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Register a new userObserving quantum coherence from photons scattered in free-space
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Quantum channels in free-space, an essential prerequisite for fundamental tests of quantum mechanics and quantum technologies in open space, have so far been based on direct line-of-sight because the predominant approaches for photon-encoding, including polarization and spatial modes, are not compatible with randomly scattered photons. Here we demonstrate a novel approach to transfer and recover quantum coherence from scattered, non-line-of-sight photons analyzed in a multimode and imaging interferometer for time-bins, combined with photon detection based on a 8x8 single-photon-detector-array. The observed time-bin visibility for scattered photons remained at a high $95%$ over a wide scattering angle range of -45 degree to +45 degree, while the individual pixels in the detector array resolve or track an image in its field of view of ca. 0.5 degrees. Using our method we demonstrate the viability of two novel applications. Firstly, using scattered photons as an indirect channel for quantum communication thereby enabling non-line-of-sight quantum communication with background suppression, and secondly, using the combined arrival time and quantum coherence to enhance the contrast of low-light imaging and laser ranging under high background light. We believe our method will instigate new lines for research and development on applying photon coherence from scattered signals to quantum sensing, imaging, and communication in free-space environments.
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It is usually considered that the spectrum of an optical cavity coupled to an atomic medium does not exhibit a normal-mode splitting unless the system satisfies the strong coupling condition, meaning the Rabi frequency of the coherent coupling exceeds the decay rates of atom and cavity excitations. Here we show that this need not be the case, but depends on the way in which the coupled system is probed. Measurements of the reflection of a probe laser from the input mirror of an overdamped cavity reveal an avoided crossing in the spectrum which is not observed when driving the atoms directly and measuring the Purcell-enhanced cavity emission. We understand these observations by noting a formal correspondence with electromagnetically-induced transparency of a three-level atom in free space, where our cavity acts as the absorbing medium and the coupled atoms play the role of the control field.
We have distributed entangled photons directly through the atmosphere to a receiver station 7.8 km away over the city of Vienna, Austria at night. Detection of one photon from our entangled pairs constitutes a triggered single photon source from the sender. With no direct time-stable connection, the two stations found coincidence counts in the detection events by calculating the cross-correlation of locally-recorded time stamps shared over a public internet channel. For this experiment, our quantum channel was maintained for a total of 40 minutes during which time a coincidence lock found approximately 60000 coincident detection events. The polarization correlations in those events yielded a Bell parameter, S=2.27/pm0.019, which violates the CHSH-Bell inequality by 14 standard deviations. This result is promising for entanglement-based free-space quantum communication in high-density urban areas. It is also encouraging for optical quantum communication between ground stations and satellites since the length of our free-space link exceeds the atmospheric equivalent.
The generation and manipulation of entanglement between isolated particles has precipitated rapid progress in quantum information processing. Entanglement is also known to play an essential role in the optical properties of atomic ensembles, but fundamental effects in the controlled emission and absorption from small, well-defined numbers of entangled emitters in free space have remained unobserved. Here we present the control of the spontaneous emission rate of a single photon from a pair of distant, entangled atoms into a free-space optical mode. Changing the length of the optical path connecting the atoms modulates the emission rate with a visibility $V = 0.27 pm 0.03$ determined by the degree of entanglement shared between the atoms, corresponding directly to the concurrence $mathcal{C_{rho}}= 0.31 pm 0.10$ of the prepared state. This scheme, together with population measurements, provides a fully optical determination of the amount of entanglement. Furthermore, large sensitivity of the interference phase evolution points to applications of the presented scheme in high-precision gradient sensing.
We propose an efficient free-space scheme to create single photons in a well-defined spatiotemporal mode. To that end, we first prepare a single source atom in an excited Rydberg state. The source atom interacts with a large ensemble of ground-state atoms via a laser-mediated dipole-dipole exchange interaction. Using an adiabatic passage with a chirped laser pulse, we produce a spatially extended spin wave of a single Rydberg excitation in the ensemble, accompanied by the transition of the source atom to another Rydberg state. The collective atomic excitation can then be converted to a propagating optical photon via a coherent coupling field. In contrast to previous approaches, our single-photon source does not rely on the strong coupling of a single emitter to a resonant cavity, nor does it require the heralding of collective excitation or complete Rydberg blockade of multiple excitations in the atomic ensemble.
A working free-space quantum key distribution (QKD) system has been developed and tested over a 205-m indoor optical path at Los Alamos National Laboratory under fluorescent lighting conditions. Results show that free-space QKD can provide secure real-time key distribution between parties who have a need to communicate secretly.
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