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Register a new userThermally induced magnetic relaxation in square artificial spin ice
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The properties of natural and artificial assemblies of interacting elements, ranging from Quarks to Galaxies, are at the heart of Physics. The collective response and dynamics of such assemblies are dictated by the intrinsic dynamical properties of the building blocks, the nature of their interactions and topological constraints. Here we report on the relaxation dynamics of the magnetization of artificial assemblies of mesoscopic spins. In our model nano-magnetic system - square artificial spin ice - we are able to control the geometrical arrangement and interaction strength between the magnetically interacting building blocks by means of nano-lithography. Using time resolved magnetometry we show that the relaxation process can be described using the Kohlrausch law and that the extracted temperature dependent relaxation times of the assemblies follow the Vogel-Fulcher law. The results provide insight into the relaxation dynamics of mesoscopic nano-magnetic model systems, with adjustable energy and time scales, and demonstrates that these can serve as an ideal playground for the studies of collective dynamics and relaxations.
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Designing and constructing model systems that embody the statistical mechanics of frustration is now possible using nanotechnology. We have arranged nanomagnets on a two-dimensional square lattice to form an artificial spin ice, and studied its fractional excitations, emergent magnetic monopoles, and how they respond to a driving field using X-ray magnetic microscopy. We observe a regime in which the monopole drift velocity is linear in field above a critical field for the onset of motion. The temperature dependence of the critical field can be described by introducing an interaction term into the Bean-Livingston model of field-assisted barrier hopping. By analogy with electrical charge drift motion, we define and measure a monopole mobility that is larger both for higher temperatures and stronger interactions between nanomagnets. The mobility in this linear regime is described by a creep model of zero-dimensional charges moving within a network of quasi-one-dimensional objects.
Artificial spin ices (ASIs) are interacting arrays of lithographically-defined nanomagnets in which novel frustrated magnetic phases can be intentionally designed. A key emergent description of fundamental excitations in ASIs is that of magnetic monopoles -- mobile quasiparticles that carry an effective magnetic charge. Here we demonstrate that the archetypal square ASI lattice can host, in specific regions of its magnetic phase diagram, high-density plasma-like regimes of mobile magnetic monopoles. By passively listening to spontaneous monopole noise in thermal equilibrium, we reveal their intrinsic dynamics and show that monopole kinetics are minimally correlated (that is, most diffusive) in the plasma phase. These results open the door to on-demand monopole regimes having field-tunable densities and dynamic properties, thereby providing a new paradigm for probing the physics of effective magnetic charges in synthetic matter.
Critical behavior is very common in many fields of science and a wide variety of many-body systems exhibit emergent critical phenomena. The beauty of critical phase transitions lies in their scale-free properties, such that the temperature dependence of physical parameters of systems differing at the microscopic scale can be described by the same generic power laws. In this work we establish the critical properties of the antiferromagnetic phase transition in artificial square ice, showing that it belongs to the two-dimensional Ising universality class, which extends the applicability of such concepts from atomistic to mesoscopic magnets. Combining soft x-ray resonant magnetic scattering experiments and Monte Carlo simulations, we characterize the transition to the low temperature long range order expected for the artificial square ice system. By measuring the critical scattering, we provide direct quantitative evidence of a continuous magnetic phase transition, obtaining critical exponents which are compatible with those of the two-dimensional Ising universality class. In addition, by varying the blocking temperature relative to the phase transition temperature, we demonstrate its influence on the out-of-equilibrium dynamics due to critical slowing down at the phase transition.
Magnetization dynamics in an artificial square spin-ice lattice made of Ni80Fe20 with magnetic field applied in the lattice plane is investigated by broadband ferromagnetic resonance spectroscopy. The experimentally observed dispersion shows a rich spectrum of modes corresponding to different magnetization states. These magnetization states are determined by exchange and dipolar interaction between individual islands, as is confirmed by a semianalytical model. In the low field regime below 400 Oe a hysteretic behavior in the mode spectrum is found. Micromagnetic simulations reveal that the origin of the observed spectra is due to the initialization of different magnetization states of individual nanomagnets. Our results indicate that it might be possible to determine the spin-ice state by resonance experiments and are a first step towards the understanding of artificial geometrically frustrated magnetic systems in the high-frequency regime.
Artificial square spin ices are structures composed of magnetic elements arranged on a geometrically frustrated lattice and located on the sites of a two-dimensional square lattice, such that there are four interacting magnetic elements at each vertex. Using a semi-analytical approach, we show that square spin ices exhibit a rich spin wave band structure that is tunable both by external magnetic fields and the configuration of individual elements. Internal degrees of freedom can give rise to equilibrium states with bent magnetization at the edges leading to characteristic excitations; in the presence of magnetostatic interactions these form separate bands analogous to impurity bands in semiconductors. Full-scale micromagnetic simulations corroborate our semi-analytical approach. Our results show that artificial square spin ices can be viewed as reconfigurable and tunable magnonic crystals that can be used as metamaterials for spin-wave-based applications at the nanoscale.
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