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Register a new userTension-free Dirac strings and steered magnetic charges in 3D artificial spin ice
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3D nano-architectures present a new paradigm in modern condensed matter physics with numerous applications in photonics, biomedicine, and spintronics. They are promising for the realisation of 3D magnetic nano-networks for ultra-fast and low-energy data storage. Frustration in these systems can lead to magnetic charges or magnetic monopoles, which can function as mobile, binary information carriers. However, Dirac strings in 2D artificial spin ices bind magnetic charges, while 3D dipolar counterparts require cryogenic temperatures for their stability. Here, we present a micromagnetic study of a highly-frustrated 3D artificial spin ice harboring tension-free Dirac strings with unbound magnetic charges at room temperature. We use micromagnetic simulations to demonstrate that the mobility threshold for magnetic charges is by $SI{2}{eV}$ lower than their unbinding energy. By applying global magnetic fields, we steer magnetic charges in a given direction omitting unintended switchings. The introduced system paves a way towards 3D magnetic networks for data transport and storage
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Systems of interacting nanomagnets known as artificial spin ices are models for exotic behavior due to their accessibility to geometries and measurement modalities that are not available in natural materials. Despite being fundamentally composed of binary moments, these systems often display collective phenomena associated with emergent higher-order frustration. We have studied the vertex-frustrated Santa Fe ice, examining its moment structure both after annealing near the ferromagnetic Curie point, and in a thermally dynamic state. We experimentally demonstrate the existence of a disordered string ground state, in which the magnetic structure can be understood through the topology of emergent strings of local excitations. We also show that the system can support a long-range-ordered ground state for certain ratios of local interactions. Both states are accessible via moment reversals only through topological surgery, i.e., the breaking of pairs of crossed strings and their reattachment in topologically inequivalent configurations. While we observe instances of topological surgery in our experimental data, such events are energetically suppressed, and we find that an apparent kinetic bottleneck associated with topological surgery precludes the system from achieving either ground state through local moment flips. Santa Fe ice thus represents an unusual instance of competition between topological complexity and ordering, suggesting analogous structures in the quantum realm.
Designing and constructing model systems that embody the statistical mechanics of frustration is now possible using nanotechnology. We have arranged nanomagnets on a two-dimensional square lattice to form an artificial spin ice, and studied its fractional excitations, emergent magnetic monopoles, and how they respond to a driving field using X-ray magnetic microscopy. We observe a regime in which the monopole drift velocity is linear in field above a critical field for the onset of motion. The temperature dependence of the critical field can be described by introducing an interaction term into the Bean-Livingston model of field-assisted barrier hopping. By analogy with electrical charge drift motion, we define and measure a monopole mobility that is larger both for higher temperatures and stronger interactions between nanomagnets. The mobility in this linear regime is described by a creep model of zero-dimensional charges moving within a network of quasi-one-dimensional objects.
While sources of magnetic fields - magnetic monopoles - have so far proven elusive as elementary particles, several scenarios have been proposed recently in condensed matter physics of emergent quasiparticles resembling monopoles. A particularly simple proposition pertains to spin ice on the highly frustrated pyrochlore lattice. The spin ice state is argued to be well-described by networks of aligned dipoles resembling solenoidal tubes - classical, and observabl
The study of magnetic correlations in dipolar-coupled nanomagnet systems with synchrotron x-ray scattering provides a means to uncover emergent phenomena and exotic phases, in particular in systems with thermally active magnetic moments. From the diffuse signal of soft x-ray resonant magnetic scattering, we have measured magnetic correlations in a highly dynamic artificial kagome spin ice with sub-70-nm Permalloy nanomagnets. On comparing experimental scattering patterns with Monte Carlo simulations based on a needle-dipole model, we conclude that kagome ice I phase correlations exist in our experimental system even in the presence of moment fluctuations, which is analogous to bulk spin ice and spin liquid behavior. In addition, we describe the emergence of quasi-pinch-points in the magnetic diffuse scattering in the kagome ice I phase. These quasi-pinch-points bear similarities to the fully developed pinch points with singularities of a magnetic Coulomb phase, and continually evolve into the latter on lowering the temperature. The possibility to measure magnetic diffuse scattering with soft x rays opens the way to study magnetic correlations in a variety of nanomagnetic systems.
The properties of natural and artificial assemblies of interacting elements, ranging from Quarks to Galaxies, are at the heart of Physics. The collective response and dynamics of such assemblies are dictated by the intrinsic dynamical properties of the building blocks, the nature of their interactions and topological constraints. Here we report on the relaxation dynamics of the magnetization of artificial assemblies of mesoscopic spins. In our model nano-magnetic system - square artificial spin ice - we are able to control the geometrical arrangement and interaction strength between the magnetically interacting building blocks by means of nano-lithography. Using time resolved magnetometry we show that the relaxation process can be described using the Kohlrausch law and that the extracted temperature dependent relaxation times of the assemblies follow the Vogel-Fulcher law. The results provide insight into the relaxation dynamics of mesoscopic nano-magnetic model systems, with adjustable energy and time scales, and demonstrates that these can serve as an ideal playground for the studies of collective dynamics and relaxations.
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