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Register a new userInterference of single photons emitted by entangled atoms in free space
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The generation and manipulation of entanglement between isolated particles has precipitated rapid progress in quantum information processing. Entanglement is also known to play an essential role in the optical properties of atomic ensembles, but fundamental effects in the controlled emission and absorption from small, well-defined numbers of entangled emitters in free space have remained unobserved. Here we present the control of the spontaneous emission rate of a single photon from a pair of distant, entangled atoms into a free-space optical mode. Changing the length of the optical path connecting the atoms modulates the emission rate with a visibility $V = 0.27 pm 0.03$ determined by the degree of entanglement shared between the atoms, corresponding directly to the concurrence $mathcal{C_{rho}}= 0.31 pm 0.10$ of the prepared state. This scheme, together with population measurements, provides a fully optical determination of the amount of entanglement. Furthermore, large sensitivity of the interference phase evolution points to applications of the presented scheme in high-precision gradient sensing.
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We propose an efficient free-space scheme to create single photons in a well-defined spatiotemporal mode. To that end, we first prepare a single source atom in an excited Rydberg state. The source atom interacts with a large ensemble of ground-state atoms via a laser-mediated dipole-dipole exchange interaction. Using an adiabatic passage with a chirped laser pulse, we produce a spatially extended spin wave of a single Rydberg excitation in the ensemble, accompanied by the transition of the source atom to another Rydberg state. The collective atomic excitation can then be converted to a propagating optical photon via a coherent coupling field. In contrast to previous approaches, our single-photon source does not rely on the strong coupling of a single emitter to a resonant cavity, nor does it require the heralding of collective excitation or complete Rydberg blockade of multiple excitations in the atomic ensemble.
We present a novel approach to engineer the photon correlations emerging from the interference between an input field and the field scattered by a single atom in free space. Nominally, the inefficient atom-light coupling causes the quantum correlations to be dominated by the input field alone. To overcome this issue, we propose the use of separate pump and probe beams, where the former increases the atomic emission to be comparable to the probe. Examining the second-order correlation function $g^{(2)}(tau)$ of the total field in the probe direction, we find that the addition of the pump formally plays the same role as increasing the coupling efficiency. We show that one can tune the correlation function $g^{(2)}(0)$ from zero (perfect anti-bunching) to infinite (extreme bunching) by a proper choice of pump amplitude. We further elucidate the origin of these correlations in terms of the transient atomic state following the detection of a photon.
Photon interference among distant quantum emitters is a promising method to generate large scale quantum networks. Interference is best achieved when photons show long coherence times. For the nitrogen-vacancy defect center in diamond we measure the coherence times of photons via optically induced Rabi oscillations. Experiments reveal a close to Fourier transform (i.e. lifetime) limited width of photons emitted even when averaged over minutes. The projected contrast of two-photon interference (0.8) is high enough to envisage the applications in quantum information processing. We report 12 and 7.8 ns excited state lifetime depending on the spin state of the defect.
We investigate the emission of single photons from CdSe/CdS dot-in-rods which are optically trapped in the focus of a deep parabolic mirror. Thanks to this mirror, we are able to image almost the full 4$pi$ emission pattern of nanometer-sized elementary dipoles and verify the alignment of the rods within the optical trap. From the motional dynamics of the emitters in the trap we infer that the single-photon emission occurs from clusters comprising several emitters. We demonstrate the optical trapping of rod-shaped quantum emitters in a configuration suitable for efficiently coupling an ensemble of linear dipoles with the electromagnetic field in free space.
A diamond nano-crystal hosting a single nitrogen vacancy (NV) center is optically selected with a confocal scanning microscope and positioned deterministically onto the subwavelength-diameter waist of a tapered optical fiber (TOF) with the help of an atomic force microscope. Based on this nano-manipulation technique we experimentally demonstrate the evanescent coupling of single fluorescence photons emitted by a single NV-center to the guided mode of the TOF. By comparing photon count rates of the fiber-guided and the free-space modes and with the help of numerical FDTD simulations we determine a lower and upper bound for the coupling efficiency of (9.5+/-0.6)% and (10.4+/-0.7)%, respectively. Our results are a promising starting point for future integration of single photon sources into photonic quantum networks and applications in quantum information science.
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