. Due to the complex and non-perturbative nature, these systems belong to the most difficult and challenging problems in the study of modern condensed matter physics, and many important fundamental problems remain open. Recently, new developments in model design and algorithm improvements enabled unbiased large-scale numerical solutions to be achieved in the close vicinity of these quantum critical points, which paves a new pathway towards achieving controlled conclusions through combined efforts of theoretical and numerical studies, as well as possible theoretical guidance for experiments in heavy-fermion compounds, Cu-based and Fe-based superconductors, ultra-cold fermionic atomic gas, twisted graphene layers, etc., where signatures of fermionic quantum criticality exist.
Quasi-two dimensional itinerant fermions in the Anti-Ferro-Magnetic (AFM) quantum-critical region of their phase diagram, such as in the Fe-based superconductors or in some of the heavy-fermion compounds, exhibit a resistivity varying linearly with temperature and a contribution to specific heat or thermopower proportional to $T ln T$. It is shown here that a generic model of itinerant AFM can be canonically transformed such that its critical fluctuations around the AFM-vector $Q$ can be obtained from the fluctuations in the long wave-length limit of a dissipative quantum XY model. The fluctuations of the dissipative quantum XY model in 2D have been evaluated recently and in a large regime of parameters, they are determined, not by renormalized spin-fluctuations but by topological excitations. In this regime, the fluctuations are separable in their spatial and temporal dependence and have a dynamical critical exponent $z =infty.$ The time dependence gives $omega/T$-scaling at criticality. The observed resistivity and entropy then follow directly. Several predictions to test the theory are also given.
Exotic physics often emerges around quantum criticality in metallic systems. Here we explore the nature of topological phase transitions between 3D double-Weyl semimetals and insulators (through annihilating double-Weyl nodes with opposite chiralities) in the presence of Coulomb interactions. From renormalization-group (RG) analysis, we find a non-Fermi-liquid quantum critical point (QCP) between the double-Weyl semimetals and insulators when artificially neglecting short-range interactions. However, it is shown that this non-Fermi-liquid QCP is actually unstable against nematic ordering when short-range interactions are correctly included in the RG analysis. In other words, the putative QCP between the semimetals and insulators is preempted by emergence of nematic phases when Coulomb interactions are present. We further discuss possible experimental relevance of the nematicity-preempted QCP to double-Weyl candidate materials HgCr2Se4 and SrSi2.
Earlier Monte-Carlo calculations on the dissipative two-dimensional XY model are extended in several directions. We study the phase diagram and the correlation functions when dissipation is very small, where it has properties of the classical 3D-XY transition, i.e. one with a dynamical critical exponent $z=1$. The transition changes from $z=1$ to the class of criticality with $z to infty$ driven by topological defects, discovered earlier, beyond a critical dissipation. We also find that the critical correlations have power-law singularities as a function of tuning the ratio of the kinetic energy to the potential energy for fixed large dissipation, as opposed to essential singularities on tuning dissipation keeping the former fixed. A phase with temporal disorder but spatial order of the Kosterlitz-Thouless form is also further investigated. We also present results for the transition when the allowed Caldeira-Leggett form of dissipation and the allowed form of dissipation coupling to the compact rotor variables are both included. The nature of the transition is then determined by the Caldeira-Leggett form.
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