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Register a new userTowards an Engineering Framework for Ultrafast Quantum Nonlinear Optics
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Added by
Ryotatsu Yanagimoto
Publication date
2021
fields
Physics
and research's language is
English
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The advent of dispersion-engineered and highly nonlinear nanophotonics is expected to open up an all-optical path towards the strong-interaction regime of quantum optics by combining high transverse field confinement with ultra-short-pulse operation. Obtaining a full understanding of photon dynamics in such broadband devices, however, poses major challenges in the modeling and simulation of multimode non-Gaussian quantum physics, highlighting the need for sophisticated reduced models that facilitate efficient numerical study while providing useful physical insight. In this manuscript, we review our recent efforts in modeling broadband optical systems at varying levels of abstraction and generality, ranging from multimode extensions of quantum input-output theory for sync-pumped oscillators to the development of numerical methods based on a field-theoretic description of nonlinear waveguides. We expect our work not only to guide ongoing theoretical and experimental efforts towards next-generation quantum devices but also to uncover essential physics of broadband quantum photonics.
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Ultra-short pulses propagating in nonlinear nanophotonic waveguides can simultaneously leverage both temporal and spatial field confinement, promising a route towards single-photon nonlinearities in an all-photonic platform. In this multimode quantum regime, however, faithful numerical simulations of pulse dynamics naively require a representation of the state in an exponentially large Hilbert space. Here, we employ a time-domain, matrix product state (MPS) representation to enable efficient simulations by exploiting the entanglement structure of the system. In order to extract physical insight from these simulations, we develop an algorithm to unravel the MPS quantum state into constituent temporal supermodes, enabling, e.g., access to the phase-space portraits of arbitrary pulse waveforms. As a demonstration, we perform exact numerical simulations of a Kerr soliton in the quantum regime. We observe the development of non-classical Wigner-function negativity in the solitonic mode as well as quantum corrections to the semiclassical dynamics of the pulse. A similar analysis of $chi^{(2)}$ simultons reveals a unique entanglement structure between the fundamental and second harmonic. Our approach is also readily compatible with quantum trajectory theory, allowing full quantum treatment of propagation loss and decoherence. We expect this work to establish the MPS technique as part of a unified engineering framework for the emerging field of broadband quantum photonics.
We present a detailed analysis of strongly driven spontaneous four-wave mixing in a lossy integrated microring resonator side-coupled to a channel waveguide. A nonperturbative, analytic solution within the undepleted pump approximation is developed for a cw pump input of arbitrary intensity. In the strongly driven regime self- and cross-phase modulation, as well as multi-pair generation, lead to a rich variety of power-dependent effects; the results are markedly different than in the low power limit. The photon pair generation rate, single photon spectrum, and joint spectral intensity (JSI) distribution are calculated. Splitting of the generated single photon spectrum into a doublet structure associated with both pump detuning and cross-phase modulation is predicted, as well as substantial narrowing of the generated signal and idler bandwidths associated with the onset of optical parametric oscillation at intermediate powers. Both the correlated and uncorrelated contributions to the JSI are calculated, and for sufficient powers the uncorrelated part of the JSI is found to form a quadruplet structure. The pump detuning is found to play a crucial role in all of these phenomena, and a critical detuning is identified which divides the system behaviour into distinct regimes, as well as an optimal detuning strategy which preserves many of the low-power characteristics of the generated photons for arbitrary input power.
Strong nonlinear interactions between photons enable logic operations for both classical and quantum-information technology. Unfortunately, nonlinear interactions are usually feeble and therefore all-optical logic gates tend to be inefficient. A quantum emitter deterministically coupled to a propagating mode fundamentally changes the situation, since each photon inevitably interacts with the emitter, and highly correlated many-photon states may be created . Here we show that a single quantum dot in a photonic-crystal waveguide can be utilized as a giant nonlinearity sensitive at the single-photon level. The nonlinear response is revealed from the intensity and quantum statistics of the scattered photons, and contains contributions from an entangled photon-photon bound state. The quantum nonlinearity will find immediate applications for deterministic Bell-state measurements and single-photon transistors and paves the way to scalable waveguide-based photonic quantum-computing architectures.
We investigate quantum nonlinear effects at a level of individual quanta in a double tripod atom-light coupling scheme involving two atomic Rydberg states. In such a scheme the slow light coherently coupled to strongly interacting Rydberg states represents a two-component or spinor light. The scheme provides additional possibilities for the control and manipulation of light quanta. A distinctive feature of the proposed setup is that it combines the spin-orbit coupling for the spinor slow light with an interaction between the photons, enabling generation of the second probe beam even when two-photon detuning is zero. Furthermore, the interaction between the photons can become repulsive if the one-photon detunings have opposite signs. This is different from a single ladder atom-light coupling scheme, in which the interaction between the photons is attractive for both positive and negative detunings, as long as the Rabi frequency of the control beam is not too large.
Multi-photon quantum interference is the underlying principle for optical quantum information processing protocols. Indistinguishability is the key to quantum interference. Therefore, the success of many protocols in optical quantum information processing relies on the availability of photon states with a well-defined spatial and temporal mode. Photons in single spatial mode can be obtained from nonlinear processes in single-mode waveguides. For the temporal mode, the common approach is to engineer the nonlinear processes. But it is complicated because the spectral properties and the nonlinear interaction are often intertwined through phase matching condition. In this paper, we study a different approach which is based on an SU(1,1) nonlinear interferometer with a pulsed pump and a controllable linear spectral phase shift for precise engineering. We systematically analyze the important figures of merit such as modal purity and heralding efficiency to investigate the feasibility of this approach. Specifically, we analyze in detail the requirement on the spectral phase engineering to optimize the figures of merit and apply numerical simulations to a fiber system. Both modal purity and efficiency are improved simultaneously. Furthermore, a novel multi-stage nonlinear interferometer is proposed and shown to achieve more precise state engineering for near-ideal single-mode operation and near-unity efficiency. We also extend the study to the case of high gain in the four-wave mixing process for the spectral engineering of quantum entanglement in continuous variables. Our investigation provides a new approach for precisely tailoring the spectral property of quantum light sources, especially, photon pairs can be engineered to simultaneously possess the features of high purity, high collection efficiency, high brightness, and high flexibility in wavelength and bandwidth selection.
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